https://horizon.documentation.ird.fr/exl-doc/pleins_textes/pleins_textes_7/b_fdi_51-52/010019285.pdf

AERONET-a federated instrument network and data archive for aerosol Characterization

Changes in Atmospheric Constituents and in Radiative Forcing

Black carbon aerosol plays a unique and important role in Earth's climate system. Black carbon is a type of carbonaceous material with a unique combination of physical properties. This assessment provides an evaluation of black-carbon climate forcing that is comprehensive in its inclusion of all known and relevant processes and that is quantitative in providing best estimates and uncertainties of the main forcing terms: direct solar absorption; influence on liquid, mixed phase, and ice clouds; and deposition on snow and ice. These effects are calculated with climate models, but when possible, they are evaluated with both microphysical measurements and field observations. Predominant sources are combustion related, namely, fossil fuels for transportation, solid fuels for industrial and residential uses, and open burning of biomass. Total global emissions of black carbon using bottom-up inventory methods are 7500 Gg yr−1 in the year 2000 with an uncertainty range of 2000 to 29000. However, global atmospheric absorption attributable to black carbon is too low in many models and should be increased by a factor of almost 3. After this scaling, the best estimate for the industrial-era (1750 to 2005) direct radiative forcing of atmospheric black carbon is +0.71 W m−2 with 90% uncertainty bounds of (+0.08, +1.27) W m−2. Total direct forcing by all black carbon sources, without subtracting the preindustrial background, is estimated as +0.88 (+0.17, +1.48) W m−2. Direct radiative forcing alone does not capture important rapid adjustment mechanisms. A framework is described and used for quantifying climate forcings, including rapid adjustments. The best estimate of industrial-era climate forcing of black carbon through all forcing mechanisms, including clouds and cryosphere forcing, is +1.1 W m−2 with 90% uncertainty bounds of +0.17 to +2.1 W m−2. Thus, there is a very high probability that black carbon emissions, independent of co-emitted species, have a positive forcing and warm the climate. We estimate that black carbon, with a total climate forcing of +1.1 W m−2, is the second most important human emission in terms of its climate forcing in the present-day atmosphere; only carbon dioxide is estimated to have a greater forcing. Sources that emit black carbon also emit other short-lived species that may either cool or warm climate. Climate forcings from co-emitted species are estimated and used in the framework described herein. When the principal effects of short-lived co-emissions, including cooling agents such as sulfur dioxide, are included in net forcing, energy-related sources (fossil fuel and biofuel) have an industrial-era climate forcing of +0.22 (−0.50 to +1.08) W m−2 during the first year after emission. For a few of these sources, such as diesel engines and possibly residential biofuels, warming is strong enough that eliminating all short-lived emissions from these sources would reduce net climate forcing (i.e., produce cooling). When open burning emissions, which emit high levels of organic matter, are included in the total, the best estimate of net industrial-era climate forcing by all short-lived species from black-carbon-rich sources becomes slightly negative (−0.06 W m−2 with 90% uncertainty bounds of −1.45 to +1.29 W m−2). The uncertainties in net climate forcing from black-carbon-rich sources are substantial, largely due to lack of knowledge about cloud interactions with both black carbon and co-emitted organic carbon. In prioritizing potential black-carbon mitigation actions, non-science factors, such as technical feasibility, costs, policy design, and implementation feasibility play important roles. The major sources of black carbon are presently in different stages with regard to the feasibility for near-term mitigation. This assessment, by evaluating the large number and complexity of the associated physical and radiative processes in black-carbon climate forcing, sets a baseline from which to improve future climate forcing estimates.

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Bounding the role of black carbon in the climate system: A scientific assessment

The Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2), is the latest atmospheric reanalysis of the modern satellite era produced by NASA’s Global Modeling and Assimilation Office (GMAO). MERRA-2 assimilates observation types not available to its predecessor, MERRA, and includes updates to the Goddard Earth Observing System (GEOS) model and analysis scheme so as to provide a viable ongoing climate analysis beyond MERRA’s terminus. While addressing known limitations of MERRA, MERRA-2 is also intended to be a development milestone for a future integrated Earth system analysis (IESA) currently under development at GMAO. This paper provides an overview of the MERRA-2 system and various performance metrics. Among the advances in MERRA-2 relevant to IESA are the assimilation of aerosol observations, several improvements to the representation of the stratosphere including ozone, and improved representations of cryospheric processes. Other improvements in the quality of M...

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The Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2)

The NCEP Climate Forecast System Reanalysis (CFSR) was completed for the 31-yr period from 1979 to 2009, in January 2010. The CFSR was designed and executed as a global, high-resolution coupled atmosphere–ocean–land surface–sea ice system to provide the best estimate of the state of these coupled domains over this period. The current CFSR will be extended as an operational, real-time product into the future. New features of the CFSR include 1) coupling of the atmosphere and ocean during the generation of the 6-h guess field, 2) an interactive sea ice model, and 3) assimilation of satellite radiances by the Gridpoint Statistical Interpolation (GSI) scheme over the entire period. The CFSR global atmosphere resolution is ~38 km (T382) with 64 levels extending from the surface to 0.26 hPa. The global ocean's latitudinal spacing is 0.25° at the equator, extending to a global 0.5° beyond the tropics, with 40 levels to a depth of 4737 m. The global land surface model has four soil levels and the global sea ice m...

