Air quality impacts from wildfires have been dramatic in recent years, with millions of people exposed to elevated and sometimes hazardous fine particulate matter (PM 2.5 ) concentrations for exten...

https://www.tandfonline.com/doi/pdf/10.1080/10962247.2020.1747802

Wildfire and prescribed burning impacts on air quality in the United States.

The Black Summer fire season of 2019–2020 in southeastern Australia contributed to an intense ‘super outbreak’ of fire-induced and smoke-infused thunderstorms, known as pyrocumulonimbus (pyroCb). More than half of the 38 observed pyroCbs injected smoke particles directly into the stratosphere, producing two of the three largest smoke plumes observed at such altitudes to date. Over the course of 3 months, these plumes encircled a large swath of the Southern Hemisphere while continuing to rise, in a manner consistent with existing nuclear winter theory. We connect cause and effect of this event by quantifying the fire characteristics, fuel consumption, and meteorology contributing to the pyroCb spatiotemporal evolution. Emphasis is placed on the unusually long duration of sustained pyroCb activity and anomalous persistence during nighttime hours. The ensuing stratospheric smoke plumes are compared with plumes injected by significant volcanic eruptions over the last decade. As the second record-setting stratospheric pyroCb event in the last 4 years, the Australian super outbreak offers new clues on the potential scale and intensity of this increasingly extreme fire-weather phenomenon in a warming climate.

/pdf/australia-s-black-summer-pyrocumulonimbus-super-outbreak-4vch8xg5s3.pdf

Australia’s Black Summer pyrocumulonimbus super outbreak reveals potential for increasingly extreme stratospheric smoke events

. We present particle optical properties of stratospheric smoke layers observed with multiwavelength polarization Raman lidar over Punta Arenas (53.2 ∘  S, 70.9 ∘  W), Chile, at the southernmost tip of South America in January 2020. The smoke originated from the record-breaking bushfires in Australia. The stratospheric aerosol optical thickness reached values up to 0.85 at 532 nm in mid-January 2020. The main goal of this rapid communication letter is to provide first stratospheric measurements of smoke extinction-to-backscatter ratios (lidar ratios) and particle linear depolarization ratios at 355 and 532 nm wavelengths. These aerosol parameters are important input parameters in the analysis of spaceborne CALIPSO and Aeolus lidar observations of the Australian smoke spreading over large parts of the Southern Hemisphere in January and February 2020 up to heights of around 30 km. Lidar and depolarization ratios, simultaneously measured at 355 and 532 nm, are of key importance regarding the homogenization of the overall Aeolus (355 nm wavelength) and CALIPSO (532 nm wavelength) lidar data sets documenting the spread of the smoke and the decay of the stratospheric perturbation, which will be observable over the entire year of 2020. We found typical values and spectral dependencies of the lidar ratio and linear depolarization ratio for aged stratospheric smoke. At 355 nm, the lidar ratio and depolarization ratio ranged from 53 to 97 sr (mean 71 sr) and 0.2 to 0.26 (mean 0.23), respectively. At 532 nm, the lidar ratios were higher (75–112 sr, mean 97 sr) and the depolarization ratios were lower with values of 0.14–0.22 (mean 0.18). The determined depolarization ratios for aged Australian smoke are in very good agreement with respective ones for aged Canadian smoke, observed with lidar in stratospheric smoke layers over central Europe in the summer of 2017. The much higher 532 nm lidar ratios, however, indicate stronger absorption by the Australian smoke particles.

/pdf/smoke-of-extreme-australian-bushfires-observed-in-the-24zgpa41j2.pdf

Smoke of extreme Australian bushfires observed in the stratosphere over Punta Arenas, Chile, in January 2020: optical thickness, lidar ratios, and depolarization ratios at 355 and 532 nm

AbstractWe describe and show results from a series of field campaigns that used balloonborne instruments launched from India and Saudi Arabia during the summers 2014–17 to study the nature, formati...

