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Showing papers on "Synchrotron radiation published in 2017"


Journal ArticleDOI
TL;DR: The beamline design and its performance allow for a highly productive and precise use of the ARPES technique at an energy resolution of 10-15 meV for fast k-space mapping studies with a photon flux up to 2 ⋅ 1013 ph/s and well below 3 mev for high resolution spectra.
Abstract: A synchrotron radiation beamline in the photon energy range of 18-240 eV and an electron spectroscopy end station have been constructed at the 3 GeV Diamond Light Source storage ring. The instrument features a variable polarisation undulator, a high resolution monochromator, a re-focussing system to form a beam spot of 50 × 50 μm2, and an end station for angle-resolved photoelectron spectroscopy (ARPES) including a 6-degrees-of-freedom cryogenic sample manipulator. The beamline design and its performance allow for a highly productive and precise use of the ARPES technique at an energy resolution of 10-15 meV for fast k-space mapping studies with a photon flux up to 2 ⋅ 1013 ph/s and well below 3 meV for high resolution spectra.

118 citations


Journal ArticleDOI
27 Jul 2017-Nature
TL;DR: The authors' measurements probe the structure of the magnetic field at an early stage of the jet, closer to its central black hole, and show that the prompt phase is produced via fast-cooling synchrotron radiation in a large-scale magnetic field that is advected from the black hole and distorted by dissipation processes within the jet.
Abstract: Newly formed black holes of stellar mass launch collimated outflows (jets) of ionized matter that approach the speed of light. These outflows power prompt, brief and intense flashes of γ-rays known as γ-ray bursts (GRBs), followed by longer-lived afterglow radiation that is detected across the electromagnetic spectrum. Measuring the polarization of the observed GRB radiation provides a direct probe of the magnetic fields in the collimated jets. Rapid-response polarimetric observations of newly discovered bursts have probed the initial afterglow phase, and show that, minutes after the prompt emission has ended, the degree of linear polarization can be as high as 30 per cent-consistent with the idea that a stable, globally ordered magnetic field permeates the jet at large distances from the central source. By contrast, optical and γ-ray observations during the prompt phase have led to discordant and often controversial results, and no definitive conclusions have been reached regarding the origin of the prompt radiation or the configuration of the magnetic field. Here we report the detection of substantial (8.3 ± 0.8 per cent from our most conservative simulation), variable linear polarization of a prompt optical flash that accompanied the extremely energetic and long-lived prompt γ-ray emission from GRB 160625B. Our measurements probe the structure of the magnetic field at an early stage of the jet, closer to its central black hole, and show that the prompt phase is produced via fast-cooling synchrotron radiation in a large-scale magnetic field that is advected from the black hole and distorted by dissipation processes within the jet.

118 citations


Journal ArticleDOI
TL;DR: The MHz repetition rates of synchrotron X-ray pulses combined with indirectX-ray detection is exploited to demonstrate the potential of XPCI with millions of frames per second multiple-frame recording, which allows for the visualization of aperiodic or stochastic transient processes which are impossible to be realized using single-shot or stroboscopic X PCI.
Abstract: Third generation synchrotron light sources offer high photon flux, partial spatial coherence, and ~10-10 s pulse widths. These enable hard X-ray phase-contrast imaging (XPCI) with single-bunch temporal resolutions. In this work, we exploited the MHz repetition rates of synchrotron X-ray pulses combined with indirect X-ray detection to demonstrate the potential of XPCI with millions of frames per second multiple-frame recording. This allows for the visualization of aperiodic or stochastic transient processes which are impossible to be realized using single-shot or stroboscopic XPCI. We present observations of various phenomena, such as crack tip propagation in glass, shock wave propagation in water and explosion during electric arc ignition, which evolve in the order of km/s (µm/ns).