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The NCEP Climate Forecast System Reanalysis

. We developed a new emission inventory for Asia (Regional Emission inventory in ASia (REAS) Version 1.1) for the period 1980–2020. REAS is the first inventory to integrate historical, present, and future emissions in Asia on the basis of a consistent methodology. We present here emissions in 2000, historical emissions for 1980–2003, and projected emissions for 2010 and 2020 of SO2, NOx, CO, NMVOC, black carbon (BC), and organic carbon (OC) from fuel combustion and industrial sources. Total energy consumption in Asia more than doubled between 1980 and 2003, causing a rapid growth in Asian emissions, by 28% for BC, 30% for OC, 64% for CO, 108% for NMVOC, 119% for SO2, and 176% for NOx. In particular, Chinese NOx emissions showed a marked increase of 280% over 1980 levels, and growth in emissions since 2000 has been extremely high. These increases in China were mainly caused by increases in coal combustion in the power plants and industrial sectors. NMVOC emissions also rapidly increased because of growth in the use of automobiles, solvents, and paints. By contrast, BC, OC, and CO emissions in China showed decreasing trends from 1996 to 2000 because of a reduction in the use of biofuels and coal in the domestic and industry sectors. However, since 2000, Chinese emissions of these species have begun to increase. Thus, the emissions of air pollutants in Asian countries (especially China) showed large temporal variations from 1980–2003. Future emissions in 2010 and 2020 in Asian countries were projected by emission scenarios and from emissions in 2000. For China, we developed three emission scenarios: PSC (policy success case), REF (reference case), and PFC (policy failure case). In the 2020 REF scenario, Asian total emissions of SO2, NOx, and NMVOC were projected to increase substantially by 22%, 44%, and 99%, respectively, over 2000 levels. The 2020 REF scenario showed a modest increase in CO (12%), a lesser increase in BC (1%), and a slight decrease in OC (−5%) compared with 2000 levels. However, it should be noted that Asian total emissions are strongly influenced by the emission scenarios for China.

/pdf/an-asian-emission-inventory-of-anthropogenic-emission-9m6zqerave.pdf

An Asian emission inventory of anthropogenic emission sources for the period 1980-2020

A new gauge-based analysis of daily precipitation has been constructed on a 0.5° latitude–longitude grid over East Asia (5°–60°N, 65°–155°E) for a 26-yr period from 1978 to 2003 using gauge observations at over 2200 stations collected from several individual sources. First, analyzed fields of daily climatology are computed by interpolating station climatology defined as the summation of the first six harmonics of the 365-calendar-day time series of the mean daily values averaged over a 20-yr period from 1978 to 1997. These fields of daily climatology are then adjusted by the Parameter-Elevation Regressions on Independent Slopes Model (PRISM) monthly precipitation climatology to correct the bias caused by orographic effects. Gridded fields of the ratio of daily precipitation to the daily climatology are created by interpolating the corresponding station values using the optimal interpolation method. Analyses of total daily precipitation are finally calculated by multiplying the daily climatology b...

A Gauge-Based Analysis of Daily Precipitation over East Asia

Aerosol trends over China, 1980-2000

Tropospheric aerosols have been observed for the period from November 1990 to April 1992 with a lidar, a sun photometer, and an optical particle counter. Variations of aerosol optical thickness derived from the lidar and the sun photometer data and measurements are presented. The simultaneous measurements of these instruments also allowed us to estimate the extinction-to-backscatter ratio (S(1)), which ranged from 20 to 70. Comparison of optical thicknesses derived from both instruments clearly shows the effect of Mt. Pinatubo's eruption and the temporal variation of optical thickness in the stratosphere over 12 km. The possible range of the complex refractive index for the columnar mean aerosols can be deduced from the probable range of S(1) derived by the use of an S(1) diagram as a function of complex refractive index (m). The imaginary part of m can be estimated provided that the real part of m is known.

Tropospheric aerosol optical properties derived from lidar, sun photometer, and optical particle counter measurements

Cloud remote sensing techniques are conventionally based on the independent pixel approximation (IPA). Here, three-dimensional (3D) radiative effects on IPA-based retrieved optical thickness from a visible-wavelength moderate-resolution (about 1 km) sensor are investigated. A Monte Carlo 3D radiative transfer model and a lognormal spectral cloud model are used to simulate monochromatic radiance reflected from overcast boundary layer cloud. A characterization of statistical properties of the optical thickness by the mean (M) and variance (S2) of the logarithm of the optical thickness is proposed, where S represents a degree of cloud inhomogeneity. Biases in retrieved values of the two parameters with the IPA are defined as ΔM and ΔS2 and attributed to neglect of net horizontal radiative transport in the IPA. Sensitivities of ΔM and ΔS2 are tested with respect to geometrical roughness, M, S, mean geometrical thickness, spectral exponent of optical thickness fluctuation, ground surface reflectance, ...

Tadahiro Hayasaka

Papers

An Asian emission inventory of anthropogenic emission sources for the period 1980-2020

A Gauge-Based Analysis of Daily Precipitation over East Asia

Aerosol trends over China, 1980-2000

Tropospheric aerosol optical properties derived from lidar, sun photometer, and optical particle counter measurements

Effects of Cloud Horizontal Inhomogeneity on the Optical Thickness Retrieved from Moderate-Resolution Satellite Data