Cavity quantum electrodynamics (QED) studies the interaction between a quantum emitter and a single radiation-field mode. When an atom is strongly coupled to a cavity mode, it is possible to realize important quantum information processing tasks, such as controlled coherent coupling and entanglement of distinguishable quantum systems. Realizing these tasks in the solid state is clearly desirable, and coupling semiconductor self-assembled quantum dots to monolithic optical cavities is a promising route to this end. However, validating the efficacy of quantum dots in quantum information applications requires confirmation of the quantum nature of the quantum-dot-cavity system in the strong-coupling regime. Here we find such confirmation by observing quantum correlations in photoluminescence from a photonic crystal nanocavity interacting with one, and only one, quantum dot located precisely at the cavity electric field maximum. When off-resonance, photon emission from the cavity mode and quantum-dot excitons is anticorrelated at the level of single quanta, proving that the mode is driven solely by the quantum dot despite an energy mismatch between cavity and excitons. When tuned to resonance, the exciton and cavity enter the strong-coupling regime of cavity QED and the quantum-dot exciton lifetime reduces by a factor of 145. The generated photon stream becomes antibunched, proving that the strongly coupled exciton/photon system is in the quantum regime. Our observations unequivocally show that quantum information tasks are achievable in solid-state cavity QED.

Quantum nature of a strongly coupled single quantum dot–cavity system

We describe the recent experimental progress in the control of spontaneous emission by manipulating optical modes with photonic crystals. It has been clearly demonstrated that the spontaneous emission from light emitters embedded in photonic crystals can be suppressed by the so-called photonic bandgap, whereas the emission efficiency in the direction where optical modes exist can be enhanced. Also, when an artificial defect is introduced into the photonic crystal, a photonic nanocavity is produced that can interact with light emitters. Cavity quality factors, or Q factors, of up to 2 million have been realized while maintaining very small mode volumes, and both spontaneous-emission modification (the Purcell effect) and strong-coupling phenomena have been demonstrated. The use of photonic crystals and nanocavities to manipulate spontaneous emission will contribute to the evolution of a variety of applications, including illumination, display, optical communication, solar energy and even quantum-information systems.

Spontaneous-emission control by photonic crystals and nanocavities

Engineering the electromagnetic environment of a nanometre-scale light emitter by use of a photonic cavity can significantly enhance its spontaneous emission rate, through cavity quantum electrodynamics in the Purcell regime. This effect can greatly reduce the lasing threshold of the emitter, providing a low-threshold laser system with small footprint, low power consumption and ultrafast modulation. An ultralow-threshold nanoscale laser has been successfully developed by embedding quantum dots into a photonic crystal cavity (PCC). However, several challenges impede the practical application of this architecture, including the random positions and compositional fluctuations of the dots, extreme difficulty in current injection, and lack of compatibility with electronic circuits. Here we report a new lasing strategy: an atomically thin crystalline semiconductor--that is, a tungsten diselenide monolayer--is non-destructively and deterministically introduced as a gain medium at the surface of a pre-fabricated PCC. A continuous-wave nanolaser operating in the visible regime is thereby achieved with an optical pumping threshold as low as 27 nanowatts at 130 kelvin, similar to the value achieved in quantum-dot PCC lasers. The key to the lasing action lies in the monolayer nature of the gain medium, which confines direct-gap excitons to within one nanometre of the PCC surface. The surface-gain geometry gives unprecedented accessibility and hence the ability to tailor gain properties via external controls such as electrostatic gating and current injection, enabling electrically pumped operation. Our scheme is scalable and compatible with integrated photonics for on-chip optical communication technologies.

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Monolayer semiconductor nanocavity lasers with ultralow thresholds

Over the past decade, advances in LEDs have enabled the potential for wide-scale replacement of traditional lighting with solid-state light sources. If LED performance targets are realized, solid-state lighting will provide significant energy savings, important environmental benefits, and dramatically new ways to utilize and control light. In this paper, we review LED performance targets that are needed to achieve these benefits and highlight some of the remaining technical challenges. We describe recent advances in LED materials and novel device concepts that show promise for realizing the full potential of LED-based white lighting.