80 citations


Journal ArticleDOI
TL;DR: In this article, the authors present a model for bow-shaking pulsar wind nebulae with bow shocks (BSPWNe) and estimate their contribution to the positron flux observed at the Earth.
Abstract: Pulsars with high spin-down power produce relativistic winds radiating a non-negligible fraction of this power over the whole electromagnetic range from radio to gamma-rays in the pulsar wind nebulae (PWNe). The rest of the power is dissipated in the interactions of the PWNe with the ambient interstellar medium (ISM). Some of the PWNe are moving relative to the ambient ISM with supersonic speeds producing bow shocks. In this case, the ultrarelativistic particles accelerated at the termination surface of the pulsar wind may undergo reacceleration in the converging flow system formed by the plasma outflowing from the wind termination shock and the plasma inflowing from the bow shock. The presence of magnetic perturbations in the flow, produced by instabilities induced by the accelerated particles themselves, is essential for the process to work. A generic outcome of this type of reacceleration is the creation of particle distributions with very hard spectra, such as are indeed required to explain the observed spectra of synchrotron radiation with photon indices $\varGamma\lesssim 1.5$ . The presence of this hard spectral component is specific to PWNe with bow shocks (BSPWNe). The accelerated particles, mainly electrons and positrons, may end up containing a substantial fraction of the shock ram pressure. In addition, for typical ISM and pulsar parameters, the $e^{+}$ released by these systems in the Galaxy are numerous enough to contribute a substantial fraction of the positrons detected as cosmic ray (CR) particles above few tens of GeV and up to several hundred GeV. The escape of ultrarelativistic particles from a BSPWN—and hence, its appearance in the far-UV and X-ray bands—is determined by the relative directions of the interstellar magnetic field, the velocity of the astrosphere and the pulsar rotation axis. In this respect we review the observed appearance and multiwavelength spectra of three different types of BSPWNe: PSR J0437-4715, the Guitar and Lighthouse nebulae, and Vela-like objects. We argue that high resolution imaging of such objects provides unique information both on pulsar winds and on the ISM. We discuss the interpretation of imaging observations in the context of the model outlined above and estimate the BSPWN contribution to the positron flux observed at the Earth.

75 citations


Journal ArticleDOI
TL;DR: An end-station for X-ray Raman scattering spectroscopy at beamline ID20 of the European Synchrotron Radiation Facility is described, dedicated to the study of shallow core electronic excitations using non-resonant inelasticX-ray scattering.
Abstract: An end-station for X-ray Raman scattering spectroscopy at beamline ID20 of the European Synchrotron Radiation Facility is described. This end-station is dedicated to the study of shallow core electronic excitations using non-resonant inelastic X-ray scattering. The spectrometer has 72 spherically bent analyzer crystals arranged in six modular groups of 12 analyzer crystals each for a combined maximum flexibility and large solid angle of detection. Each of the six analyzer modules houses one pixelated area detector allowing for X-ray Raman scattering based imaging and efficient separation of the desired signal from the sample and spurious scattering from the often used complicated sample environments. This new end-station provides an unprecedented instrument for X-ray Raman scattering, which is a spectroscopic tool of great interest for the study of low-energy X-ray absorption spectra in materials under in situ conditions, such as in operando batteries and fuel cells, in situ catalytic reactions, and extreme pressure and temperature conditions.

71 citations


Journal ArticleDOI
TL;DR: Beniamini et al. as discussed by the authors considered a model for the prompt phase of Gamma-Ray Burst (GRB) emission arising from a magnetized jet undergoing gradual energy dissipation due to magnetic reconnection.
Abstract: We considered a model for the prompt phase of Gamma-Ray Burst (GRB) emission arising from a magnetized jet undergoing gradual energy dissipation due to magnetic reconnection. The dissipated magnetic energy is translated to bulk kinetic energy and to acceleration of particles. The energy in these particles is released via synchrotron radiation as they gyrate around the strong magnetic fields in the jet. At small radii, the optical depth is large, and the radiation is reprocessed through Comptonization into a narrow, strongly peaked, component. At larger distances the optical depth becomes small and radiation escapes the jet with a non-thermal distribution. The obtained spectra typically peak around $\approx 300$keV (as observed) and with spectral indices below and above the peak that are, for a broad range of the model parameters, close to the observed values. The small radius of dissipation causes the emission to become self absorbed at a few keV and can sufficiently suppress the optical and X-ray fluxes within the limits required by observations (Beniamini & Piran 2014).

