Summary form only given. Fundamental processes in atoms, molecules, as well as condensed matter are triggered or mediated by the motion of electrons inside or between atoms. Electronic dynamics on atomic length scales tends to unfold within tens to thousands of attoseconds (1 attosecond [as] = 10-18 s). Recent breakthroughs in laser science are now opening the door to watching and controlling these hitherto inaccessible microscopic dynamics. The key to accessing the attosecond time domain is the control of the electric field of (visible) light, which varies its strength and direction within less than a femtosecond (1 femtosecond = 1000 attoseconds). Atoms exposed to a few oscillations cycles of intense laser light are able to emit a single extreme ultraviolet (XUV) burst lasting less than one femtosecond. Full control of the evolution of the electromagnetic field in laser pulses comprising a few wave cycles have recently allowed the reproducible generation and measurement of isolated sub-femtosecond XUV pulses, demonstrating the control of microscopic processes (electron motion and photon emission) on an attosecond time scale. These tools have enabled us to visualize the oscillating electric field of visible light with an attosecond "oscilloscope", to control single-electron and probe multi-electron dynamics in atoms, molecules and solids. Recent experiments hold promise for the development of an attosecond X-ray source, which may pave the way towards 4D electron imaging with sub-atomic resolution in space and time.

Attosecond Physics

Ion acceleration driven by superintense laser pulses is attracting an impressive and steadily increasing effort. Motivations can be found in the applicative potential and in the perspective to investigate novel regimes as available laser intensities will be increasing. Experiments have demonstrated, over a wide range of laser and target parameters, the generation of multi-MeV proton and ion beams with unique properties such as ultrashort duration, high brilliance, and low emittance. An overview is given of the state of the art of ion acceleration by laser pulses as well as an outlook on its future development and perspectives. The main features observed in the experiments, the observed scaling with laser and plasma parameters, and the main models used both to interpret experimental data and to suggest new research directions are described.

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Ion acceleration by superintense laser-plasma interaction

For many years, laser-driven ion acceleration, mainly proton acceleration, has been proposed and a number of proof-of-principle experiments have been carried out with lasers whose pulse duration was in the nanosecond range. In the 1990s, ion acceleration in a relativistic plasma was demonstrated with ultra-short pulse lasers based on the chirped pulse amplification technique which can provide not only picosecond or femtosecond laser pulse duration, but simultaneously ultra-high peak power of terawatt to petawatt levels. Starting from the year 2000, several groups demonstrated low transverse emittance, tens of MeV proton beams with a conversion efficiency of up to several percent. The laser-accelerated particle beams have a duration of the order of a few picoseconds at the source, an ultra-high peak current and a broad energy spectrum, which make them suitable for many, including several unique, applications. This paper reviews, firstly, the historical background including the early laser-matter interaction studies on energetic ion acceleration relevant to inertial confinement fusion. Secondly, we describe several implemented and proposed mechanisms of proton and/or ion acceleration driven by ultra-short high-intensity lasers. We pay special attention to relatively simple models of several acceleration regimes. The models connect the laser, plasma and proton/ion beam parameters, predicting important features, such as energy spectral shape, optimum conditions and scalings under these conditions for maximum ion energy, conversion efficiency, etc. The models also suggest possible ways to manipulate the proton/ion beams by tailoring the target and irradiation conditions. Thirdly, we review experimental results on proton/ion acceleration, starting with the description of driving lasers. We list experimental results and show general trends of parameter dependences and compare them with the theoretical predictions and simulations. The fourth topic includes a review of scientific, industrial and medical applications of laser-driven proton or ion sources, some of which have already been established, while the others are yet to be demonstrated. In most applications, the laser-driven ion sources are complementary to the conventional accelerators, exhibiting significantly different properties. Finally, we summarize the paper.

https://iopscience.iop.org/article/10.1088/0034-4885/75/5/056401/pdf

Review of laser-driven ion sources and their applications.

The past few years have seen remarkable progress in the development of laser-based particle accelerators. The ability to produce ultrabright beams of multi-megaelectronvolt protons routinely has many potential uses from engineering to medicine, but for this potential to be realized substantial improvements in the performances of these devices must be made. Here we show that in the laser-driven accelerator that has been demonstrated experimentally to produce the highest energy protons, scaling laws derived from fluid models and supported by numerical simulations can be used to accurately describe the acceleration of proton beams for a large range of laser and target parameters. This enables us to evaluate the laser parameters needed to produce high-energy and high-quality proton beams of interest for radiography of dense objects or proton therapy of deep-seated tumours.

