2D Layered Materials: Synthesis, Nonlinear Optical Properties, and Device Applications

Solitons are stable localized wave packets that can propagate long distance in dispersive media without changing their shapes. As particle-like nonlinear localized waves, solitons have been investigated in different physical systems. Owing to potential applications in optical communication and optical signal processing systems, optical solitons have attracted intense interest in the past three decades. To experimentally study the formation and dynamics of temporal optical solitons, fiber lasers are considered as a wonderful nonlinear system. During the last decade, several kinds of theoretically predicted solitons were observed experimentally in fiber lasers. In this review, we present a detailed overview of the experimentally verified optical solitons in fiber lasers, including bright solitons, dark solitons, vector solitons, dissipative solitons, dispersion-managed solitons, polarization domain wall solitons, and so on. An outlook for the development on the solitons in fiber lasers is also provided and discussed.

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Recent progress of study on optical solitons in fiber lasers

In this paper, both nonlinear saturable absorption and two-photon absorption (TPA) of few-layer molybdenum diselenide (MoSe2) were observed at 1.56 μm wavelength and further applied to mode-locked ultrafast fiber laser for the first time to our knowledge. Few-layer MoSe2 nanosheets were prepared by liquid-phase exfoliation method and characterized by x ray diffractometer, Raman spectroscopy, and atomic force microscopy. The obtained few-layer MoSe2 dispersion is further composited with a polymer material for convenient fabrication of MoSe2 thin films. Then, we investigated the nonlinear optical (NLO) absorption property of the few-layer MoSe2 film using a balanced twin-detector measurement technique. Both the saturable absorption and TPA effects of the few-layer MoSe2 film were found by increasing the input optical intensity. The saturable absorption shows a modulation depth of 0.63% and a low nonsaturable loss of ∼3.5%, corresponding to the relative modulation depth of 18%. The TPA effect occurred when the input optical intensity exceeds ∼260  MW/cm2. Furthermore, we experimentally exploit the saturable absorption of few-layer MoSe2 film to mode lock an all-fiber erbium-doped fiber laser. Stable soliton mode locking at 1558 nm center wavelength is achieved with pulse duration of 1.45 ps. It was also observed that the TPA process suppresses the mode-locking operation in the case of higher optical intensity. Our results indicate that layered MoSe2, as another two-dimensional nanomaterial, can provide excellent NLO properties (e.g., saturable absorption and TPA) for potential applications in ultrashort pulse generation and optical limiting.

Nonlinear optical absorption of few-layer molybdenum diselenide (MoSe 2 ) for passively mode-locked soliton fiber laser [Invited]

We reported on the generation of dual-wavelength rectangular pulses in a Yb-doped fiber laser (YDFL) by using a microfiber-based graphene saturable absorber (GSA). The duration of dual-wavelength rectangular pulse could be varied from 1.41 ns to 4.23 ns with the increasing pump power. With a tunable bandpass filter, it was found that the characteristics of the rectangular pulses centered at 1061.8 nm and 1068.8 nm are similar to each other. Moreover, the dual-wavelength switchable operation was also realized by properly rotating the polarization controllers (PCs). The demonstration of the dual-wavelength rectangular pulses from a YDFL would open some applications for fields such as spectroscopy, biomedicine and sensing research.

Dual-wavelength rectangular pulse Yb-doped fiber laser using a microfiber-based graphene saturable absorber.

In this paper, we first achieve nanosecond-scale dissipative soliton resonance (DSR) generation in a thulium-doped double-clad fiber (TDF) laser with all-anomalous-dispersion regime, and also first scale the average power up to 100.4 W by employing only two stage TDF amplifiers, corresponding to gains of 19.3 and 14.4 dB, respectively. It is noted that both the fiber laser oscillator and the amplification system employ double-clad fiber as the gain medium for utilizing the advantages in high-gain-availability, high-power-handling and good-mode-quality-maintaining. DSR mode-locking of the TDF oscillator is realized by using a nonlinear optical loop mirror (NOLM), which exhibits all-fiber-format, high nonlinear and passive saturable absorption properties. The TDF oscillator can deliver rectangular-shape pulses with duration ranging from ~3.74 to ~72.19 ns while maintaining a nearly equal output peak power level of ~0.56 W, namely peak power clamping (PPC) effect. Comparatively, the two stage amplifiers can scale the seeding pulses to similar average power levels, but to dramatically different peak powers ranging from ~0.94 to ~18.1 kW depending on the durations. Our TDF master-oscillator-power-amplifier (MOPA) system can provide a high power 2-μm band all-fiber-format laser source both tunable in pulse duration and peak power.

100 W dissipative soliton resonances from a thulium-doped double-clad all-fiber-format MOPA system.

We reported on the dissipative soliton resonance (DSR) phenomenon in a mode-locked Yb-doped fiber laser by using the nonlinear polarization rotation technique. It was found that the multi-pulse oscillation under high pump power could be circumvented by properly adjusting the polarization controllers, namely, the wave-breaking-free rectangular pulse in DSR region was achieved. As the DSR signature, the pulse duration varied from 8.8 ps to 22.92 ns with the increasing pump power. Correspondingly, the maximum pulse energy was 3.24 nJ. The results demonstrated that the DSR phenomenon could exist in Yb-doped fiber lasers, which could be used to achieve wave-breaking-free, ultrahigh-energy pulse.

Wave-breaking-free pulse in an all-fiber normal-dispersion Yb-doped fiber laser under dissipative soliton resonance condition.

We reported on the trapping of soliton molecule in a passively mode-locked ytterbium-doped fiber laser with a microfiber-based graphene saturable absorber (GSA). By virtue of the highly nonlinear effect of microfiber-based GSA, the multipulse formation, such as the soliton molecule, is greatly enhanced despite of the all-normal dispersion regime. Depending on the cavity parameter selections, it was found that the conventional multisoliton could be reconstructed and then evolve into the soliton molecule. The soliton molecule trapping of two polarization components with a 0.65-nm wavelength separation was observed, which propagated as a group-velocity locked vector soliton despite of the cavity birefringence. The obtained results provide an enhanced understanding of dynamics of the soliton molecule.

Lan Liu

Papers

Wave-breaking-free pulse in an all-fiber normal-dispersion Yb-doped fiber laser under dissipative soliton resonance condition.

Trapping of Soliton Molecule in a Graphene-Based Mode-Locked Ytterbium-Doped Fiber Laser