71 citations


Journal ArticleDOI
TL;DR: It is demonstrated here that spatially resolved microfocus infrared spectroscopy using synchrotron radiation can be applied in conjunction with periodic density functional theory calculations to predict spectral changes or to extract information on structural changes that occur as a consequence of bending.
Abstract: The range of unit cell orientations generated at the kink of a bent single crystal poses unsurmountable challenges with diffraction analysis and limits the insight into the molecular-scale mechanism of bending. On a plastically bent crystal of hexachlorobenzene, it is demonstrated here that spatially resolved microfocus infrared spectroscopy using synchrotron radiation can be applied in conjunction with periodic density functional theory calculations to predict spectral changes or to extract information on structural changes that occur as a consequence of bending. The approach reproduces well the observed trends, such as the wall effects, and provides estimations of the vibrational shifts, unit cell deformations, and intramolecular parameters. Generally, expansion of the lattice induces red-shift while compression induces larger blue-shift of the characteristic ν(C–C) and ν(C–Cl) modes. Uniform or non-uniform expansion or contraction of the unit cell of 0.1 A results in shifts of several cm–1, whereas def...

56 citations



Journal ArticleDOI
02 Jun 2017-Polymer
TL;DR: In this paper, three distinct features of the structure evolution are observed in temperature space, which can be described with three different deformation models, namely amorphization, crystalline block slip and melt recrystallization, respectively.

52 citations


Journal ArticleDOI
TL;DR: In this paper, a gyrotron-like undulator with a period down to submillimetre level based on a spontaneous electric field that is driven by a femtosecond laser was proposed.
Abstract: The capability of synchrotron radiation to produce ultrabright emission has attracted considerable interest over the last half a century. To date, magnetic undulators with a period of several centimetres are commonly used for wiggling relativistic electrons in a modulated field. Here, we propose a novel compact undulator with a period down to the submillimetre level based on a spontaneous electric field that is driven by a femtosecond laser. Both the guided energetic electrons and the gyrotron-like undulator are spontaneously produced by irradiating a thin metallic wire with an intense laser pulse. An intense radial electric field instantaneously created on the wire can guide the electrons' helical motion along the wire and induce periodic THz emission. We have demonstrated that this scheme can produce intense THz sources with a conversion efficiency of 1% that are frequency-tunable by adjusting the diameter of the wire. Amplified emission of THz radiation by more than tenfold has been observed.

51 citations


Journal ArticleDOI
TL;DR: The photon-ion merged-beams technique for photoionization of mass/charge selected ionized atoms, molecules and clusters by x-rays from synchrotron radiation sources is introduced in this article.
Abstract: The photon-ion merged-beams technique for the photoionization of mass/charge selected ionized atoms, molecules and clusters by x-rays from synchrotron radiation sources is introduced. Examples for photoionization of atomic ions are discussed by going from outer-shell ionization of simple few-electron systems to inner-shell ionization of complex many-electron ions. Fundamental ionization mechanisms are elucidated and the importance of the results for applications in astrophysics and plasma physics is pointed out. Finally, the unique capabilities of the photon-ion merged-beams technique for the study of photoabsorption by nanoparticles are demonstrated by the example of endohedral fullerene ions.

