2D layered materials (2DLMs) are a subject of intense research for a wide variety of applications (e.g., electronics, photonics, and optoelectronics) due to their unique physical properties. Most recently, increasing research efforts on 2DLMs are projected toward the nonlinear optical properties of 2DLMs, which are not only fascinating from the fundamental science point of view but also intriguing for various potential applications. Here, the current state of the art in the field of nonlinear optics based on 2DLMs and their hybrid structures (e.g., mixed-dimensional heterostructures, plasmonic structures, and silicon/fiber integrated structures) is reviewed. Several potential perspectives and possible future research directions of these promising nanomaterials for nonlinear optics are also presented.

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Nonlinear Optics with 2D Layered Materials.

2D Layered Materials: Synthesis, Nonlinear Optical Properties, and Device Applications

Broadband Nonlinear Photoresponse of 2D TiS2 for Ultrashort Pulse Generation and All-Optical Thresholding Devices

Solitons are stable localized wave packets that can propagate long distance in dispersive media without changing their shapes. As particle-like nonlinear localized waves, solitons have been investigated in different physical systems. Owing to potential applications in optical communication and optical signal processing systems, optical solitons have attracted intense interest in the past three decades. To experimentally study the formation and dynamics of temporal optical solitons, fiber lasers are considered as a wonderful nonlinear system. During the last decade, several kinds of theoretically predicted solitons were observed experimentally in fiber lasers. In this review, we present a detailed overview of the experimentally verified optical solitons in fiber lasers, including bright solitons, dark solitons, vector solitons, dissipative solitons, dispersion-managed solitons, polarization domain wall solitons, and so on. An outlook for the development on the solitons in fiber lasers is also provided and discussed.

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Recent progress of study on optical solitons in fiber lasers

Ultrafast fiber lasers have significant applications in ultra-precision manufacturing, medical diagnostics, medical treatment, precision measurement and astronomical detection, owing to their ultra-short pulse width and ultra-high peak-power. Since graphene was first explored as an optical saturable absorber for passively mode-locked lasers in 2009, many other 2D materials beyond graphene, including phosphorene, antimonene, bismuthene, transition metal dichalcogenides (TMDs), topological insulators (TIs), metal–organic frameworks (MOFs) and MXenes, have been successively explored, resulting in rapid development of novel 2D materials-based saturable absorbers. Herein, we review the latest progress of the emerging 2D materials beyond graphene for passively mode-locked fiber laser application. These 2D materials are classified into mono-elemental, dual-elemental and multi-elemental 2D materials. The atomic structure, band structure, nonlinear optical properties, and preparation methods of 2D materials are summarized. Diverse integration strategies for applying 2D materials into fiber laser systems are introduced, and the mode-locking performance of the 2D materials-based fiber lasers working at 1–3 μm are discussed. Finally, the perspectives and challenges facing 2D materials-based mode-locked fiber lasers are highlighted.

Emerging 2D materials beyond graphene for ultrashort pulse generation in fiber lasers.

The pulse energy in the ultrafast soliton fiber laser oscillators is usually limited by the well-known wave-breaking phenomenon owing to the absence of a desirable real saturable absorber (SA) with high power tolerance and large modulation depth. Here, we report a type of microfiber-based MoTe2 SA fabricated by the magnetron-sputtering deposition (MSD) method. High-energy wave-breaking free soliton pulses were generated with pulse duration/pulse energy/average output power of 229 fs/2.14 nJ/57 mW in the 1.5 μm regime and 1.3 ps/13.8 nJ/212 mW in the 2 μm regime, respectively. To our knowledge, the generated soliton pulses at 1.5 μm had the shortest pulse duration and the highest output power among the reported erbium-doped fiber lasers mode locked by transition metal dichalcogenides. Moreover, this was the first demonstration of a MoTe2-based SA in fiber lasers in the 2 μm regime, and the pulse energy/output power are the highest in the reported thulium-doped fiber lasers mode locked by two-dimensional materials. Our results suggest that a microfiber-based MoTe2 SA could be used as an excellent photonic device for ultrafast pulse generation, and the MSD technique opens a promising route to produce a high-performance SA with high power tolerance and large modulation depth, which are beneficial for high-energy wave-breaking free pulse generation.

