/pdf/laser-ablation-for-analytical-sampling-what-can-we-learn-1ro1qr2fjg.pdf

Laser ablation for analytical sampling: what can we learn from modeling?

The pulsed laser deposition is a new technique for the growth of thin films,which has been attended generally by people recently The physical principle, unique characteristics and the proceeding of the study were introduced briefly In addation, the result of the PtSi nanometer thin film based on silicon prepared by the pulsed laser deposition was describedPULS

Pulsed laser deposition of thin films

Effect of laser parameters on laser ablation and laser-induced plasma formation: A numerical modeling investigation

We investigated spatio-temporal evolution of ns laser ablation plumes at atmospheric pressure, a favored condition for laser-induced breakdown spectroscopy and laser-ablation inductively coupled plasma mass-spectrometry. The 1064 nm, 6 ns pulses from a Nd:YAG laser were focused on to an Al target and the generated plasma was allowed to expand in 1 atm Ar. The hydrodynamic expansion features were studied using focused shadowgraphy and gated 2 ns self-emission visible imaging. Shadowgram images showed material ejection and generation of shock fronts. A secondary shock is observed behind the primary shock during the time window of 100-500 ns with instabilities near the laser cone angle. By comparing the self-emission images obtained using fast photography, it is concluded that the secondary shocks observed in the shadowgraphy were generated by fast moving target material. The plume front estimates using fast photography exhibited reasonable agreement with data obtained from shadowgraphy at early times ≤400 n...

Experimental and computational study of complex shockwave dynamics in laser ablation plumes in argon atmosphere

A one-dimensional gas-dynamic model is presented for the laser ablation of Cu and the expansion of the Cu vapor in a background gas (He) at 1atm. The ionization of Cu and He, the inverse bremsstrahlung absorption processes and photoionization process, and the back flux onto the target are considered simultaneously. The binary diffusion, the viscosity, and the thermal conduction including the electron thermal conduction are considered as well. Numerical results show that the consideration of ionization and laser absorption in the plume greatly influences the gas dynamics. The ionization of Cu enables the recondensation at the target surface to happen even during the laser pulse. The ionization degree of Cu and He may change greatly with the location in the plume. For laser irradiances ranging from 2to9×1012W∕m2, the simulations show that the second-order ionization of Cu competes with the first-order ionization. In the region close to the target surface, the first-order ionization of Cu dominates. In the c...

Laser ablation of Cu and plume expansion into 1 atm ambient gas

The effect of ambient gas on the expansion dynamics of the plasma generated by laser ablation of an aluminum target has been investigated using frequency doubled radiation from a Q-switched Nd:YAG laser. The diagnostic tools include fast photography of overall visible plume emission using a 2 ns gated intensified charged coupled device and space and time resolved emission spectroscopy using a 50 cm monochromator/spectrograph and photomultiplier tube. The expansion behavior of the plasma was studied with ambient air pressure ranging from 10−6 to 100 Torr. Free expansion, plume splitting and sharpening, hydrodynamic instability, and stagnation of the plume were observed at different pressure levels. Space and time resolved emission spectroscopic studies showed a twin peak distribution for Al and Al+ species at farther distances illustrating plume splitting at pressures higher than 100 mTorr. Combining imaging together with time resolved emission diagnostics, a triple structure of the plume was observed. The expansion of the plume front was compared with various expansion models and found to be generally in good agreement.

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Internal structure and expansion dynamics of laser ablation plumes into ambient gases

Plume splitting and sharpening were observed in laser-produced aluminium plasma created using 532 nm, 8 ns pulses from a frequency doubled Nd : YAG laser. Measurements were made using 2 ns gated fast photography as well as space and time resolved optical emission spectroscopy. The motion of the leading edge of the plume was studied with several background air pressures and the expansion of the plume front was compared with various expansion models. Combining imaging together with time resolved emission diagnostics, a triple structure of the plume was observed.

/pdf/plume-splitting-and-sharpening-in-laser-produced-aluminium-4pzrxkqimu.pdf

Plume splitting and sharpening in laser-produced aluminium plasma

The energy absorption and laser propagation characteristics of air and argon sparks at one atmosphere have been investigated. To create the sparks, 532 nm pulses from a frequency doubled Q-switched Nd : YAG laser are used. We employed 2 ns gated fast photography for studying the time evolution of the kernel at early times. Optical emission spectroscopy is used to infer temperature and density of the sparks. Significant energy absorption by the plasma is observed just above the breakdown threshold. The energy absorption and propagation in the spark indicated that argon plasma is more absorptive than air plasma. The absorption of the spark increases with laser energy, and at higher energies absorption saturation is observed. A spiky behavior is observed in the transmitted temporal profiles of lasers at higher energies and this is explained as due to the formation of a self-regulating regime.

/pdf/energy-absorption-and-propagation-in-laser-created-sparks-14d2t9ff3l.pdf

Energy Absorption and Propagation in Laser-Created Sparks

The energy absorption and laser propagation characteristics of air and argon sparks at one atmosphere have been investigated. To create the sparks, 532 nm pulses from a frequency doubled Q-switched Nd: YAG laser are used. We employed 2 ns gated fast photography for studying the time evolution of the kernel at early times. Optical emission spectroscopy is used to infer temperature and density of the sparks. Significant energy absorption by the plasma is observed just above the breakdown threshold. The energy absorption and propagation in the spark indicated that argon plasma is more absorptive than air plasma. The absorption of the spark increases with laser energy, and at higher energies absorption saturation is observed. A spiky behavior is observed in the transmitted temporal profiles of lasers at higher energies and this is explained as due to the formation of a self-regulating regime.

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Energy absorption and propagation in laser-created sparks - eScholarship

The laser propagation and energy absorption of an argon spark induced by a laser at different pressures is investigated. 8 ns pulses from a frequency-doubled Q-switched Nd:YAG laser are used to create the spark. The pressure of the argon is varied from 1 atm to 10 Torr. Significant energy absorption by the plasma is observed at high pressures (>100 Torr) while there is negligible absorption when the pressure is lower than 50 Torr. The plasma kernel showed distinct behavior with respect to laser energy. At a laser energy well above the breakdown threshold, the spark moved only in the backward direction and the forward component was absent indicating the strong absorption of the laser by the spark front. A spiky behavior is observed in the transmitted temporal profiles of the laser at higher energies and at high pressures and can be due to the formation of a self-regulating regime.

/pdf/laser-propagation-and-energy-absorption-by-an-argon-spark-4mbvu6t3dv.pdf

A. C. Gaeris

Papers

Internal structure and expansion dynamics of laser ablation plumes into ambient gases

Plume splitting and sharpening in laser-produced aluminium plasma

Energy Absorption and Propagation in Laser-Created Sparks

Energy absorption and propagation in laser-created sparks - eScholarship

Laser propagation and energy absorption by an argon spark