BookDOI
20 Mar 2017
TL;DR: In this article, the authors present new and emerging methods of materials characterization in the field of 3D characterization techniques like three-dimensional X-ray diffraction microscopy, as well as direct imaging and tomography.
Abstract: The second part then focuses on such characterization techniques as diffraction and scattering methods, as well as direct imaging and tomography. The third part presents new and emerging methods of materials characterization in the field of 3D characterization techniques like three-dimensional X-ray diffraction microscopy. The fourth and final part is a collection of examples that demonstrate the application of the methods introduced in the first parts to problems in materials science.

Journal ArticleDOI
TL;DR: In this paper, a non-resonant acceleration mechanism arising from the second adiabatic invariant in magnetic turbulence was introduced to study the prompt emission spectra of gamma-ray bursts (GRBs).
Abstract: We introduce a non-resonant acceleration mechanism arising from the second adiabatic invariant in magnetic turbulence and apply it to study the prompt emission spectra of gamma-ray bursts (GRBs). The mechanism contains both the first- and second-order Fermi acceleration, originating from the interacting turbulent reconnection and dynamo processes. It leads to a hard electron energy distribution up to a cutoff energy at the balance between the acceleration and synchrotron cooling. The sufficient acceleration rate ensures a rapid hardening of any initial energy distribution to a power-law distribution with the index $p \sim 1$, which naturally produces a low-energy photon index $\alpha \sim -1$ via the synchrotron radiation. For typical GRB parameters, the synchrotron emission can extend to a characteristic photon energy on the order of $\sim 100$ keV.

Journal ArticleDOI
TL;DR: A novel technique is proposed for directly imprinting strong coherent microbunching on the electron beam with very small laser-induced energy spread and it is demonstrated that this technique can be used for the generation of megawatt-scale level, fully temporal coherent femtosecond EUV and soft x-ray radiation pulses at a storage ring light source.
Abstract: Generation of ultrashort coherent radiation pulses in the extreme ultraviolet (EUV) and x-ray regime is of remarkable interest in the synchrotron radiation user community. In this work, a novel technique is proposed for directly imprinting strong coherent microbunching on the electron beam with very small laser-induced energy spread. Theoretical analysis and numerical simulations demonstrated that this technique can be used for the generation of megawatt-scale level, fully temporal coherent femtosecond EUV and soft x-ray radiation pulses at a storage ring light source.

Journal ArticleDOI
TL;DR: In this article, the authors investigated the contribution of thermal, non-accelerated electrons to synchrotron absorption and emission in the standard afterglow model, and showed that these thermal electrons provided an additional source of opacity, and yield an additional emission component at higher energies.
Abstract: To date, nearly all multi-wavelength modeling of long-duration gamma-ray bursts has ignored synchrotron radiation from the significant population of electrons expected to pass the shock without acceleration into a power-law distribution. We investigate the effect of including the contribution of thermal, non-accelerated electrons to synchrotron absorption and emission in the standard afterglow model, and show that these thermal electrons provide an additional source of opacity to synchrotron self-absorption, and yield an additional emission component at higher energies. The extra opacity results in an increase in the synchrotron self-absorption frequency by factors of 10--100 for fiducial parameters. The nature of the additional emission depends on the details of the thermal population, but is generally observed to yield a spectral peak in the optical brighter than radiation from the nonthermal population by similar factors a few seconds after the burst, remaining detectable at millimeter and radio frequencies several days later.

