Recent developments in chip-based nonlinear photonics offer the tantalizing prospect of realizing many applications that can use optical frequency comb devices that have form factors smaller than 1 cm3 and that require less than 1 W of power. A key feature that enables such technology is the tight confinement of light due to the high refractive index contrast between the core and the cladding. This simultaneously produces high optical nonlinearities and allows for dispersion engineering to realize and phase match parametric nonlinear processes with laser-pointer powers across large spectral bandwidths. In this Review, we summarize the developments, applications and underlying physics of optical frequency comb generation in photonic-chip waveguides via supercontinuum generation and in microresonators via Kerr-comb generation that enable comb technology from the near-ultraviolet to the mid-infrared regime. This Review discusses the developments and applications of on-chip optical frequency comb generation based on two concepts—supercontinuum generation in photonic-chip waveguides and Kerr-comb generation in microresonators.

Photonic-chip-based frequency combs

Quantum technologies comprise an emerging class of devices capable of controlling superposition and entanglement of quantum states of light or matter, to realize fundamental performance advantages over ordinary classical machines. The technology of integrated quantum photonics has enabled the generation, processing and detection of quantum states of light at a steadily increasing scale and level of complexity, progressing from few-component circuitry occupying centimetre-scale footprints and operating on two photons, to programmable devices approaching 1,000 components occupying millimetre-scale footprints with integrated generation of multiphoton states. This Review summarizes the advances in integrated photonic quantum technologies and its demonstrated applications, including quantum communications, simulations of quantum chemical and physical systems, sampling algorithms, and linear-optic quantum information processing. This Review covers recent progress in integrated quantum photonics (IQP) technologies and their applications. The challenges and opportunities of realizing large-scale, monolithic IQP circuits for future quantum applications are discussed.

Integrated photonic quantum technologies

Non-magnetic non-reciprocal transparency and amplification is experimentally achieved by optomechanics using a whispering-gallery microresonator. The idea may lead to integrated all-optical isolators or non-reciprocal phase shifters.

Experimental realization of optomechanically induced non-reciprocity

We demonstrate broadband frequency comb generation in the mid-infrared (MIR) from 2.3 to 3.5 μm in a Si(3)N(4) microresonator. We engineer the dispersion of the structure in the MIR using a Sellmeier equation we derive from experimental measurements performed on Si(3)N(4) films from the UV to the IR. We use deposition-anneal cycling to decrease absorption losses due to vibrational transitions in the MIR and achieve a Q-factor of 1.0×10(6). To our knowledge, this is the highest Q reported in this wavelength range for any on-chip resonator.

Broadband mid-infrared frequency comb generation in a Si(3)N(4) microresonator.

Generations of technologies with fundamentally new information processing capabilities will emerge if microscopic physical systems can be controlled to encode, transmit, and process quantum information, at scale and with high fidelity. In the decade after its 2008 inception, the technology of integrated quantum photonics enabled the generation, processing, and detection of quantum states of light, at a steadily increasing scale and level of complexity. Using both established and advanced fabrication techniques, the field progressed from the demonstrations of fixed circuits comprising few components and operating on two photons, to programmable circuitry approaching 1000 components with integrated generation of multi-photon states. A continuation in this trend over the next decade would usher in a versatile platform for future quantum technologies. This Review summarises the advances in integrated photonic quantum technologies (materials, devices, and functionality), and its demonstrated on-chip applications including secure quantum communications, simulations of quantum physical and chemical systems, Boson sampling, and linear-optic quantum information processing.

Integrated Photonic Quantum Technologies

Quantum-photonic chips, which integrate quantum light sources alongside active and passive optical elements, as well as single-photon detectors, show great potential for photonic quantum information processing and quantum technology. Mature semiconductor nanofabrication processes allow for scaling such photonic integrated circuits to on-chip networks of increasing complexity. Second-order nonlinear materials are the method of choice for generating photonic quantum states in the overwhelming majority of linear optic experiments using bulk components, but integration with waveguide circuitry on a nanophotonic chip proved to be challenging. Here, we demonstrate such an on-chip parametric down-conversion source of photon pairs based on second-order nonlinearity in an aluminum-nitride microring resonator. We show the potential of our source for quantum information processing by measuring the high visibility anti-bunching of heralded single photons with nearly ideal state purity. Our down-conversion source yields measured coincidence rates of 80 Hz, which implies MHz generation rates of correlated photon pairs. Low noise performance is demonstrated by measuring high coincidence-to-accidental ratios. The generated photon pairs are spectrally far separated from the pump field, providing great potential for realizing sufficient on-chip filtering and monolithic integration of quantum light sources, waveguide circuits and single-photon detectors. A chip-based source of photon pairs for applications in quantum information processing has been built by a team of scientists in the US. Xiang Guo and co-workers from Yale University built the quantum light source from an aluminum nitride microring resonator. The strong second-order nonlinearity of the aluminum nitride yields efficient parametric down-conversion. This allows 775-nm-wavelength pump photons to be converted into a pair of entangled photons in the telecommunications window of 1550 nm. Tests indicated that the heralded photons generated by the microring source are anti-bunched and have high visibility and a high purity of state, indicating that they are highly suitable for use in quantum optics experiments. In principle, the on-chip source is compatible with megahertz generation rates and large-scale manufacture of integrated optical circuits.

