This Review summarizes recent progress of single-photon emitters based on defects in solids and highlights new research directions. The photophysical properties of single-photon emitters and efforts towards scalable system integration are also discussed.

Solid-state single-photon emitters

Integrated quantum nanophotonics Technologies that exploit the rules of quantum mechanics offer a potential advantage over classical devices in terms of sensitivity. Sipahigil et al. combined the quantum optical features of silicon-vacancy color centers with diamond-based photonic cavities to form a platform for integrated quantum nanophotonics (see the Perspective by Hanson). They could thus generate single photons from the color centers, optically switch light in the cavity by addressing the state of the color center, and quantum-mechanically entangle two color centers positioned in the cavity. The work presents a viable route to develop an integrated platform for quantum networks. Science, this issue p. 847; see also p. 835 An integrated quantum optical platform is demonstrated using silicon vacancy color centers and diamond photonics. Efficient interfaces between photons and quantum emitters form the basis for quantum networks and enable optical nonlinearities at the single-photon level. We demonstrate an integrated platform for scalable quantum nanophotonics based on silicon-vacancy (SiV) color centers coupled to diamond nanodevices. By placing SiV centers inside diamond photonic crystal cavities, we realize a quantum-optical switch controlled by a single color center. We control the switch using SiV metastable states and observe optical switching at the single-photon level. Raman transitions are used to realize a single-photon source with a tunable frequency and bandwidth in a diamond waveguide. By measuring intensity correlations of indistinguishable Raman photons emitted into a single waveguide, we observe a quantum interference effect resulting from the superradiant emission of two entangled SiV centers.

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An integrated diamond nanophotonics platform for quantum optical networks

We control the electronic structure of the silicon-vacancy (SiV) color-center in diamond by changing its static strain environment with a nano-electro-mechanical system This allows deterministic and local tuning of SiV optical and spin transition frequencies over a wide range, an essential step towards multiqubit networks In the process, we infer the strain Hamiltonian of the SiV revealing large strain susceptibilities of order 1 PHz/strain for the electronic orbital states We identify regimes where the spin-orbit interaction results in a large strain susceptibility of order 100 THz/strain for spin transitions, and propose an experiment where the SiV spin is strongly coupled to a nanomechanical resonator

Strain engineering of the silicon-vacancy center in diamond

There has been rapidly growing interest in hybrid quantum devices involving a solid-state spin and a macroscopic mechanical oscillator. Such hybrid devices create exciting opportunities to mediate interactions between disparate qubits and to explore the quantum regime of macroscopic mechanical objects. In particular, a system consisting of the nitrogen-vacancy defect center in diamond coupled to a high quality factor mechanical oscillator is an appealing candidate for such a hybrid quantum device, as it utilizes the highly coherent and versatile spin properties of the defect center. In this paper, we will review recent experimental progress on diamond-based hybrid quantum devices in which the spin and orbital dynamics of single defects are driven by the motion of a mechanical oscillator. In addition, we discuss prospective applications for this device, including long range, phonon-mediated spin-spin interactions, and phonon cooling in the quantum regime. We conclude the review by evaluating the experimental limitations of current devices and identifying alternative device architectures that may reach the strong coupling regime.

https://iopscience.iop.org/article/10.1088/2040-8986/aa52cd/pdf

Topical Review: Spins and mechanics in diamond

Radio-frequency communication systems have long used bulk- and surface-acoustic-wave devices supporting ultrasonic mechanical waves to manipulate and sense signals. These devices have greatly improved our ability to process microwaves by interfacing them to orders-of-magnitude slower and lower-loss mechanical fields. In parallel, long-distance communications have been dominated by low-loss infrared optical photons. As electrical signal processing and transmission approach physical limits imposed by energy dissipation, optical links are now being actively considered for mobile and cloud technologies. Thus there is a strong driver for wavelength-scale mechanical wave or “phononic” circuitry fabricated by scalable semiconductor processes. With the advent of these circuits, new micro- and nanostructures that combine electrical, optical, and mechanical elements have emerged. In these devices, such as optomechanical waveguides and resonators, optical photons and gigahertz phonons are ideally matched to one another, as both have wavelengths on the order of micrometers. The development of phononic circuits has thus emerged as a vibrant field of research pursued for optical signal processing and sensing applications as well as emerging quantum technologies. In this review, we discuss the key physics and figures of merit underpinning this field. We also summarize the state of the art in nanoscale electro- and optomechanical systems with a focus on scalable platforms such as silicon. Finally, we give perspectives on what these new systems may bring and what challenges they face in the coming years. In particular, we believe hybrid electro- and optomechanical devices incorporating highly coherent and compact mechanical elements on a chip have significant untapped potential for electro-optic modulation, quantum microwave-to-optical photon conversion, sensing, and microwave signal processing.