Journal ArticleDOI
TL;DR: In this article, the authors presented multi-wavelength polarization predictions for rotation-powered pulsars and showed that measurements over a range of frequencies can be particularly important for constraining the emission location, radiation mechanisms, and system geometry.
Abstract: Polarization measurements provide strong constraints on models for emission from rotation-powered pulsars. We present multiwavelength polarization predictions showing that measurements over a range of frequencies can be particularly important for constraining the emission location, radiation mechanisms, and system geometry. The results assume a generic model for emission from the outer magnetosphere and current sheet in which optical to hard X-ray emission is produced by synchrotron radiation (SR) from electron-positron pairs and gamma-ray emission is produced by curvature radiation (CR) or SR from accelerating primary electrons. The magnetic field structure of a force-free magnetosphere is assumed and the phase-resolved and phase-averaged polarization is calculated in the frame of an inertial observer. We find that large position angle (PA) swings and deep depolarization dips occur during the light-curve peaks in all energy bands. For synchrotron emission, the polarization characteristics are strongly dependent on photon emission radius with larger, nearly 180deg, PA swings for emission outside the light cylinder (LC)‚ as the line of sight crosses the current sheet. The phase-averaged polarization degree for SR is less that 10% and around 20% for emission starting inside and outside the LC, respectively, while the polarization degree for CR is much larger, up to 40%-60%. Observing a sharp increase in polarization degree and a change in PA at the transition between X-ray and gamma-ray spectral components would indicate that CR is the gamma-ray emission mechanism.

Journal ArticleDOI
TL;DR: A rotatable high-resolution angle-resolved photoemission spectroscopy system that utilizes tunable linear-polarization geometries on the linear undulator beamline BL-1 at Hiroshima Synchrotron Radiation Center is described.
Abstract: A rotatable high-resolution angle-resolved photoemission spectroscopy (ARPES) system has been developed to utilize tunable linear-polarization geometries on the linear undulator beamline (BL-1) at Hiroshima Synchrotron Radiation Center. By rotating the whole ARPES measurement system, the photoelectron detection plane can be continuously changed from parallel to normal against the electric field vector of linearly polarized undulator radiation. This polarization tunability enables us to identify the symmetry of the initial electronic states with respect to the mirror planes, and to selectively observe the electronic states based on the dipole selection rule in the photoemission process. Specifications of the rotatable high-resolution ARPES system are described, as well as its capabilities with some representative experimental results.

Journal ArticleDOI
TL;DR: In this paper, a companion orbiting a primary black hole and perturbing its relativistic jet is considered, and the effects of repeated magneto-hydrodynamic stresses along the jet's inner electron acceleration and radiative processes are investigated.
Abstract: We study particle acceleration and radiative processes in Blazar jets under recurring conditions set by gravitational perturbations in supermassive binary systems. We consider the action from a companion orbiting a primary black hole of $\sim 10^8 \, M_{\odot}$, and perturbing its relativistic jet. We discuss how such conditions induce repetitive magneto-hydrodynamic stresses along the jet, and affect its inner electron acceleration and radiative processes. Specifically, we study how macroscopic perturbations related to increased jet "magnetization" end up into higher radiative outputs in the optical, X-ray and gamma-ray bands. We find first an increase in magnetic field strength as gauged in the optical band from the Synchrotron emission of electrons accelerated in kinetic processes stimulated by reconnecting magnetic lines. The energetic electrons then proceed to up-scatter the Synchrotron photons to GeV energies after the canonical Synchrotron-Self Compton radiation process. Our model implies a specific, recurring pattern in the optical to gamma-ray emissions, made of high peaks and wide troughs. Progressing accelerations caused by spreading reconnections will produce an additional Synchrotron keV component. Such outbursts provide a diagnostics for enhanced acceleration of electrons which can up-scatter photons into the TeV range. We discuss how our model applies to the BL Lac object PG 1553+113, arguably the best candidate to now for high amplitude, recurring modulations in its gamma-ray emissions. We also consider other BL Lacs showing correlated keV - TeV radiations such as Mrk 421.

