Femtosecond filamentation in transparent media

Summary form only given. Fundamental processes in atoms, molecules, as well as condensed matter are triggered or mediated by the motion of electrons inside or between atoms. Electronic dynamics on atomic length scales tends to unfold within tens to thousands of attoseconds (1 attosecond [as] = 10-18 s). Recent breakthroughs in laser science are now opening the door to watching and controlling these hitherto inaccessible microscopic dynamics. The key to accessing the attosecond time domain is the control of the electric field of (visible) light, which varies its strength and direction within less than a femtosecond (1 femtosecond = 1000 attoseconds). Atoms exposed to a few oscillations cycles of intense laser light are able to emit a single extreme ultraviolet (XUV) burst lasting less than one femtosecond. Full control of the evolution of the electromagnetic field in laser pulses comprising a few wave cycles have recently allowed the reproducible generation and measurement of isolated sub-femtosecond XUV pulses, demonstrating the control of microscopic processes (electron motion and photon emission) on an attosecond time scale. These tools have enabled us to visualize the oscillating electric field of visible light with an attosecond "oscilloscope", to control single-electron and probe multi-electron dynamics in atoms, molecules and solids. Recent experiments hold promise for the development of an attosecond X-ray source, which may pave the way towards 4D electron imaging with sub-atomic resolution in space and time.

Attosecond Physics

Modern laser sources nowadays deliver ultrashort light pulses reaching few cycles in duration and peak powers exceeding several terawatt (TW). When such pulses propagate through optically transparent media, they first self-focus in space and grow in intensity, until they generate a tenuous plasma by photo-ionization. For free electron densities and beam intensities below their breakdown limits, these pulses evolve as self-guided objects, resulting from successive equilibria between the Kerr focusing process, the chromatic dispersion of the medium and the defocusing action of the electron plasma. Discovered one decade ago, this self-channeling mechanism reveals a new physics, widely extending the frontiers of nonlinear optics. Implications include long-distance propagation of TW beams in the atmosphere, supercontinuum emission, pulse shortening as well as high-order harmonic generation. This review presents the landmarks of the 10-odd-year progress in this field. Particular emphasis is laid on the theoretical modeling of the propagation equations, whose physical ingredients are discussed from numerical simulations. The dynamics of single filaments created over laboratory scales in various materials such as noble gases, liquids and dielectrics reveal new perspectives in pulse shortening techniques. Far-field spectra provide promising diagnostics. Attention is also paid to the multifilamentation instability of broad beams, breaking up the energy distribution into small-scale cells along the optical path. The robustness of the resulting filaments in adverse weathers, their large conical emission exploited for multipollutant remote sensing, nonlinear spectroscopy and the possibility of guiding electric discharges in air are finally addressed on the basis of experimental results.

https://iopscience.iop.org/article/10.1088/0034-4885/70/10/R03/pdf

Ultrashort filaments of light in weakly ionized, optically transparent media

The state of the art of investigations on filamentation of a high-power femtosecond laser radiation in transparent media is reviewed. The physical picture of this phenomenon is presented and its relation to the fundamental concepts of nonlinear optics and practical applications is demonstrated. Experimental and theoretical methods are briefly considered and laser radiation parameters in the case of filamentation are given. The review can be of interest both for specialists and researches wanting to become familiar with a new, rapidly developing direction in laser physics.

