Liam Wilbraham

TL;DR: The use of hydrogen as a fuel, when generated from water using semiconductor photocatalysts and driven by sunlight, is a sustainable alternative to fossil fuels as discussed by the authors, however, our understanding of the key properties underlying their photoinitiated redox processes has not kept pace, and this impedes further progress to generate cost-competitive technologies.

TL;DR: This work integrates robotic experimentation with high-throughput computation to navigate the available structure–property space and discovers new polymers with sacrificial hydrogen evolution rates (HERs) of more than 6 mmol g–1 h–1.

TL;DR: In this article, three series of conjugated microporous polymers (CMPs) were used as photocatalysts for hydrogen production from water using a sacrificial hole scavenger.

TL;DR: The recent advances in the development and application of density-based indexes for the description of the nature and quantification of the extent of charge transfer associated with a given electronic transition are reviewed in this paper.