Abstract Surface acoustic wave (SAW) devices offer many attractive features for application as vapour phase chemical microsensors. This paper describes the characteristics of SAW devices and techniques by which they can be employed as vapour sensors. The perturbation of SAW velocity by polymeric coating films is investigated both theoretically and experimentally. Highest sensitivity can be achieved when the device is used as the resonating element in a delay line oscillator circuit. A simple equation has been developed from theoretical considerations which offers reasonably accurate quantitative predictions of SAW device frequency shifts when subjected to a given mass loading. In this mode the SAW device behaves very like conventional bulk-wave quartz crystal microbalances except that the sensitivity can be several orders of magnitude higher and the device size can be several orders of magnitude smaller. Detection of mass changes of a few femtograms by a SAW device having a surface area of 10−4 cm2 is theoretically possible.

Mechanism of operation and design considerations for surface acoustic wave device vapor sensors

A topical review of numerical and experimental studies of supercontinuum generation in photonic crystal fiber is presented over the full range of experimentally reported parameters, from the femtosecond to the continuous-wave regime. Results from numerical simulations are used to discuss the temporal and spectral characteristics of the supercontinuum, and to interpret the physics of the underlying spectral broadening processes. Particular attention is given to the case of supercontinuum generation seeded by femtosecond pulses in the anomalous group velocity dispersion regime of photonic crystal fiber, where the processes of soliton fission, stimulated Raman scattering, and dispersive wave generation are reviewed in detail. The corresponding intensity and phase stability properties of the supercontinuum spectra generated under different conditions are also discussed.

Supercontinuum generation, photonic crystal fiber

Lithium niobate (LN), an outstanding and versatile material, has influenced our daily life for decades: from enabling high-speed optical communications that form the backbone of the Internet to realizing radio-frequency filtering used in our cell phones. This half-century-old material is currently embracing a revolution in thin-film LN integrated photonics. The success of manufacturing wafer-scale, high-quality, thin films of LN on insulator (LNOI), accompanied with breakthroughs in nanofabrication techniques, have made high-performance integrated nanophotonic components possible. With rapid development in the past few years, some of these thin-film LN devices, such as optical modulators and nonlinear wavelength converters, have already outperformed their legacy counterparts realized in bulk LN crystals. Furthermore, the nanophotonic integration enabled ultra-low-loss resonators in LN, which unlocked many novel applications such as optical frequency combs and quantum transducers. In this Review, we cover -- from basic principles to the state of the art -- the diverse aspects of integrated thin-film LN photonics, including the materials, basic passive components, and various active devices based on electro-optics, all-optical nonlinearities, and acousto-optics. We also identify challenges that this platform is currently facing and point out future opportunities. The field of integrated LNOI photonics is advancing rapidly and poised to make critical impacts on a broad range of applications in communication, signal processing, and quantum information.

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Integrated photonics on thin-film lithium niobate

Controlling thermal transport has become relevant in recent years. Traditionally, this control has been achieved by tuning the scattering of phonons by including various types of scattering centres in the material (nanoparticles, impurities, etc). Here we take another approach and demonstrate that one can also use coherent band structure effects to control phonon thermal conductance, with the help of periodically nanostructured phononic crystals. We perform the experiments at low temperatures below 1 K, which not only leads to negligible bulk phonon scattering, but also increases the wavelength of the dominant thermal phonons by more than two orders of magnitude compared to room temperature. Thus, phononic crystals with lattice constants ≥1 μm are shown to strongly reduce the thermal conduction. The observed effect is in quantitative agreement with the theoretical calculation presented, which accurately determined the ballistic thermal conductance in a phononic crystal device.

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Engineering thermal conductance using a two-dimensional phononic crystal

The wide range of functions that are possible with lithium niobate (LN) waveguide devices, including phase and intensity modulation, second-harmonic generation, and difference-frequency generation, makes it attractive as a potential microcomb material. LN microcombs would combine essential comb self-referencing and control functions with the pulse generation process in a single microresonator device. Here, we demonstrate a soliton microcomb in a monolithic high-Q LN resonator. Direct frequency doubling of the soliton spectrum is observed inside the same cavity. The LN soliton mode-locking process also self-starts and allows bi-directional switching of soliton states, effects that are shown to result from the LN photorefractive effect. The Kerr solitons exhibit a self-frequency shift resulting from the Raman effect of LN. This microcomb platform can dramatically simplify miniature time keeping, frequency synthesis/division, and spectroscopy systems. Moreover, direct generation of femtosecond timescale pulses within LN microresonators can benefit quantum photonics and signal processing systems.