High energy soliton pulse generation by a magnetron-sputtering-deposition-grown MoTe 2 saturable absorber

Two-dimensional (2D) layered transition metal dichalcogenides (TMDs) have attracted significant interest in various optoelectronic applications due to their excellent nonlinear optical properties. One of the most important applications of TMDs is to be employed as an extraordinary optical modulation material (e.g., the saturable absorber (SA)) in ultrafast photonics. The main challenge arises while embedding TMDs into fiber laser systems to generate ultrafast pulse trains and thus constraints their practical applications. Herein, few-layered WS2 with a large-area was directly transferred on the facet of the pigtail and acted as a SA for erbium-doped fiber laser (EDFL) systems. In our study, WS2 SA exhibited remarkable nonlinear optical properties (e.g., modulation depth of 15.1% and saturable intensity of 157.6 MW cm-2) and was used for ultrafast pulse generation. The soliton pulses with remarkable performances (e.g., ultrashort pulse duration of 1.49 ps, high stability of 71.8 dB, and large pulse average output power of 62.5 mW) could be obtained in a telecommunication band. To the best of our knowledge, the average output power of the mode-locked pulse trains is the highest by employing TMD materials in fiber laser systems. These results indicate that atomically large-area WS2 could be used as excellent optical modulation materials in ultrafast photonics.

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Large-area tungsten disulfide for ultrafast photonics

A passively mode-locked thulium-doped fiber (TDF) laser was realized by employing chemical vapor deposited few-layer molybdenum ditelluride (MoTe2) as a saturable absorber (SA). The few-layer MoTe2 film was transferred onto the waist of a microfiber and then incorporated into a TDF laser with a typical all-fiber ring cavity configuration. Stable soliton pulses emitting at 1930.22 nm were obtained with a 3 dB bandwidth of 4.45 nm, a pulse duration of 952 fs, and an average power of 36.7 mW.

Mode-locked thulium-doped fiber laser with chemical vapor deposited molybdenum ditelluride.

Ultrafast pulse generation was demonstrated in a thulium-doped fiber laser mode-locked by magnetron-sputtering deposited WTe2 with a modulation depth, a nonsaturable loss, and a saturable intensity of 31%, 34.3%, and 7.6  MW/cm2, respectively. Stable soliton pulses could be obtained at a 1915.5 nm central wavelength with a pulse duration of 1.25 ps, an average output power of 39.9 mW, and a signal-to-noise ratio of 95 dB. To the best of our knowledge, this was the first demonstration of WTe2-based saturable absorbers in fiber lasers at a 2 μm regime.

Magnetron-sputtering deposited WTe 2 for an ultrafast thulium-doped fiber laser

In this Letter, high-quality WS2 film and MoS2 film were vertically stacked on the tip of a single-mode fiber in turns to form heterostructure (WS2-MoS2-WS2)-based saturable absorbers with all-fiber integrated features. Their nonlinear saturable absorption properties were remarkable, such as a large modulation depth (∼16.99%) and a small saturable intensity (6.23  MW·cm−2). Stable pulses at 1.55 μm with duration as short as 296 fs and average power as high as 25 mW were obtained in an erbium-doped fiber laser system. The results demonstrate that the proposed heterostructures own remarkable nonlinear optical properties and offer a platform for adjusting nonlinear optical properties by stacking different transition-metal dichalcogenides or modifying the thickness of each layer, paving the way for engineering functional ultrafast photonics devices with desirable properties.

Zike Jiang

Papers

High energy soliton pulse generation by a magnetron-sputtering-deposition-grown MoTe 2 saturable absorber

Large-area tungsten disulfide for ultrafast photonics

Mode-locked thulium-doped fiber laser with chemical vapor deposited molybdenum ditelluride.

Magnetron-sputtering deposited WTe 2 for an ultrafast thulium-doped fiber laser

Transition-metal dichalcogenides heterostructure saturable absorbers for ultrafast photonics.