Journal ArticleDOI
TL;DR: A review of the technical and scientific aspects of scintillators used in synchrotron radiation (i.e., storage rings and x-ray free-electron lasers) can be found in this paper.
Abstract: Indirect detection is a versatile way to detect hard x-rays. It is based on an x-ray-to-light converter, optical coupling, and a visible light detector. The converter screen, known as a scintillator, is deployed in both imaging and point detection, using either signal integration or counting. Two applications are explored in this review—sample examination and x-ray beam diagnostics for synchrotron sources. A large variety of scintillators are available to fulfill the needs of synchrotron applications. High dynamic range, small pixel size, and radiation hardness are the major advantages of scintillators. This article provides a review of the technical and scientific aspects of scintillators used in synchrotron radiation (i.e., storage rings and x-ray free-electron lasers). The advantages and drawbacks of implementation of the most popular scintillators on synchrotron beamlines are described.

Journal ArticleDOI
TL;DR: In this paper, the potential of Near Ambient Pressure XPS (NAP-XPS) for the estimation of the surface electronic structure of electrochemically active interfaces is discussed.

Journal ArticleDOI
TL;DR: A review of recent developments in polymer applications of synchrotron SAXS is presented in this article, where the authors review the progress in data analyses from the following aspects: ultra-small-angle X-ray scattering, anomalous SAXs, X -ray photon correlation spectroscopy, new types of simultaneous measurements, grazing-incidence SA XS, new trends in nanoparticle analyses and industrial applications.
Abstract: Synchrotron radiation facilities have been established and become very familiar in the polymer community not only from academic but also industrial viewpoints. It is not so unusual now to conduct simultaneous measurements of small-angle X-ray scattering (SAXS) with other techniques such as wide-angle X-ray scattering, stress–strain, light scattering, and so forth. New techniques have also been established and have become more familiar in recent years. In this review, recent developments in polymer applications of synchrotron SAXS are summarized. Instrumental developments and progress in data analyses are reviewed from the following aspects: ultra-small-angle X-ray scattering, anomalous SAXS, X-ray photon correlation spectroscopy, new types of simultaneous measurements, grazing-incidence SAXS, new trends in nanoparticle analyses and industrial applications. © 2016 Society of Chemical Industry

Journal ArticleDOI
TL;DR: The first direct observation of these pulse shapes with a few picoseconds resolution, and of their dynamics over a long time, confirm in a very direct way the theories predicting an interplay between two physical processes.
Abstract: In recent synchrotron radiation facilities, the use of short (picosecond) electron bunches is a powerful method for producing giant pulses of terahertz coherent synchrotron radiation. Here we report on the first direct observation of these pulse shapes with a few picoseconds resolution, and of their dynamics over a long time. We thus confirm in a very direct way the theories predicting an interplay between two physical processes. Below a critical bunch charge, we observe a train of identical THz pulses (a broadband Terahertz comb) stemming from the shortness of the electron bunches. Above this threshold, a large part of the emission is dominated by drifting structures, which appear through spontaneous self-organization. These challenging single-shot THz recordings are made possible by using a recently developed photonic time stretch detector with a high sensitivity. The experiment has been realized at the SOLEIL storage ring.

Journal ArticleDOI
TL;DR: In this article, a brief introduction on hydrogen storage materials, X-ray powder diffraction (XRPD), and synchrotron radiation light source is given, and the applications of ex situ and in situ time-resolved SR-X-RPD in hydrogen storage material, are reviewed in detail.

Journal ArticleDOI
TL;DR: The world’s first dedicated synchrotron instrument for long-duration experiments has been built and commissioned at Diamond Light Source, designed for the study of slow kinetics in polycrystalline materials.
Abstract: A new synchrotron X-ray powder diffraction instrument has been built and commissioned for long-duration experiments on beamline I11 at Diamond Light Source. The concept is unique, with design features to house multiple experiments running in parallel, in particular with specific stages for sample environments to study slow kinetic systems or processes. The instrument benefits from a high-brightness X-ray beam and a large area detector. Diffraction data from the commissioning work have shown that the objectives and criteria are met. Supported by two case studies, the results from months of measurements have demonstrated the viability of this large-scale instrument, which is the world's first dedicated facility for long-term studies (weeks to years) using synchrotron radiation.