Self-starting bi-chromatic LiNbO 3 soliton microcomb

Lithium niobate (LN), dubbed by many as the silicon of photonics, has recently risen to the forefront of chip-scale nonlinear optics research since its demonstration as an ultralow-loss integrated photonics platform. Due to its significant quadratic nonlinearity (χ(2)), LN inspires many important applications such as second-harmonic generation (SHG), spontaneous parametric downconversion, and optical parametric oscillation. Here, we demonstrate high-efficiency SHG in dual-resonant, periodically poled z-cut LN microrings, where quasi-phase matching is realized by field-assisted domain engineering. Meanwhile, dual-band operation is accessed by optimizing the coupling conditions in fundamental and second-harmonic bands via a single pulley waveguide. As a result, when pumping a periodically poled LN microring in the low power regime at around 1617 nm, an on-chip SHG efficiency of 250,000%/W is achieved, a state-of-the-art value reported among current integrated photonics platforms. An absolute conversion efficiency of 15% is recorded with a low pump power of 115 μW in the waveguide. Such periodically poled LN microrings also present a versatile platform for other cavity-enhanced quasi-phase-matched χ(2) nonlinear optical processes.

Periodically poled thin-film lithium niobate microring resonators with a second-harmonic generation efficiency of 250,000%/W

High-index-contrast optical waveguides are crucial for the development of photonic integrated circuits with complex functionalities. Despite many similarities between optical and acoustic waves, high-acoustic-index-contrast phononic waveguides remain elusive, preventing intricate manipulation of phonons on par with its photonic counterpart. Here, we present the realization of such phononic waveguides and the formation of phononic integrated circuits through exploiting a gallium-nitride-on-sapphire platform, which provides strong confinement and control of phonons. By demonstrating key building blocks analogous to photonic circuit components, we establish the functionality and scalability of the phononic circuits. Moreover, the unidirectional excitation of propagating phononic modes allows the exploration of unconventional spin-orbit interaction of phonons in this circuit platform, which opens up the possibility of novel applications such as acoustic gyroscopic and non-reciprocal devices. Such phononic integrated circuits could provide an invaluable resource for both classical and quantum information processing.

/pdf/phononic-integrated-circuitry-and-spin-orbit-interaction-of-3kmgigu795.pdf

Phononic integrated circuitry and spin-orbit interaction of phonons.

Lithium niobate (LN), dubbed by many as the silicon of photonics, has recently risen to the forefront of chip-scale nonlinear optics research since its demonstration as an ultralow-loss integrated photonics platform. Due to its significant quadratic nonlinearity ($\chi^{(2)}$), LN inspires many important applications such as second-harmonic generation (SHG), spontaneous parametric down-conversion, and optical parametric oscillation. Here, we demonstrate high-efficiency SHG in dual-resonant, periodically poled z-cut LN microrings, where quasi-phase matching is realized by field-assisted domain engineering. Meanwhile, dual-band operation is accessed by optimizing the coupling conditions in fundamental and second-harmonic bands via a single pulley waveguide. As a result, when pumping a periodically poled LN microring in the low power regime at around 1617nm, an on-chip SHG efficiency of 250,000%/W is achieved, a state-of-the-art value reported among current integrated photonics platforms. An absolute conversion efficiency of 15% is recorded with a low pump power of 115$\mu$W in the waveguide. Such periodically poled LN microrings also present a versatile platform for other cavity-enhanced quasi-phase matched $\chi^{(2)}$ nonlinear optical processes.

Periodically poled thin film lithium niobate microring resonators with a second-harmonic generation efficiency of 250,000%/W

We demonstrate octave-spanning supercontinuum generation in unpoled lithium niobate waveguides, which are engineered to possess anomalous dispersion and pumped by a turn-key femtosecond laser centered at 1560 nm. Tunable dispersive waves and strong phase-matched second-harmonic generation are both observed by controlling the widths of the waveguides. The major features of the experimental spectra are reproduced by numerical modeling of the generalized nonlinear Schrodinger equation, which can be used to guide waveguide designs for tailoring the supercontinuum spectrum. Our results identify a path to a simple and integrable supercontinuum source in lithium niobate nanophotonic platform and will enable new capabilities in precision frequency metrology.

Octave-spanning supercontinuum generation in nanoscale lithium niobate waveguides.

Chip-based soliton frequency combs have been demonstrated on various material platforms, offering broadband, mutually coherent, and equally spaced frequency lines desired for many applications. Lithium niobate (LN), possessing both second- and third-order optical nonlinearities, as well as integrability on insulating substrates, has emerged as a novel source for microcomb generation and controlling. Here we demonstrate mode-locked soliton microcombs generated around 2 μm in a high-Q z-cut LN microring resonator. The intracavity photorefractive effect is found to be still dominant over the thermal effect in the 2 μm region, which facilitates direct accessing soliton states in the red-detuned regime, as reported in the telecom band. We also find that intracavity stimulated Raman scattering is greatly suppressed when moving the pump wavelength from the telecom band to 2 μm, thus alleviating Raman–Kerr comb competition. This Letter expands mode-locked LN microcombs to 2 μm, and could enable a variety of potential applications based on LN nanophotonic platform.

Yuntao Xu

Papers

Periodically poled thin-film lithium niobate microring resonators with a second-harmonic generation efficiency of 250,000%/W

Phononic integrated circuitry and spin-orbit interaction of phonons.

Periodically poled thin film lithium niobate microring resonators with a second-harmonic generation efficiency of 250,000%/W

Octave-spanning supercontinuum generation in nanoscale lithium niobate waveguides.

Soliton microcomb generation at 2 μm in z-cut lithium niobate microring resonators.