Nanomechanical oscillators are at the heart of ultrasensitive detectors of force, mass and motion. As these detectors progress to even better sensitivity, they will encounter measurement limits imposed by the laws of quantum mechanics. If the imprecision of a measurement of the displacement of an oscillator is pushed below a scale set by the standard quantum limit, the measurement must perturb the motion of the oscillator by an amount larger than that scale. Here we show a displacement measurement with an imprecision below the standard quantum limit scale. We achieve this imprecision by measuring the motion of a nanomechanical oscillator with a nearly shot-noise limited microwave interferometer. As the interferometer is naturally operated at cryogenic temperatures, the thermal motion of the oscillator is minimized, yielding an excellent force detector with a sensitivity of 0.51 aN Hz(-1/2). This measurement is a critical step towards observing quantum behaviour in a mechanical object.

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Nanomechanical motion measured with an imprecision below the standard quantum limit

The importance of thermoelastic damping as a fundamental dissipation mechanism for small-scale mechanical resonators is evaluated in light of recent efforts to design high-Q micrometer- and nanometer-scale electromechanical systems. The equations of linear thermoelasticity are used to give a simple derivation for thermoelastic damping of small flexural vibrations in thin beams. It is shown that Zener’s well-known approximation by a Lorentzian with a single thermal relaxation time slightly deviates from the exact expression.

Thermoelastic Damping in Micro- and Nano-Mechanical Systems.

Graphene and related two-dimensional (2D) materials associate remarkable mechanical, electronic, optical and phononic properties. As such, 2D materials are promising for hybrid systems that couple their elementary excitations (excitons, phonons) to their macroscopic mechanical modes. These built-in systems may yield enhanced strain-mediated coupling compared to bulkier architectures, e.g., comprising a single quantum emitter coupled to a nano-mechanical resonator. Here, using micro-Raman spectroscopy on pristine monolayer graphene drums, we demonstrate that the macroscopic flexural vibrations of graphene induce dynamical optical phonon softening. This softening is an unambiguous fingerprint of dynamically-induced tensile strain that reaches values up to ≈4 × 10−4 under strong non-linear driving. Such non-linearly enhanced strain exceeds the values predicted for harmonic vibrations with the same root mean square (RMS) amplitude by more than one order of magnitude. Our work holds promise for dynamical strain engineering and dynamical strain-mediated control of light-matter interactions in 2D materials and related heterostructures. Here, the authors use Raman spectroscopy on circular graphene drums to demonstrate dynamical softening of optical phonons induced by the macroscopic flexural motion of graphene, and find evidence that the strain in graphene is enhanced under non-linear driving.

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Dynamically-enhanced strain in atomically thin resonators.

Abstract The quantum ground state of a massive mechanical system is a stepping stone for investigating macroscopic quantum states and building high fidelity sensors. With the recent achievement of ground-state cooling of a single motional mode, levitated nanoparticles have entered the quantum domain. To overcome detrimental cross-coupling and decoherence effects, quantum control needs to be expanded to more system dimensions, but the effect of a decoupled dark mode has so far hindered cavity-based ground-state cooling of multiple mechanical modes. Here, we demonstrate two-dimensional ground-state cooling of an optically levitated nanoparticle. Utilizing coherent scattering into an optical cavity mode, we reduce the occupation numbers of two separate centre-of-mass modes to 0.83 and 0.81, respectively. By controlling the frequency separation and the cavity coupling strengths of the nanoparticle’s mechanical modes, we show the transition from 1D to 2D ground-state cooling. This 2D control lays the foundations for quantum-limited orbital angular momentum states for rotation sensing and, combined with ground-state cooling along the third motional axis shown previously, may allow full 3D ground-state cooling of a massive object. 

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Simultaneous ground-state cooling of two mechanical modes of a levitated nanoparticle

Nanomechanics has brought mesoscopic physics into the world of vibrations. Because nanomechanical systems are small, fluctuations are significant, the vibrations become nonlinear already for comparatively small amplitudes, and new mechanisms of dissipation come into play. At the same time, the exquisite control of these systems makes them a platform for studying many problems of classical and quantum physics far from thermal equilibrium in a well-characterized setting. This review describes, at a conceptual level, basic theoretical ideas and explicative experiments pertaining to mesoscopic physics of nanomechanical systems. Major applications of nanomechanics in science and technology are also outlined. A broad range of phenomena related to the conservative as well as dissipative nonlinearity and fluctuations are discussed within a unifying framework. They include the linear response of single and coupled vibrational modes as well as nonlinear effects of periodic driving. Such driving breaks the continuous time-translation symmetry and the detailed balance, with conspicuous consequences for fluctuations, particularly in the presence of the driving-induced bi- and multistability. Mathematical techniques are described in the appendices to streamline the reading, but also to provide an introduction to the theory. The goal of the review is to show the richness of the physics at work. The continuous experimental and theoretical advances make nanomechanical systems a vibrant area of research, with many new phenomena to discover. 