Journal ArticleDOI
TL;DR: In this article, the European Synchrotron Radiation Facility (ESRF) provided beam time and the ID03 staff for technical assistance, and the authors gratefully acknowledge financial support by the Deutsche Forschungsgemeinschaft viaMA1618/13 andMA 1618/20.
Abstract: We thank the European Synchrotron Radiation Facility for providing beam time and the ID03 staff for technical assistance. MR, FR, BR, JS, and OMM gratefully acknowledge financial support by the Deutsche Forschungsgemeinschaft viaMA1618/13 andMA1618/20. DAH thanks NSERC for financial support.

Journal ArticleDOI
TL;DR: In this article, the authors used the SOFT (Synchrotron-detecting Orbit Following Toolkit) to simulate synchrotor images and spectra using Fokker-Planck simulations for parameters from an Alcator C-Mod discharge.
Abstract: Improved understanding of the dynamics of runaway electrons can be obtained by measurement and interpretation of their synchrotron radiation emission. Models for synchrotron radiation emitted by relativistic electrons are well established, but the question of how various geometric effects -- such as magnetic field inhomogeneity and camera placement -- influence the synchrotron measurements and their interpretation remains open. In this paper we address this issue by simulating synchrotron images and spectra using the new synthetic synchrotron diagnostic tool SOFT (Synchrotron-detecting Orbit Following Toolkit). We identify the key parameters influencing the synchrotron radiation spot and present scans in those parameters. Using a runaway electron distribution function obtained by Fokker-Planck simulations for parameters from an Alcator C-Mod discharge, we demonstrate that the corresponding synchrotron image is well-reproduced by SOFT simulations, and we explain how it can be understood in terms of the parameter scans. Geometric effects are shown to significantly influence the synchrotron spectrum, and we show that inherent inconsistencies in a simple emission model (i.e. not modeling detection) can lead to incorrect interpretation of the images.

Journal ArticleDOI
TL;DR: In this article, the impact of the presence of inhomogeneities or clumps in the stellar wind on the high-energy non-thermal radiation of high-mass binaries hosting a non-accreting pulsar was studied.
Abstract: Context. Binaries hosting a massive star and a non-accreting pulsar are powerful non-thermal emitters owing to the interaction of the pulsar and the stellar wind. The winds of massive stars are thought to be inhomogeneous, which could have an impact on the non-thermal emission.Aims. We study numerically the impact of the presence of inhomogeneities or clumps in the stellar wind on the high-energy non-thermal radiation of high-mass binaries hosting a non-accreting pulsar.Methods. We compute the trajectories and physical properties of the streamlines in the shocked pulsar wind without clumps, with a small clump, and with a large clump. This information is used to characterize the injection and the steady state distribution of non-thermal particles accelerated at shocks formed in the pulsar wind. The synchrotron and inverse Compton emission from these non-thermal particles is calculated, accounting also for the effect of gamma-ray absorption through pair creation. A specific study is done for PSR B1259-63/LS2883.Results. When stellar wind clumps perturb the two-wind interaction region, the associated non-thermal radiation in the X-ray band, of synchrotron origin, and in the GeV–TeV band, of inverse Compton origin, is affected by several equally important effects: (i) strong changes in the plasma velocity direction that result in Doppler boosting factor variations; (ii) strengthening of the magnetic field that mainly enhances the synchrotron radiation; (iii) strengthening of the pulsar wind kinetic energy dissipation at the shock, potentially available for particle acceleration; and (iv) changes in the rate of adiabatic losses that affect the lower energy part of the non-thermal particle population. The radiation above 100 GeV detected, presumably, during the post-periastron crossing of the Be star disc in PSR B1259-63/LS2883, can be roughly reproduced assuming that the crossing of the disc is modelled as the encounter with a large inhomogeneity.Conclusions. Because of the likely diverse nature of clumps in the stellar wind, and hydrodynamical instabilities, the non-thermal radiation of high-mass binaries with a non-accreting pulsar is expected to be boosted somewhat chaotically, and to present different superimposed variability patterns. Some of the observed variability in gamma rays from PSR B1259-63/LS2883 is qualitatively reproduced by our calculations.

