Fine-particle pollution associated with winter haze threatens the health of more than 400 million people in the North China Plain. Sulfate is a major component of fine haze particles. Record sulfate concentrations of up to ~300 μg m −3 were observed during the January 2013 winter haze event in Beijing. State-of-the-art air quality models that rely on sulfate production mechanisms requiring photochemical oxidants cannot predict these high levels because of the weak photochemistry activity during haze events. We find that the missing source of sulfate and particulate matter can be explained by reactive nitrogen chemistry in aerosol water. The aerosol water serves as a reactor, where the alkaline aerosol components trap SO 2 , which is oxidized by NO 2 to form sulfate, whereby high reaction rates are sustained by the high neutralizing capacity of the atmosphere in northern China. This mechanism is self-amplifying because higher aerosol mass concentration corresponds to higher aerosol water content, leading to faster sulfate production and more severe haze pollution.

Reactive nitrogen chemistry in aerosol water as a source of sulfate during haze events in China

Formation, features and controlling strategies of severe haze-fog pollutions in China

Thick haze plagued northeastern China in January 2013, strongly affecting both regional climate and human respiratory health. Here, we present dual carbon isotope constrained (Δ14C and δ13C) source apportionment for combustion-derived black carbon aerosol (BC) for three key hotspot regions (megacities): North China Plain (NCP, Beijing), the Yangtze River Delta (YRD, Shanghai), and the Pearl River Delta (PRD, Guangzhou) for January 2013. BC, here quantified as elemental carbon (EC), is one of the most health-detrimental components of PM2.5 and a strong climate warming agent. The results show that these severe haze events were equally affected (∼30%) by biomass combustion in all three regions, whereas the sources of the dominant fossil fuel component was dramatically different between north and south. In the NCP region, coal combustion accounted for 66% (46–74%, 95% C.I.) of the EC, whereas, in the YRD and PRD regions, liquid fossil fuel combustion (e.g., traffic) stood for 46% (18–66%) and 58% (38–68%), re...

Regionally-Varying Combustion Sources of the January 2013 Severe Haze Events over Eastern China

Long-range transport and regional sources of PM2.5 in Beijing based on long-term observations from 2005 to 2010

Formation process of the widespread extreme haze pollution over northern China in January 2013: Implications for regional air quality and climate

A multisource observation study of the severe prolonged regional haze episode over eastern China in January 2013

A multisource observation study of the severe prolonged regional haze

To track moving targets and signals in space, multiple characteristics as large orientational workspace and excellent kinematic performance are required for the satellite antenna driving mechanism. Due to variable orientational center and axes, the 3-RSR mechanism is capable of 1T2R with continuous workspace and becomes a promising solution for the satellite antenna driving mechanism. Influenced by the topological structure characteristics as none fixed orientation center and axes, the performances of 3-RSR mechanism are significantly impacted by the parameter perturbation. According to the differential mapping between finite screw and instantaneous screw, the structure, kinematics, performance, and optimization are unified under the FIS theory. To be applied for the satellite antenna driving mechanism, this paper carries out the multi-objective optimization of 3-RSR mechanism under the influence of parameter perturbation based on the FIS theory. Firstly, the orientational workspace is obtained by finite screw and the instantaneous motion description of the mechanism is derived through calculation principle of FIS theory. Secondly, the orientational workspace and kinematics indices of the mechanism are proposed towards the actual requirements of the satellite antenna driving, and the relationship with the parameters is established. The discrete operation becomes extremely complex owing to parameter perturbation, and the RSMs (response surface model) of indices without considering and considering parameter perturbation are modeled. The multi-objectives optimization of 3-RSR mechanism influenced by parameter perturbation is carried out and its Pareto frontier is obtained. Finally, a point preferred strategy is proposed and the optimum value of the parameter from Pareto frontier is selected.

Yu Wang

Papers

A multisource observation study of the severe prolonged regional haze episode over eastern China in January 2013

A multisource observation study of the severe prolonged regional haze

Multi-Objective Optimization of 1T2R Parallel Mechanisms Without Fixed Orientation Center and Axis Under the Influence of Parameter Perturbation