BATAL: Balloon measurement campaigns of the Asian Tropopause Aerosol Layer

Significance Large wildfires have been observed to inject smoke into the stratosphere, raising questions about their potential to affect the stratospheric ozone layer that protects life on Earth from biologically damaging ultraviolet radiation. Multiple observations of aerosol and NO2 concentrations from three independent satellite instruments are used here together with model calculations to identify decreases in stratospheric NO2 concentrations following major Australian 2019 through 2020 wildfires. The data confirm that important chemistry did occur on the smoke particle surfaces. The observed behavior in NO2 with increasing particle concentrations is a marker for surface chemistry that contributes to midlatitude ozone depletion. The results indicate that increasing wildfire activity in a warming world may slow the recovery of the ozone layer.

On the stratospheric chemistry of midlatitude wildfire smoke

. Six months of stratospheric aerosol observations with the European Aerosol Research Lidar Network (EARLINET) from August 2017 to January 2018 are presented. The decay phase of an unprecedented, record-breaking stratospheric perturbation caused by wildfire smoke is reported and discussed in terms of geometrical, optical, and microphysical aerosol properties. Enormous amounts of smoke were injected into the upper troposphere and lower stratosphere over fire areas in western Canada on 12 August 2017 during strong thunderstorm–pyrocumulonimbus activity. The stratospheric fire plumes spread over the entire Northern Hemisphere in the following weeks and months. Twenty-eight European lidar stations from northern Norway to southern Portugal and the eastern Mediterranean monitored the strong stratospheric perturbation on a continental scale. The main smoke layer (over central, western, southern, and eastern Europe) was found at heights between 15 and 20 km since September 2017 (about 2 weeks after entering the stratosphere). Thin layers of smoke were detected at heights of up to 22–23 km. The stratospheric aerosol optical thickness at 532 nm decreased from values >  0.25 on 21–23 August 2017 to 0.005–0.03 until 5–10 September and was mainly 0.003–0.004 from October to December 2017 and thus was still significantly above the stratospheric background (0.001–0.002). Stratospheric particle extinction coefficients (532 nm) were as high as 50–200 Mm −1 until the beginning of September and on the order of 1 Mm −1 (0.5–5 Mm −1 ) from October 2017 until the end of January 2018. The corresponding layer mean particle mass concentration was on the order of 0.05–0.5  µ g m −3 over these months. Soot particles (light-absorbing carbonaceous particles) are efficient ice-nucleating particles (INPs) at upper tropospheric (cirrus) temperatures and available to influence cirrus formation when entering the tropopause from above. We estimated INP concentrations of 50–500 L −1 until the first days in September and afterwards 5–50 L −1 until the end of the year 2017 in the lower stratosphere for typical cirrus formation temperatures of − 55  ∘ C and an ice supersaturation level of 1.15. The measured profiles of the particle linear depolarization ratio indicated a predominance of nonspherical smoke particles. The 532 nm depolarization ratio decreased slowly with time in the main smoke layer from values of 0.15–0.25 (August–September) to values of 0.05–0.10 (October–November) and  0.05 (December–January). The decrease of the depolarization ratio is consistent with aging of the smoke particles, growing of a coating around the solid black carbon core (aggregates), and thus change of the shape towards a spherical form. We found ascending aerosol layer features over the most southern European stations, especially over the eastern Mediterranean at 32–35 ∘  N, that ascended from heights of about 18–19 to 22–23 km from the beginning of October to the beginning of December 2017 (about 2 km per month). We discuss several transport and lifting mechanisms that may have had an impact on the found aerosol layering structures.

/pdf/the-unprecedented-2017-2018-stratospheric-smoke-event-decay-3knbnwf9zl.pdf

Karen Acheson

Papers

The unprecedented 2017–2018 stratospheric smoke event: decay phase and aerosol properties observed with the EARLINET