https://iopscience.iop.org/article/10.1070/QE2009v039n03ABEH013916/pdf

Filamentation of high-power femtosecond laser radiation

This is a review of some recent development in femtosecond filamentation science with emphasis on our collective work. Previously reviewed work in the field will not be discussed. We thus start with a very brief description of the fundamental physics of single filamentation of powerful femtosecond laser pulses in air. Intensity clamping is emphasized. One consequence is that the peak intensity inside one or more filaments would not increase significantly even if one focuses the pulse at very high peak power even up to the peta-watt level. Another is that the clamped intensity is independent of pressure. One interesting outcome of the high intensity inside a filament is filament fusion which comes from the nonlinear change of index of refraction inside the filament leading to cross beam focusing. Because of the high intensity inside the filament, one can envisage nonlinear phenomena taking place inside a filament such as a new type of Raman red shift and the generation of very broad band supercontinuum into the infrared through four-wave-mixing. This is what we call by filamentation nonlinear optics. It includes also terahertz generation from inside the filament. The latter is discussed separately because of its special importance to those working in the field of safety and security in recent years. When the filamenting pulse is linearly polarized, the isotropic nature of air becomes birefringent both electronically (instantaneous) and through molecular wave packet rotation and revival (delayed). Such birefringence is discussed in detailed. Because, in principle, a filament can be projected to a long distance in air, applications to pollution measurement as well as other atmospheric science could be earned out. We call this filamentation atmospheric science. Thus, the following subjects are discussed briefly, namely, lightning control, rain making, remote measurement of electric field, microwave guidance and remote sensing of pollutants. A discussion on the higher order Kerr effect on the physics of filamentation is also given. This is a new hot subject of current debate. This review ends on giving our view of the prospect of progress of this field of filamentation in the future. We believe it hinges upon the development of the laser technology based upon the physical understanding of filamentation and on the reduction in price of the laser system.

Advances in intense femtosecond laser filamentation in air

Pulse self-compression in normally dispersive bulk media

The spectral and the temporal behavior of high-intensity negatively chirped femtosecond pulses in normally dispersive media at different input parameters are experimentally studied. The spectrum of the pulse is reshaped due to strong self-actions. The pulse is self-compressed, instead of broadening, accompanied with the spectral FWHM bandwidth shortened. Steepening of the leading edge of the pulse and spectral red-shift are observed in the experiment. The numerical simulation shows that the result is in agreement with the experimental result.

Spectrum reshaping and pulse self-compression in normally dispersive media with negatively chirped femtosecond pulses.

Two-cycle optical pulses with duration of 5 fs and energy of 0.7 mJ have been generated at 1 kHz by compressing the 38 fs laser pulses from a carrier-envelope phase (CEP) controlled Ti:sapphire laser system through a cascade filamentation compression technique. A simple and effective method is developed to suppress multiple filament formation and stabilize a single filament by inserting a soft aperture with an appropriate diameter into the driving laser beam prior to focusing, resulting in an excellent compressed beam quality. The good beam quality and potentially higher peak power make this ultrashort laser pulse source a significant tool for high-field physics applications.

Generation of 5 fs, 0.7 mJ pulses at 1 kHz through cascade filamentation

We experimentally demonstrate the generation of an extreme-ultraviolet (XUV) supercontinuum in argon with a two-color laser field consisting of an intense 7 fs pulse at 800 nm and a relatively weak 37 fs pulse at 400 nm. By controlling the relative time delay between the two laser pulses, we observe enhanced high-order harmonic generation as well as spectral broadening of the supercontinuum. A method to produce isolated attosecond pulses with variable width and intensity is proposed.

Enhancement and broadening of extreme-ultraviolet supercontinuum in a relative phase controlled two-color laser field.

A optical parameter chirp pulse amplification laser system, includes a titanium gem femtosecond mode-locking pulse oscillator, a first splitting film, a CEP steady signal pulse source, an OPCPA synchronous pumping source, an OPCPA amplifier stage and compressor. In the output beam direction of the titanium gem femtosecond mode-locking pulse oscillator is the first splitting film, which divides a laser beam into a transmission light beam and a reflection light beam, and in the said transmission light beam is said CEP steady signal pulse source, OPCPA amplifier stage and compressor in order. The said CEP steady signal pulse source comprises a photonic crystal optical fiber, a chirp mirror, a period polarization lithium niobate crystal and a stretcher; said OPCPA amplifier stage comprises a first two-tone mirror, a first nonlinear crystal, a second two-tone mirror and a second nonlinear crystal; said OPCPA synchronous pumping source comprises a Q-tuning frequency-multiplier YAG laser, a narrowband titanium gem regenerating amplifier and a second splitting film, and a holophote. The invention apparatus may get a near-infrared ultrashort laser pulse output with a pulse width less than 30 femtoseconds.

Xiaowei Chen

Papers

Pulse self-compression in normally dispersive bulk media

Spectrum reshaping and pulse self-compression in normally dispersive media with negatively chirped femtosecond pulses.

Generation of 5 fs, 0.7 mJ pulses at 1 kHz through cascade filamentation

Enhancement and broadening of extreme-ultraviolet supercontinuum in a relative phase controlled two-color laser field.

Optical parameter chirp impulse amplification laser system