Recent years have seen a rapid expansion of research into nanophotonics based on surface plasmon–polaritons. These electromagnetic waves propagate along metal–dielectric interfaces and can be guided by metallic nanostructures beyond the diffraction limit. This remarkable capability has unique prospects for the design of highly integrated photonic signal-processing systems, nanoresolution optical imaging techniques and sensors. This Review summarizes the basic principles and major achievements of plasmon guiding, and details the current state-of-the-art in subwavelength plasmonic waveguides, passive and active nanoplasmonic components for the generation, manipulation and detection of radiation, and configurations for the nanofocusing of light. Potential future developments and applications of nanophotonic devices and circuits are also discussed, such as in optical signals processing, nanoscale optical devices and near-field microscopy with nanoscale resolution.

Plasmonics beyond the diffraction limit

In 1873, Ernst Abbe discovered what was to become a well-known paradigm: the inability of a lens-based optical microscope to discern details that are closer together than half of the wavelength of light. However, for its most popular imaging mode, fluorescence microscopy, the diffraction barrier is crumbling. Here, I discuss the physical concepts that have pushed fluorescence microscopy to the nanoscale, once the prerogative of electron and scanning probe microscopes. Initial applications indicate that emergent far-field optical nanoscopy will have a strong impact in the life sciences and in other areas benefiting from nanoscale visualization.

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Far-Field Optical Nanoscopy

Artificially engineered metamaterials are now demonstrating unprecedented electromagnetic properties that cannot be obtained with naturally occurring materials. In particular, they provide a route to creating materials that possess a negative refractive index and offer exciting new prospects for manipulating light. This review describes the recent progress made in creating nanostructured metamaterials with a negative index at optical wavelengths, and discusses some of the devices that could result from these new materials.

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Optical negative-index metamaterials

Metamaterials, or engineered materials with rationally designed, subwavelength-scale building blocks, allow us to control the behavior of physical fields in optical, microwave, radio, acoustic, heat transfer, and other applications with flexibility and performance that are unattainable with naturally available materials. In turn, metasurfaces-planar, ultrathin metamaterials-extend these capabilities even further. Optical metasurfaces offer the fascinating possibility of controlling light with surface-confined, flat components. In the planar photonics concept, it is the reduced dimensionality of the optical metasurfaces that enables new physics and, therefore, leads to functionalities and applications that are distinctly different from those achievable with bulk, multilayer metamaterials. Here, we review the progress in developing optical metasurfaces that has occurred over the past few years with an eye toward the promising future directions in the field.

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Planar Photonics with Metasurfaces

We present the science and technology roadmap for graphene, related two-dimensional crystals, and hybrid systems, targeting an evolution in technology, that might lead to impacts and benefits reaching into most areas of society. This roadmap was developed within the framework of the European Graphene Flagship and outlines the main targets and research areas as best understood at the start of this ambitious project. We provide an overview of the key aspects of graphene and related materials (GRMs), ranging from fundamental research challenges to a variety of applications in a large number of sectors, highlighting the steps necessary to take GRMs from a state of raw potential to a point where they might revolutionize multiple industries. We also define an extensive list of acronyms in an effort to standardize the nomenclature in this emerging field.

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Science and technology roadmap for graphene, related two-dimensional crystals, and hybrid systems

We present a novel formalism to describe diffractive optics of metasurfaces, diffractive interface theory (DIT).

Diffraction interface theory: A nonlocal approach to metasurfaces

We present a technique for subwavelength far-field focusing of light in planar non-resonant structures. The approach
combines the diffraction gratings that generate high-wavevector waves and planar slabs of homogeneous anisotropic
metamaterials that propagate these waves and combine them at the subwavelength focal spots. The technique has all the
benefits of Fresnel lens, near-field zone plate, hyperlens, and superlens, and at the same time resolves their fundamental
limitations. Several realizations of hypergratings for visible, near-IR, and mid-IR frequencies are proposed, and their
performance is analyzed. Generalization of the developed approach for sub-diffractional imaging and on-chip photonics
is suggested.

Hypergratings: far-field subwavelength focusing in planar metamaterials

We propose to use silver/gold sandwich structures to combine the advantages of silver and gold - two materials of choice for nanoplasmoics and metamaterials. We report on the preparation, characterization, and theoretical modeling of the proposed system.

Surface plasmon polaritons in silver-gold sandwich structure

We study optical properties of metal nanowires and show that electric and magnetic dipole responses of the coupled-wire system can be both opposite to the excitation irradiation. This opens up the possibility to develop left-handed materials based on metal nanowires with negative refraction in the near-infrared and optical spectral ranges.

Plasmonic nanowires as left-handed media

The interaction of free electrons with electromagnetic excitation is the fundamental mechanism responsible for ultra-strong confinement of light that, in turn, enables biosensing, near-field microscopy, optical cloaking, sub-wavelength focusing, and super-resolution imaging. These unique phenomena and functionalities critically rely on the negative permittivity of optical elements resulting from the free electrons. As result, progress in nanophotonics and nano-optics is often related to the development of new negative permittivity (plasmonic) media at the optical frequency of interest. Here we show that the essential mobility of free charge carriers in such conducting media dramatically alters the well-known optical response of free electron gases. We demonstrate that a ballistic resonance associated with the interplay of the time-periodic motion of the free electrons in the confines of a sub-wavelength scale nanostructure and the time periodic electromagnetic field leads to a dramatic enhancement of the electric polarization of the medium - to the point where a plasmonic response can be achieved in a composite material using only positive bulk permittivity components. This ballistic resonance opens the fields of plasmonics, nanophotonics, and metamaterials to many new constituent materials that until now were considered unsuitable for such applications, and extends the operational frequency range of existing materials to substantially shorter wavelengths. As a proof of concept, we experimentally demonstrate that ballistic resonance in all-semiconductor metamaterials results in strongly anisotropic (hyperbolic) response well above the plasma frequencies of the metamaterial components.

Viktor A. Podolskiy

Papers

Diffraction interface theory: A nonlocal approach to metasurfaces

Hypergratings: far-field subwavelength focusing in planar metamaterials

Surface plasmon polaritons in silver-gold sandwich structure

Plasmonic nanowires as left-handed media

Ballistic Metamaterials