. On 11 March 2011, an earthquake occurred about 130 km off the Pacific coast of Japan's main island Honshu, followed by a large tsunami. The resulting loss of electric power at the Fukushima Dai-ichi nuclear power plant developed into a disaster causing massive release of radioactivity into the atmosphere. In this study, we determine the emissions into the atmosphere of two isotopes, the noble gas xenon-133 (133Xe) and the aerosol-bound caesium-137 (137Cs), which have very different release characteristics as well as behavior in the atmosphere. To determine radionuclide emissions as a function of height and time until 20 April, we made a first guess of release rates based on fuel inventories and documented accident events at the site. This first guess was subsequently improved by inverse modeling, which combined it with the results of an atmospheric transport model, FLEXPART, and measurement data from several dozen stations in Japan, North America and other regions. We used both atmospheric activity concentration measurements as well as, for 137Cs, measurements of bulk deposition. Regarding 133Xe, we find a total release of 15.3 (uncertainty range 12.2–18.3) EBq, which is more than twice as high as the total release from Chernobyl and likely the largest radioactive noble gas release in history. The entire noble gas inventory of reactor units 1–3 was set free into the atmosphere between 11 and 15 March 2011. In fact, our release estimate is higher than the entire estimated 133Xe inventory of the Fukushima Dai-ichi nuclear power plant, which we explain with the decay of iodine-133 (half-life of 20.8 h) into 133Xe. There is strong evidence that the 133Xe release started before the first active venting was made, possibly indicating structural damage to reactor components and/or leaks due to overpressure which would have allowed early release of noble gases. For 137Cs, the inversion results give a total emission of 36.6 (20.1–53.1) PBq, or about 43% of the estimated Chernobyl emission. Our results indicate that 137Cs emissions peaked on 14–15 March but were generally high from 12 until 19 March, when they suddenly dropped by orders of magnitude at the time when spraying of water on the spent-fuel pool of unit 4 started. This indicates that emissions may not have originated only from the damaged reactor cores, but also from the spent-fuel pool of unit 4. This would also confirm that the spraying was an effective countermeasure. We explore the main dispersion and deposition patterns of the radioactive cloud, both regionally for Japan as well as for the entire Northern Hemisphere. While at first sight it seemed fortunate that westerly winds prevailed most of the time during the accident, a different picture emerges from our detailed analysis. Exactly during and following the period of the strongest 137Cs emissions on 14 and 15 March as well as after another period with strong emissions on 19 March, the radioactive plume was advected over Eastern Honshu Island, where precipitation deposited a large fraction of 137Cs on land surfaces. Radioactive clouds reached North America on 15 March and Europe on 22 March. By middle of April, 133Xe was fairly uniformly distributed in the middle latitudes of the entire Northern Hemisphere and was for the first time also measured in the Southern Hemisphere (Darwin station, Australia). In general, simulated and observed concentrations of 133Xe and 137Cs both at Japanese as well as at remote sites were in good quantitative agreement. Altogether, we estimate that 6.4 PBq of 137Cs, or 18% of the total fallout until 20 April, were deposited over Japanese land areas, while most of the rest fell over the North Pacific Ocean. Only 0.7 PBq, or 1.9% of the total fallout were deposited on land areas other than Japan.

Xenon-133 and caesium-137 releases into the atmosphere from the Fukushima Dai-ichi nuclear power plant: determination of the source term, atmospheric dispersion, and deposition

The Hellenide orogen in Greece is part of the AlpineHimalaya mountian belt, created during the destruction of Tethys by the convergence of Gondwana and Eurasia. Within Greece, there is the record of a complete Wilson tectonic cycle of continental rifting, sea-fl oor spreading, plate subduction, and continental collision during Mesozoic and Cenozoic time. This book presents a new synthesis of the geological history of Greece as revealed by the varied igneous rocks. It is based on more than 30 years of fi eld and laboratory studies by the authors together with a synthesis of the widely scattered published literature that has been written in many different languagues. Basement rocks record Hercynian subduction and plutonism on the northern margin of Gondwana, which in the Permian and Triassic rifted into several microcontinents, thereby creating the eastern Mediterranean Neotethys ocean. Partial closure of strands of the Neotethys ocean resulted in widespread emplacement of Jurassic and Cretaceous ophiolites. Early Tertiary collision produced a Hellenide mountian chain similar to the Alps and Himalayas. Rapid Neogene extension of the Hellenides behind the modern South Aegean arc has formed the Aegean Sea, triggered widespread backarc igneous activity, and unroofed mid-crustal rocks. The geological setting, geochemistry, and tectonic signifi cance of each group of rocks is presented in detail, with numerous original maps and fi gures.

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The igneous rocks of Greece: The anatomy of an orogen. Georgia Pe-Piper and David J.W. Piper.

In environmental monitoring campaigns for anthropogenic radionuclides released in the course of the Fukushima nuclear accident (2011), most focus had been on gamma-emitting radionuclides. More than 99% of the released activity was due to radionuclides of the elements Kr, Te, I, Xe, and Cs. However, little work had been done on the monitoring of radionuclides other than 131I, 132Te, 134Cs, 136Cs, and 137Cs. Radionuclides such as those of less volatile elements (e.g., 89Sr, 90Sr, 103Ru, 106Ru, plutonium), pure beta-emitters (3H, 14C, 35S), gaseous radionuclides (85Kr, 133Xe, 135Xe) or radionuclides with very long half-lives (e.g., 36Cl, 99Tc, 129I, some actinides such as 236U) have been understudied by comparison. In this review, we summarize previous monitoring work on these “orphan” radionuclides in various environmental media and outline further challenges for future monitoring campaigns. Some of the understudied radionuclides are of radiological concern, others are promising tracers for environmental, g...

Fukushima’s Forgotten Radionuclides: A Review of the Understudied Radioactive Emissions

Climate change, vegetation history, and landscape responses on the Tibetan Plateau during the Holocene: A comprehensive review

CO2 capture and storage: A way forward for sustainable environment.

A 9-year record of stable isotope ratios of precipitation in Eastern Hungary: Implications on isotope hydrology and regional palaeoclimatology

Groundwater flow system as an archive of palaeotemperature: Noble gas, radiocarbon, stable isotope and geochemical study in the Pannonian Basin, Hungary

Using an ultrapure 4He spike in tritium measurements of environmental water samples by the 3He-ingrowth method.

In-reservoir mixing of mantle-derived CO2 and metasedimentary CH4–N2 fluids – Noble gas and stable isotope study of two multistacked fields (Pannonian Basin System, W-Hungary)

László Palcsu

Papers

A 9-year record of stable isotope ratios of precipitation in Eastern Hungary: Implications on isotope hydrology and regional palaeoclimatology

Groundwater flow system as an archive of palaeotemperature: Noble gas, radiocarbon, stable isotope and geochemical study in the Pannonian Basin, Hungary

Using an ultrapure 4He spike in tritium measurements of environmental water samples by the 3He-ingrowth method.

In-reservoir mixing of mantle-derived CO2 and metasedimentary CH4–N2 fluids – Noble gas and stable isotope study of two multistacked fields (Pannonian Basin System, W-Hungary)

Tritium and radiocarbon in the western North Pacific waters: post-Fukushima situation.