Collective electronic excitations at metal surfaces are well known to play a key role in a wide spectrum of science, ranging from physics and materials science to biology. Here we focus on a theoretical description of the many-body dynamical electronic response of solids, which underlines the existence of various collective electronic excitations at metal surfaces, such as the conventional surface plasmon, multipole plasmons and the recently predicted acoustic surface plasmon. We also review existing calculations, experimental measurements and applications.

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Theory of surface plasmons and surface-plasmon polaritons

Heat-assisted magnetic recording is a promising approach for enabling large increases in the storage density of hard disk drives. A laser is used to momentarily heat the recording area of the medium to reduce its coercivity below that of the applied magnetic field from the recording head. In such a system, the recording materials have a very high magnetic anisotropy, which is essential for the thermal stability of the magnetization of the extremely small grains in the medium. This technology involves new recording physics, new approaches to near field optics, a recording head that integrates optics and magnetics, new recording materials, lubricants that can withstand extremely high temperatures, and new approaches to the recording channel design. This paper surveys the challenges for this technology and the progress that has been made in addressing them.

Heat Assisted Magnetic Recording

Nanoantennas for visible and infrared radiation can strongly enhance the interaction of light with nanoscale matter by their ability to efficiently link propagating and spatially localized optical fields. This ability unlocks an enormous potential for applications ranging from nanoscale optical microscopy and spectroscopy over solar energy conversion, integrated optical nanocircuitry, opto-electronics and density-of-states engineering to ultra-sensing as well as enhancement of optical nonlinearities. Here we review the current understanding of metallic optical antennas based on the background of both well-developed radiowave antenna engineering and plasmonics. In particular, we discuss the role of plasmonic resonances on the performance of nanoantennas and address the influence of geometrical parameters imposed by nanofabrication. Finally, we give a brief account of the current status of the field and the major established and emerging lines of investigation in this vivid area of research.

https://iopscience.iop.org/article/10.1088/0034-4885/75/2/024402/pdf

Nanoantennas for visible and infrared radiation.

Fluorescence spectroscopy is widely used in biological research. Until recently, essentially all fluorescence experiments were performed using optical energy which has radiated to the far-field. By far-field we mean at least several wavelengths from the fluorophore, but propagating far-field radiation is usually detected at larger macroscopic distances from the sample. In recent years there has been a growing interest in the interactions of fluorophores with metallic surfaces or particles. Near-field interactions are those occurring within a wavelength distance of an excited fluorophore. The spectral properties of fluorophores can be dramatically altered by near-field interactions with the electron clouds present in metals. These interactions modify the emission in ways not seen in classical fluorescence experiments. In this review we provide an intuitive description of the complex physics of plasmons and near-field interactions. Additionally, we summarize the recent work on metal-fluorophore interactions and suggest how these effects will result in new classes of experimental procedures, novel probes, bioassays and devices.

Plasmon-controlled fluorescence: a new paradigm in fluorescence spectroscopy

The optical properties of plasmonic dipole and bowtie nanoantennas are investigated in detail using the Green’s tensor technique. The influence of the geometrical parameters (antenna length, gap dimension and bow angle) on the antenna field enhancement and spectral response is discussed. Dipole and bowtie antennas confine the field in a volume well below the diffraction limit, defined by the gap dimensions. The dipole antenna produces a stronger field enhancement than the bowtie antenna for all investigated antenna geometries. This enhancement can reach three orders of magnitude for the smallest examined gap. Whereas the dipole antenna is monomode in the considered spectral range, the bowtie antenna exhibits multiple resonances. Furthermore, the sensitivity of the antennas to index changes of the environment and of the substrate is investigated in detail for biosensing applications; the bowtie antennas show slightly higher sensitivity than the dipole antenna.

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Engineering the optical response of plasmonic nanoantennas

We demonstrate that bowtie apertures can be used for contact lithography to achieve nanometer scale resolution. The bowtie apertures with a 30 nm gap size are fabricated in aluminum thin films coated on quartz substrates. Lithography results show that holes of sub-50-nm dimensions can be produced in photoresist by illuminating the apertures with a 355 nm laser beam polarized in the direction across the gap. Experimental results show enhanced transmission and light concentration of bowtie apertures compared to square and rectangular apertures of the same opening area. Finite different time domain simulations are used to explain the experimental results.

Nanolithography using high transmission nanoscale bowtie apertures.

A near-field scanning optical microscope probe integrated with nanoscale bowtie aperture for enhanced optical transmission is demonstrated. The bowtie-shape aperture allows a propagating mode in the bowtie gap region, which enables simultaneous nanoscale optical resolution and enhanced optical transmission. The optical characteristics of the bowtie aperture are demonstrated by measuring the optical near fields produced by the aperture. It is shown that bowtie aperture probes have one order of magnitude increase in transmission over probes with a regular shape aperture of the same resolution. The imaging results using bowtie aperture are in agreement with those obtained from numerical calculations.

High transmission nanoscale bowtie-shaped aperture probe for near-field optical imaging

Nanoscale ridge aperture antennas have been shown to have high transmission efficiency and confined nanoscale radiation in the near field region compared with regularly-shaped apertures. The radiation enhancement is attributed to the fundamental electric-magnetic field propagating in the TE10 mode concentrated in the gap between the ridges. This paper reports experimental demonstration of field enhancement using such ridge antenna apertures in a bowtie shape for the manufacture of nanometer size structures using an NSOM (near field scanning optical microscopy) probe integrated with nanoscale bowtie aperture. Consistent lines with width of 59 nm and as small as 24 nm have be written on photoresist using such probes.

/pdf/nanopatterning-using-nsom-probes-integrated-with-high-3c8b9wdibr.pdf

Nanopatterning using NSOM probes integrated with high transmission nanoscale bowtie aperture

C-shaped ridge apertures are used in contact nanolithography to achieve nanometer scale resolution. Lithography results demonstrated that holes as small as 60 nm can be produced in the photoresist by illuminating the apertures with a 355 nm laser beam. Experiments are also performed using comparable square and rectangular apertures. Results show enhanced transmission and light concentration of C apertures compared to the apertures with regular shapes. Finite difference time domain simulations are used to design the apertures and explain the experimental results.

/pdf/contact-optical-nanolithography-using-nanoscale-c-shaped-15lc6xtp00.pdf

Contact optical nanolithography using nanoscale C-shaped apertures.

We report spectroscopic measurements of transmitted field through bowtie-shaped nanoscale apertures in visible wavelength region. Resonance in these apertures and its relation with the aperture geometry are investigated. The near-field spectral response is also investigated using finite difference time domain (FDTD) computation and compared with the spectroscopic measurements. The dependences of the peak wavelength and peak amplitude on the geometry of the bowtie aperture are illustrated. Design rules are proposed to optimize the bowtie aperture for producing a sub-wavelength, high transmission field.

Liang Wang

Papers

Nanolithography using high transmission nanoscale bowtie apertures.

High transmission nanoscale bowtie-shaped aperture probe for near-field optical imaging

Nanopatterning using NSOM probes integrated with high transmission nanoscale bowtie aperture

Contact optical nanolithography using nanoscale C-shaped apertures.

Spectral resonance of nanoscale bowtie apertures in visible wavelength