https://biblio.ugent.be/publication/8626734/file/8626737.pdf

Controlling phonons and photons at the wavelength scale: integrated photonics meets integrated phononics

Cavity-optomechanical systems realized in single-crystal diamond are poised to benefit from its extraordinary material properties, including low mechanical dissipation and a wide optical transparency window. Diamond is also rich in optically active defects, such as the nitrogen-vacancy (NV) and silicon-vacancy (SiV) centers, which behave as atom-like systems in the solid state. Predictions and observations of coherent coupling of the NV electronic spin to phonons via lattice strain have motivated the development of diamond nanomechanical devices aimed at the realization of hybrid quantum systems in which phonons provide an interface with diamond spins. In this work, we demonstrate diamond optomechanical crystals (OMCs), a device platform to enable such applications, wherein the co-localization of ∼200  THz photons and few to 10 GHz phonons in a quasi-periodic diamond nanostructure leads to coupling of an optical cavity field to a mechanical mode via radiation pressure. In contrast to other material systems, diamond OMCs operating in the resolved-sideband regime possess large intracavity photon capacities (>10^5) and sufficient optomechanical coupling rates to reach a cooperativity of ∼20 at room temperature, allowing for the observation of optomechanically induced transparency and the realization of large-amplitude optomechanical self-oscillations.

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Diamond optomechanical crystals

Cavity-optomechanical systems realized in single-crystal diamond are poised to benefit from its extraordinary material properties, including low mechanical dissipation and a wide optical transparency window. Diamond is also rich in optically active defects, such as the nitrogen-vacancy (NV) and silicon-vacancy (SiV) centers, which behave as atom-like systems in the solid state. Predictions and observations of coherent coupling of the NV electronic spin to phonons via lattice strain has motivated the development of diamond nanomechanical devices aimed at realization of hybrid quantum systems, in which phonons provide an interface with diamond spins. In this work, we demonstrate diamond optomechanical crystals (OMCs), a device platform to enable such applications, wherein the co-localization of ~ 200 THz photons and few to 10 GHz phonons in a quasi-periodic diamond nanostructure leads to coupling of an optical cavity field to a mechanical mode via radiation pressure. In contrast to other material systems, diamond OMCs operating in the resolved-sideband regime possess large intracavity photon capacity (> 10$^5$) and sufficient optomechanical coupling rates to reach a cooperativity of ~ 20 at room temperature, allowing for the observation of optomechanically induced transparency and the realization of large amplitude optomechanical self-oscillations.

We describe an apparatus for the implementation of hybrid optomechanical systems at 4 K. The platform is based on a high-finesse, micrometer-scale fiber Fabry-Perot cavity, which can be widely tuned using piezoelectric positioners. A mechanical resonator can be positioned within the cavity in the object-in-the-middle configuration by a second set of positioners. A high level of stability is achieved without sacrificing either performance or tunability, through the combination of a stiff mechanical design, passive vibration isolation, and an active Pound-Drever-Hall feedback lock incorporating a reconfigurable digital filter. The stability of the cavity length is demonstrated to be better than a few picometers over many hours both at room temperature and at 4 K.

https://aip.scitation.org/doi/pdf/10.1063/5.0098140

A tunable fiber Fabry-Perot cavity for hybrid optomechanics stabilized at 4 K.

We image and characterize the mechanical modes of a 2D drum resonator made of hBN suspended over a high-stress Si3N4 membrane. Our measurements demonstrate hybridization between various modes of the hBN resonator and those of the Si3N4 membrane. The measured resonance frequencies and spatial profiles of the modes are consistent with finite-element simulations based on idealized geometry. Spectra of the thermal motion reveal that, depending on the degree of hybridization with modes of the heavier and higher-quality-factor Si3N4 membrane, the quality factors and the motional mass of the hBN drum modes can be shifted by orders of magnitude. This effect could be exploited to engineer hybrid drum/membrane modes that combine the low motional mass of 2D materials with the high quality factor of Si3N4 membranes for optomechanical or sensing applications.

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Mechanical Mode Imaging of a High-Q Hybrid hBN/Si3N4 Resonator.

We demonstrate diamond optomechanical crystals (OMCs), which support a ∼6 GHz mechanical cavity coupled to a co-resonant ∼200 THz photon field. Diamond OMCs are optically driven to a cooperativity >1, highlighted by observed ‘phonon lasing’.

Thibaud Ruelle

Papers

Diamond optomechanical crystals

Diamond optomechanical crystals

A tunable fiber Fabry-Perot cavity for hybrid optomechanics stabilized at 4 K.

Mechanical Mode Imaging of a High-Q Hybrid hBN/Si3N4 Resonator.

Diamond optomechanical crystals in the resolved-sideband regime