The rapid detection of biological and chemical substances in real time is particularly important for public health and environmental monitoring and in the military sector If the process of substance detection to visual reporting can be implemented into a single miniaturized sensor, there could be a profound impact on practical applications Here, we propose a compact sensor platform that integrates liquid crystals (LCs) and holographic metasurfaces to autonomously sense the existence of a volatile gas and provide an immediate visual holographic alarm By combining the advantage of the rapid responses to gases realized by LCs with the compactness of holographic metasurfaces, we develop ultracompact gas sensors without additional complex instruments or machinery to report the visual information of gas detection To prove the applicability of the compact sensors, we demonstrate a metasurface-integrated gas sensor on safety goggles via a one-step nanocasting process that is attachable to flat, curved, and flexible surfaces

Holographic metasurface gas sensors for instantaneous visual alarms.

Vectorial holography has gained a lot of attention due to the promise of versatile polarization control of structured light for enhanced optical security and multi-channel optical communication. Here, we propose a bifunctional metasurface which combines both structural color printing and vectorial holography with eight polarization channels towards advanced encryption applications. The structural colour prints are observed under white light while the polarization encoded holograms are reconstructed under laser illumination. To encode multiple holographic images for different polarization states, a pixelated metasurface is adopted. As a proof-of-concept, we devise an electrically tunable optical security platform incorporated with liquid crystals. The optical security platform is doubly encrypted: an image under white light is decrypted to provide the first key and the corresponding information is used to fully unlock the encrypted information via projected vectorial holographic images. Such an electrically tunable optical security platform may enable smart labels for security and anticounterfeiting applications. The authors present a bi-functional metasurface, combining structural color printing observed under white light and polarization encoded It is appropriate. vectorial holography. A pixelated design is used encode multiple holographic images, and they demonstrate an electrically tunable optical security platform.

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Pixelated bifunctional metasurface-driven dynamic vectorial holographic color prints for photonic security platform.

Optical metasurfaces can offer high-quality multichannel displays by modulating different degrees of freedom of light, demonstrating great potential in the next generation of optical encryption and anti-counterfeiting. Different from the direct imaging modality of metasurfaces, single-pixel imaging (SPI) as a typical computational imaging technique obtains the object image from a decryption-like computational process. Here, we propose an optical encryption scheme by introducing metasurface-images (meta-images) into the encoding and decoding processes as the keys of SPI encryption. Different high-quality meta-images generated by a dual-channel Malus metasurface play the role of keys to encode multiple target images and retrieve them following the principle of SPI. Our work eliminates the conventional digital transmission process of keys in SPI encryption, enables the reusability of a single metasurface in different encryption processes, and thereby paves the way toward a high-security optical encryption between direct and indirect imaging methods.

https://advances.sciencemag.org/content/advances/7/21/eabg0363.full.pdf

Metasurface-based key for computational imaging encryption

Optically variable devices (OVDs) are in tremendous demand as optical indicators against the increasing threat of counterfeiting. Conventional OVDs are exposed to the danger of fraudulent replication with advances in printing technology and widespread copying methods of security features. Metasurfaces, two-dimensional arrays of subwavelength structures known as meta-atoms, have been nominated as a candidate for a new generation of OVDs as they exhibit exceptional behaviors that can provide a more robust solution for optical anti-counterfeiting. Unlike conventional OVDs, metasurface-driven OVDs (mOVDs) can contain multiple optical responses in a single device, making them difficult to reverse engineered. Well-known examples of mOVDs include ultrahigh-resolution structural color printing, various types of holography, and polarization encoding. In this review, we discuss the new generation of mOVDs. The fundamentals of plasmonic and dielectric metasurfaces are presented to explain how the optical responses of metasurfaces can be manipulated. Then, examples of monofunctional, tunable, and multifunctional mOVDs are discussed. We follow up with a discussion of the fabrication methods needed to realize these mOVDs, classified into prototyping and manufacturing techniques. Finally, we provide an outlook and classification of mOVDs with respect to their capacity and security level. We believe this newly proposed concept of OVDs may bring about a new era of optical anticounterfeit technology leveraging the novel concepts of nano-optics and nanotechnology.

Metasurface-Driven Optically Variable Devices.

Symmetric spin–orbit interaction (SOI)‐based approaches apply a practical limit on helicity multiplexed metaoptics, i.e., center symmetric information encoding. Contrarily, asymmetric SOI's based on the combination of geometric and propagation phase‐delay approaches can effectively address such limitations for multifunctional multiplexed metaoptics on the cost of design complexities. In this paper, a simple asymmetric SOI‐based technique is realized for multifunctional metaoptics, employing only a single unit cell, breaking the conventional tradeoff between design complexity and efficient asymmetric transmission efficiency. The design approach depends on geometric phase alone, which eases the fabrication challenges and decreases the computational cost associated with previous asymmetric SOI‐based metaoptics. Furthermore, this study utilizes a new, low‐cost CMOS‐compatible material to optimize the proposed single unit cell for low loss and high transmission efficiency over the complete visible domain. On‐axis and off‐axis holographic metasurfaces are designed and integrated with pressure‐sensitive liquid crystal cells to demonstrate actively tunable metaholography with no limitation of center symmetric information encoding. The simple design technique, cost‐effective fabrication, and finger touch‐enabled holographic output switching make this integrated setup a potential candidate for many applications such as smart safety labeling, motion or touch recognition, and interactive displays for impact monitoring of precious artworks and products.

Novel Spin‐Decoupling Strategy in Liquid Crystal‐Integrated Metasurfaces for Interactive Metadisplays

Flat optics, realized by the artificially created 2D material platform called optical metasurfaces, is currently undergoing a science-to-technology transition. However, "real-time" active operations of such flat optical devices remain yet unresolved. Here, liquid crystals (LCs)-integrated metaholograms for ultracompact dynamic holographic displays are proposed. The anisotropic nature of the LCs allows facile and repeatable manipulation of the polarization of light. Specifically designed ("designer") LCs and efficient helicity-encoded metaholograms are combined to realize stimuli-responsive dynamic displays. The designer LC modulators are used as switches that enable a variety of external stimuli (e.g., electric field, heat, surface pressure) to operate holographic images in real-time. Such a dynamic metaholographic platform will provide a path to external stimuli-driven "smart" sensing and display applications such as hologram labels for temperature/pressure/touch monitoring and interactive holographic displays with haptic motion recognition.

Won-Sik Kim

Papers

Holographic metasurface gas sensors for instantaneous visual alarms.

Stimuli-Responsive Dynamic Metaholographic Displays with Designer Liquid Crystal Modulators.