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Mesoscopic physics of nanomechanical systems

The nature of the quantum-to-classical crossover remains one of the most challenging open question of Science to date. In this respect, moving objects play a specific role. Pioneering experiments over the last few years have begun exploring quantum behaviour of micron-sized mechanical systems, either by passively cooling single GHz modes, or by adapting laser cooling techniques developed in atomic physics to cool specific low-frequency modes far below the temperature of their surroundings. Here instead we describe a very different approach, passive cooling of a whole micromechanical system down to 500 μK, reducing the average number of quanta in the fundamental vibrational mode at 15 MHz to just 0.3 (with even lower values expected for higher harmonics); the challenge being to be still able to detect the motion without disturbing the system noticeably. With such an approach higher harmonics and the surrounding environment are also cooled, leading to potentially much longer mechanical coherence times, and enabling experiments questioning mechanical wave-function collapse, potentially from the gravitational background, and quantum thermodynamics. Beyond the average behaviour, here we also report on the fluctuations of the fundamental vibrational mode of the device in-equilibrium with the cryostat. These reveal a surprisingly complex interplay with the local environment and allow characteristics of two distinct thermodynamic baths to be probed. Compared to active techniques, passive cooling of mechanical modes allows to work with devices in equilibrium with their environment without excess damping. Here, the authors demonstrate passive cooling and thermalisation of a 15 μm drum-head device with MHz fundamental flexure to its quantum ground state.

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A macroscopic object passively cooled into its quantum ground state of motion beyond single-mode cooling.

We apply the well-established theoretical method developed for geometrical nonlinearities of micro-/nano-mechanical clamped beams to circular drums. The calculation is performed under the same hypotheses, the extra difficulty being to analytically describe the (coordinate-dependent) additional stress generated in the structure by the motion. Specifically, the model applies to non-axisymmetric mode shapes. An analytic expression is produced for the Duffing (hardening) nonlinear coefficient, which requires only the knowledge of the mode shape functions to be evaluated. This formulation is simple to handle and does not rely on complex numerical methods. Moreover, no hypotheses are made on the drive scheme and the nature of the in-plane stress: it is not required to be of an electrostatic origin. We confront our predictions with both typical experimental devices and relevant theoretical results from the literature. Generalization of the presented method to Duffing-type mode-coupling should be a straightforward extension of this work. We believe that the presented modeling will contribute to the development of nonlinear physics implemented in 2D micro-/nano-mechanical structures.

Geometrical nonlinearity of circular plates and membranes: An alternative method

We explore the nonlinear dynamics of a cavity optomechanical system. Our realization consisting of a drumhead nano-electro-mechanical resonator (NEMS) coupled to a microwave cavity, allows for a nearly ideal platform to study the nonlinearities arising purely due to radiation-pressure physics. Experiments are performed under a strong microwave Stokes pumping which triggers mechanical self-sustained oscillations. We analyze the results in the framework of an extended nonlinear optome-chanical theory, and demonstrate that quadratic and cubic coupling terms in the opto-mechanical Hamiltonian have to be considered. Quantitative agreement with the measurements is obtained considering only genuine geometrical nonlinearities: no thermo-optical instabilities are observed, in contrast with laser-driven systems. Based on these results, we describe a method to quantify nonlin-ear properties of microwave optomechanical devices. Such a technique, available now in the quantum electro-mechanics toolbox, but completely generic, is mandatory for the development of new schemes where higher-order coupling terms are proposed as a new resource, like Quantum Non-Demolition measurements, or in the search for new fundamental quantum signatures, like Quantum Gravity. We also find that the motion imprints a wide comb of extremely narrow peaks in the microwave output field, which could also be exploited in specific microwave-based measurements, potentially limited only by the quantum noise of the optical and the mechanical fields for a ground-state cooled NEMS device.

https://hal.archives-ouvertes.fr/hal-02949631/document

Beyond linear coupling in microwave optomechanics

We report on the generic classical electric circuit modeling that describes standard single-tone microwave optomechanics. Based on a parallel RLC circuit in which a mechanical oscillator acts as a movable capacitor, derivations of analytical expressions are presented, including key features such as the back-action force, the input-output expressions, and the spectral densities associated, all in the classical regime. These expressions coincide with the standard quantum treatment performed in optomechanics when the occupation number of both cavity and mechanical oscillator are large. Besides, the derived analytics transposes optical elements and properties into electronics terms, which is mandatory for quantitative measurement and design purposes. Finally, the direct comparison between the standard quantum treatment and the classical model addresses the bounds between quantum and classical regimes, highlighting the features which are truly quantum, and those which are not.

Electric circuit model of microwave optomechanics

We report on measurements of dissipation and frequency noise at millikelvin temperatures of nanomechanical devices covered with aluminum. A clear excess damping is observed after switching the metallic layer from superconducting to the normal state with a magnetic field. Beyond the standard model of internal tunneling systems coupled to the phonon bath, here we consider the relaxation to the conduction electrons together with the nature of the mechanical dispersion laws for stressed/unstressed devices. With these key ingredients, a model describing the relaxation of two-level systems inside the structure due to interactions with electrons and phonons with well separated timescales captures the data. In addition, we measure an excess 1/f-type frequency noise in the normal state, which further emphasizes the impact of conduction electrons.

Dylan Cattiaux

Papers

A macroscopic object passively cooled into its quantum ground state of motion beyond single-mode cooling.

Geometrical nonlinearity of circular plates and membranes: An alternative method

Beyond linear coupling in microwave optomechanics

Electric circuit model of microwave optomechanics

Nanomechanical damping via electron-assisted relaxation of two-level systems