Showing papers by "Manish Shrivastava published in 2006"

Emissions from open biomass burning in India: Integrating the inventory approach with high-resolution Moderate Resolution Imaging Spectroradiometer (MODIS) active-fire and land cover data

Abstract: [1] Climatological mean estimates of forest burning and crop waste burning based on broad assumptions of the amounts burned have so far been used for India in global inventories. Here we estimate open biomass burning representative of 1995–2000 from forests using burned area and biomass density specific for Indian ecosystems and crop waste burning as a balance between generation and known uses as fuel and fodder. High-resolution satellite data of active fires and land cover classification from MODIS, both on a scale of 1 km × 1 km, were used to capture the seasonal variability of forest and crop waste burning and in conjunction with field reporting. Correspondence in satellite-detected fire cycles with harvest season was used to identify types crop waste burned in different regions. The fire season in forest areas was from February to May, and that in croplands varied with geographical location, with peaks in April and October, corresponding to the two major harvest seasons. Spatial variability in amount of forest biomass burned differed from corresponding forest fire counts with biomass burned being largest in central India but fire frequency being highest in the east-northeast. Unutilized crop waste and MODIS cropland fires were predominant in the western Indo-Gangetic plain. However, the amounts of unutilized crop waste in the four regions were not strictly proportional to the fire counts. Fraction crop waste burned in fields ranged from 18 to 30% on an all-India basis and had a strong regional variation. Open burning contributes importantly (about 25%) to black carbon, organic matter, and carbon monoxide emissions, a smaller amount (9–13%) to PM2.5 (particulate mass in particles smaller than 2.5 micron diameter) and CO2 emissions, and negligibly to SO2 emissions (1%). However, it cannot explain a large “missing source” of BC or CO from India.

Modeling semivolatile organic aerosol mass emissions from combustion systems.

Abstract: Experimental measurements of gas-particle partitioning and organic aerosol mass in diluted diesel and wood combustion exhaust are interpreted using a two-component absorptive-partitioning model. The model parameters are determined by fitting the experimental data. The changes in partitioning with dilution of both wood smoke and diesel exhaust can be described by two lumped compounds in roughly equal abundance with effective saturation concentrations of ∼1600 μg m-3 and ∼20 μg m-3. The model is used to investigate gas-particle partitioning of emissions across a wide range of atmospheric conditions. Under the highly dilute conditions found in the atmosphere, the partitioning of the emissions is strongly influenced by the ambient temperature and the background organic aerosol concentration. The model predicts large changes in primary organic aerosol mass with varying atmospheric conditions, indicating that it is not possible to specify a single value for the organic aerosol emissions. Since atmospheric condi...