/pdf/laser-driven-proton-scaling-laws-and-new-paths-towards-3j3b6i3ziz.pdf

Laser-driven proton scaling laws and new paths towards energy increase

Relativistic interaction of short-pulse lasers with underdense plasmas has recently led to the emergence of a novel generation of femtosecond x-ray sources. Based on radiation from electrons accelerated in plasma, these sources have the common properties to be compact and to deliver collimated, incoherent, and femtosecond radiation. In this article, within a unified formalism, the betatron radiation of trapped and accelerated electrons in the so-called bubble regime, the synchrotron radiation of laser-accelerated electrons in usual meter-scale undulators, the nonlinear Thomson scattering from relativistic electrons oscillating in an intense laser field, and the Thomson backscattered radiation of a laser beam by laser-accelerated electrons are reviewed. The underlying physics is presented using ideal models, the relevant parameters are defined, and analytical expressions providing the features of the sources are given. Numerical simulations and a summary of recent experimental results on the different mechanisms are also presented. Each section ends with the foreseen development of each scheme. Finally, one of the most promising applications of laser-plasma accelerators is discussed: the realization of a compact free-electron laser in the x-ray range of the spectrum. In the conclusion, the relevant parameters characterizing each sources are summarized. Considering typical laser-plasma interaction parameters obtained with currently available lasers, examples of the source features are given. The sources are then compared to each other in order to define their field of applications.

https://hal.archives-ouvertes.fr/hal-01164031/document

Femtosecond x rays from laser-plasma accelerators

Specular reflection is one of the most fundamental processes of optics. At moderate light intensities generated by conventional light sources this process is well understood. But at those capable of being produced by modern ultrahigh-intensity lasers, many new and potentially useful phenomena arise. When a pulse from such a laser hits an optically polished surface, it generates a dense plasma that itself acts as a mirror, known as a plasma mirror (PM). PMs do not just reflect the remainder of the incident beam, but can act as active optical elements. Using a set of three consecutive PMs in different regimes, we significantly improve the temporal contrast of femtosecond pulses, and demonstrate that high-order harmonics of the laser frequency can be generated through two distinct mechanisms. A better understanding of these processes should aid the development of laser-driven attosecond sources for use in fields from materials science to molecular biology.

Plasma mirrors for ultrahigh-intensity optics

We present a new mechanism for high-order harmonic generation by reflection of a laser beam from an overdense plasma, efficient even at moderate laser intensities (down to $I{\ensuremath{\lambda}}^{2}\ensuremath{\approx}4\ifmmode\times\else\texttimes\fi{}{10}^{15}\text{ }\text{ }\mathrm{W}\text{ }{\mathrm{cm}}^{\ensuremath{-}2}\text{ }\ensuremath{\mu}{\mathrm{m}}^{2}$). In this mechanism, a transient phase matching between the electromagnetic field and plasma oscillations within a density gradient leads to the emission of harmonics up to the plasma frequency. These plasma oscillations are periodically excited in the wake of attosecond electron bunches which sweep across the density gradient. This process leads to a train of unevenly spaced chirped attosecond pulses and, hence, to broadened and chirped harmonics. This last effect is confirmed experimentally.

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Coherent wake emission of high-order harmonics from overdense plasmas.

We report on simultaneous measurements of backward- and forward-accelerated protons spectra when an ultrahigh intensity ($\ensuremath{\sim}5\ifmmode\times\else\texttimes\fi{}{10}^{18}\text{ }\text{ }\mathrm{W}/{\mathrm{cm}}^{2}$), ultrahigh contrast ($g{10}^{10}$) laser pulse interacts with foils of thickness ranging from 0.08 to $105\text{ }\text{ }\ensuremath{\mu}\mathrm{m}$. Under such conditions, free of preplasma originating from ionization of the laser-irradiated surface, we show that the maximum proton energies are proportional to the $p$ component of the laser electric field only and not to the ponderomotive force and that the characteristics of the proton beams originating from both target sides are almost identical. All these points have been corroborated by extensive 1D and 2D particle-in-cell simulations showing a very good agreement with the experimental data.

Proton acceleration with high-intensity ultrahigh-contrast laser pulses.

We present and characterize a very efficient optical device that employs the plasma mirror technique to increase the contrast of high-power laser systems. Contrast improvements higher than 104 with 50% transmission are shown to be routinely achieved on a typical 10 TW laser system when the pulse is reflected on two consecutive plasma mirrors. Used at the end of the laser system, this double plasma mirror preserves the spatial profile of the initial beam, is unaffected by shot-to-shot fluctuations, and is suitable for most high peak power laser systems. We use the generation of high-order harmonics as an effective test for the contrast improvement produced by the double plasma mirrors.

Double plasma mirror for ultrahigh temporal contrast ultraintense laser pulses

As a high-intensity laser-pulse reflects on a plasma mirror, high-order harmonics of the incident frequency can be generated in the reflected beam. We present a numerical study of the phase properties of these individual harmonics, and demonstrate experimentally that they can be coherently controlled through the phase of the driving laser field. The harmonic intrinsic phase, resulting from the generation process, is directly related to the coherent sub-laser-cycle dynamics of plasma electrons, and thus constitutes a new experimental probe of these dynamics.

/pdf/phase-properties-of-laser-high-order-harmonics-generated-on-55r4bqll4x.pdf

P. Monot

Papers

Plasma mirrors for ultrahigh-intensity optics

Coherent wake emission of high-order harmonics from overdense plasmas.

Proton acceleration with high-intensity ultrahigh-contrast laser pulses.

Double plasma mirror for ultrahigh temporal contrast ultraintense laser pulses

Phase Properties of Laser High-Order Harmonics Generated on Plasma Mirrors