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Parametric down-conversion photon pair source on a nanophotonic chip

Photonic integrated circuits hold promise as miniaturized and scalable platforms for classical and quantum photonic information processing. Second-order nonlinearity (χ(2)) is the basis of many important applications such as second-harmonic generation, spontaneous parametric down-conversion, and optical parametric oscillation. Here, we present systematical investigation and optimization of the second-harmonic generation in a dual-resonant aluminum nitride microring resonator. By optimizing the quality factor, independently engineering the coupling conditions for dual-band operation, and perfectly fulfilling phase-match conditions through thermal tuning, we demonstrate a second-harmonic generation efficiency of 2500%  W−1 in the low-pump-power regime. To the best of our knowledge, this is a state-of-the-art value among all the integrated photonic platforms. We also study the high-power regime where the pump power depletion is non-negligible. A conversion efficiency of 12% is realized with 27 mW pump power. Our high-efficiency second-harmonic generator enables integrated frequency conversion and frequency locking between visible and infrared systems, and our approach can also apply to other photonic platforms.

Second-harmonic generation in aluminum nitride microrings with 2500%/W conversion efficiency

A new device that can potentially be scaled up for quantum computing converts visible light to infrared light suitable for fiber-optic transmission without destroying the light's quantum state.

On-Chip Strong Coupling and Efficient Frequency Conversion between Telecom and Visible Optical Modes.

Leveraging the quantum information-processing ability of superconducting circuits and long-distance distribution ability of optical photons promises the realization of complex and large-scale quantum networks. In such a scheme, a coherent and efficient quantum transducer between superconducting and photonic circuits is critical. However, this quantum transducer is still challenging because the use of intermediate excitations in current schemes introduces extra noise and limits bandwidth. We realize direct and coherent transduction between superconducting and photonic circuits based on the triple-resonance electro-optic principle, with integrated devices incorporating both superconducting and optical cavities on the same chip. Electromagnetically induced transparency is observed, indicating the coherent interaction between microwave and optical photons. Internal conversion efficiency of 25.9 ± 0.3% has been achieved, with 2.05 ± 0.04% total efficiency. Superconducting cavity electro-optics offers broad transduction bandwidth and high scalability and represents a significant step toward integrated hybrid quantum circuits and distributed quantum computation.

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Superconducting cavity electro-optics: A platform for coherent photon conversion between superconducting and photonic circuits.

On-chip frequency comb generations enable compact broadband sources for spectroscopic sensing and precision spectroscopy. Recent microcomb studies focus on the infrared spectral regime and have difficulty accessing the visible regime. We demonstrate comb-like visible frequency line generation through second-harmonic, third-harmonic, and sum-frequency conversion of a Kerr comb within a high-Q aluminum nitride (AlN) microring resonator pumped by a single telecom laser. The strong power enhancement, in conjunction with the unique combination of Pockels (χ2) and Kerr (χ3) optical nonlinearity of AlN, leads to cascaded frequency conversions in the visible spectrum. High-resolution spectroscopic study of the visible frequency lines indicates matched free spectrum range over all the bands. This frequency doubling and tripling effect in a single microcomb structure offers great potential for comb spectroscopy and self-referencing comb.

Xiang Guo

Papers

Parametric down-conversion photon pair source on a nanophotonic chip

Second-harmonic generation in aluminum nitride microrings with 2500%/W conversion efficiency

On-Chip Strong Coupling and Efficient Frequency Conversion between Telecom and Visible Optical Modes.

Superconducting cavity electro-optics: A platform for coherent photon conversion between superconducting and photonic circuits.

Green, red, and IR frequency comb line generation from single IR pump in AlN microring resonator