Journal ArticleDOI
TL;DR: A portable double-sided pulsed laser heating system for diamond anvil cells has been developed that is able to stably produce laser pulses as short as a few microseconds with repetition frequencies up to 100 kHz.
Abstract: A portable double-sided pulsed laser heating system for diamond anvil cells has been developed that is able to stably produce laser pulses as short as a few microseconds with repetition frequencies up to 100 kHz. In situ temperature determination is possible by collecting and fitting the thermal radiation spectrum for a specific wavelength range (particularly, between 650 nm and 850 nm) to the Planck radiation function. Surface temperature information can also be time-resolved by using a gated detector that is synchronized with the laser pulse modulation and space-resolved with the implementation of a multi-point thermal radiation collection technique. The system can be easily coupled with equipment at synchrotron facilities, particularly for nuclear resonance spectroscopy experiments. Examples of applications include investigations of high-pressure high-temperature behavior of iron oxides, both in house and at the European Synchrotron Radiation Facility using the synchrotron Mossbauer source and nuclear inelastic scattering.

Journal ArticleDOI
TL;DR: The influence of the properties of the radiation source, such as the electron bunch shape and spectral bandwidth of the emitted radiation, on near-field infrared spectra of silicon-carbide (SiC) is investigated to exploit the full potential of nano-FTIR spectroscopy.
Abstract: Synchrotron radiation-based nano-FTIR spectroscopy utilizes the highly brilliant and ultra-broadband infrared (IR) radiation provided by electron storage rings for the infrared spectroscopic characterization of samples at the nanoscale. In order to exploit the full potential of this approach we investigated the influence of the properties of the radiation source, such as the electron bunch shape and spectral bandwidth of the emitted radiation, on near-field infrared spectra of silicon-carbide (SiC). The adapted configuration of the storage ring optics enables a modification of the transverse electron bunch profile allowing an increase of the measured near-field signal amplitude. Additionally, the decay of the signal amplitude due to the decreasing storage ring current is also eliminated. Further options for improving the sensitivity of nano-FTIR spectroscopy, which can also be applied to other broadband radiation sources, are the adaption of the spectral bandwidth to the wavelength range of interest or the use of polarization optics. The sensitivity enhancement emerging from these options is verified by comparing near-field spectra collected from crystalline SiC samples. The improvement in sensitivity by combining these approaches is demonstrated by acquiring nano-FTIR spectra from thin organic films, which show weak resonances in the IR-regime.

Journal ArticleDOI
TL;DR: In this article, it was shown that the synchrotron radiation should be anisotropic when the angular distribution of accelerated electrons has a preferable orientation, and this anisotropy would naturally lead to a steeper decay for the high-latitude emission if the intrinsic emission is limb-brightened.
Abstract: When an emitting spherical shell with a constant Lorentz factor turns off emission abruptly at some radii, its high-latitude emission would obey the relation of (the temporal index) = (the spectral index). However, this relation is violated by the X-ray fares in some gamma-ray bursts (GRBs), whose is much more steeper. We show that the synchrotron radiation should be anisotropic when the angular distribution of accelerated electrons has a preferable orientation, and this anisotropy would naturally lead to a steeper decay for the high-latitude emission if the intrinsic emission is limb-brightened. We use this simple toy model to reproduce the temporal and spectral evolution of X-ray flares. We show that our model can well interpret the steep decay of the X-ray flares in the three GRBs selected as an example. Recent simulations on particle acceleration may support the specific anisotropic distribution of the electrons adopted in our work. Reversely, confirmation of the anisotropy in the radiation would provide meaningful clues to the details of electron acceleration in the emitting region.