LEDs for Solid-State Lighting: Performance Challenges and Recent Advances

DNA has become one of the most extensively used molecular building blocks for engineering self-assembling materials. DNA origami is a technique that uses hundreds of short DNA oligonucleotides, called staple strands, to fold a long single-stranded DNA, which is called a scaffold strand, into various designer nanoscale architectures. DNA origami has dramatically improved the complexity and scalability of DNA nanostructures. Due to its high degree of customization and spatial addressability, DNA origami provides a versatile platform with which to engineer nanoscale structures and devices that can sense, compute, and actuate. These capabilities open up opportunities for a broad range of applications in chemistry, biology, physics, material science, and computer science that have often required programmed spatial control of molecules and atoms in three-dimensional (3D) space. This review provides a comprehensive survey of recent developments in DNA origami structure, design, assembly, and directed self-assemb...

DNA Origami: Scaffolds for Creating Higher Order Structures

We demonstrate that very few (2\char21{}4) quantum dots as a gain medium are sufficient to realize a photonic-crystal laser based on a high-quality nanocavity. Photon correlation measurements show a transition from a thermal to a coherent light state proving that lasing action occurs at ultralow thresholds. Observation of lasing is unexpected since the cavity mode is in general not resonant with the discrete quantum dot states and emission at those frequencies is suppressed. In this situation, the quasicontinuous quantum dot states become crucial since they provide an energy-transfer channel into the lasing mode, effectively leading to a self-tuned resonance for the gain medium.

https://web.physics.ucsb.edu/~quopt/self_tun.pdf

Self-tuned quantum dot gain in photonic crystal lasers.

We relate the currently limited efficiency of photonic crystal (PhC)-assisted gallium nitride light-emitting diodes (LEDs) to the existence of unextracted guided modes. To remedy this, we introduce epitaxial structures which modify the distribution of guided modes. LEDs are fabricated according to this concept, and the tailored band structure is determined experimentally. We investigate theoretically the consequences of this improvement, which significantly enhances the potential for efficient light extraction by PhCs.

/pdf/photonic-crystal-gan-light-emitting-diodes-with-tailored-18poym3n5y.pdf

Photonic-crystal GaN light-emitting diodes with tailored guided modes distribution

The authors demonstrate a technique to achieve high-precision tuning of photonic crystal nanocavities by atomic force microscope nano-oxidation of the cavity surface. Relative tuning between two nanocavity modes is achieved though careful choice of the oxide pattern, allowing them to restore the spectral degeneracy conditions necessary to create polarization-entangled quantum states. Tuning steps less than the linewidth (1A) of the high quality factor modes are obtained, allowing for virtually continuous tuning ability.

Tuning photonic nanocavities by atomic force microscope nano-oxidation

We study the response of GaAs photonic crystal membrane resonators to thin-film deposition. Slow spectral shifts of the cavity mode of several nanometers are observed at low temperatures, caused by cryo-gettering of background molecules. Heating the membrane resets the drift and shielding will prevent drift altogether. In order to explore the drift as a tool to detect surface layers, or to intentionally shift the cavity resonance frequency, we studied the effect of self-assembled monolayers of polypeptide molecules attached to the membranes. The 2-nm-thick monolayers lead to a discrete step in the resonance frequency and partially passivate the surface.

/pdf/frequency-control-of-photonic-crystal-membrane-resonators-by-4f6zczamma.pdf

Frequency control of photonic crystal membrane resonators by monolayer deposition

Photonic crystal membrane cavities play a key role as building blocks in the realization of several applications, including quantum information and photonic circuits. Thus far, there has been no work on defect cavities with active layers emitting in the UV to green range of the spectrum based on the (Al,In,Ga)N material system. While this material system has great potential for a new generation of optoelectronic devices, there are several obstacles for the fabrication of GaN-based membrane cavities, including the absence of a conventional selective chemical wet etch. Here, we demonstrate the first fabrication of fully undercut GaN photonic crystal membranes containing an InGaN multiquantum well layer, fabricated using band-gap-selective photoelectrochemical etching. A postfabrication coating of Ta2O5 is used to tune the cavity modes into resonance with the quantum well emission, and the fabricated membranes exhibit resonant modes with Q=300.

Evelyn Hu

Papers

Self-tuned quantum dot gain in photonic crystal lasers.

Photonic-crystal GaN light-emitting diodes with tailored guided modes distribution

Tuning photonic nanocavities by atomic force microscope nano-oxidation

Frequency control of photonic crystal membrane resonators by monolayer deposition

Visible resonant modes in GaN-based photonic crystal membrane cavities