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Quantitative investigation of the multiphoton intrapulse interference phase scan method for simultaneous phase measurement and compensation of femtosecond laser pulses

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TLDR
In this article, a femtosecond pulse characterization and compensation using multiphoton intrapulse interference phase scan (MIIPS) was rigorously tested and was found to have 3 mrad precision within the 90 nm bandwidth of the pulses.
Abstract
Femtosecond pulse characterization and compensation using multiphoton intrapulse interference phase scan (MIIPS) [Opt. Lett.29, 775 (2004)] was rigorously tested. MIIPS was found to have 3 mrad precision within the 90 nm bandwidth of the pulses. Group-velocity dispersion measurements of glass and quartz provided independent accuracy tests. Phase distortions from high-numerical-aperture objectives were measured and corrected using MIIPS, an important requirement for reproducible two-photon microscopy. Phase compensation greatly improved the pulse-shaping results through a more accurate delivery of continuous and binary phase functions to the sample. MIIPS measurements were possible through the scattering of biological tissue, a consideration for biomedical imaging.

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Citations
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Journal ArticleDOI

Ultrafast optical pulse shaping: A tutorial review

TL;DR: In this paper, a tutorial on the field of femtosecond pulse shaping, a technology that enables generation of nearly arbitrary, user defined, ultrafast optical waveforms, with control of phase, amplitude, and polari-zation, is presented.
Journal ArticleDOI

Characterization of ultrashort electromagnetic pulses

TL;DR: In this paper, a review of advances made in the latter field over this period, indicating the general principles involved, how these have been implemented in various experimental approaches, and how the most popular methods encode the temporal electric field of a short optical pulse in the measured signal and extract the field from the data.
Journal ArticleDOI

Quantum coherent energy transfer over varying pathways in single light-harvesting complexes.

TL;DR: It is found that quantum coherences between electronically coupled energy eigenstates persist at least 400 femtoseconds and that distinct energy-transfer pathways that change with time can be identified in each complex.
Patent

Control system and apparatus for use with ultra-fast laser

TL;DR: In this paper, a control system and apparatus for use with an ultra-fast laser is described, which includes a laser, pulse shaper, detection device and control system, and a multiphoton intrapulse interference method is used to characterize the spectral phase of laser pulses.
Journal ArticleDOI

Simultaneous compression and characterization of ultrashort laser pulses using chirped mirrors and glass wedges

TL;DR: A simple and robust technique to retrieve the phase of ultrashort laser pulses, based on a chirped mirror and glass wedges compressor, which uses the compression system itself as a diagnostic tool, thereby making unnecessary the use of complementary diagnostic tools.
References
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Journal ArticleDOI

Interspecimen Comparison of the Refractive Index of Fused Silica

TL;DR: In this paper, the index of refraction of optical quality fused silica (SiO2) was determined for 60 wavelengths from 0.21 to 3.71 μ at 20°C.
Journal ArticleDOI

Femtosecond pulse shaping using spatial light modulators

TL;DR: In this article, the field of femtosecond pulse shaping is reviewed, and applications of pulse shaping to optical communications, biomedical optical imaging, high power laser amplifiers, quantum control, and laser-electron beam interactions are reviewed.
Journal ArticleDOI

Control of Chemical Reactions by Feedback-Optimized Phase-Shaped Femtosecond Laser Pulses

TL;DR: Tailored femtosecond laser pulses from a computer-controlled pulse shaper were used to optimize the branching ratios of different organometallic photodissociation reaction channels, showing that two different bond-cleaving reactions can be selected, resulting in chemically different products.
Journal ArticleDOI

Measuring ultrashort laser pulses in the time-frequency domain using frequency-resolved optical gating

TL;DR: In this article, the authors summarize the problem of measuring an ultrashort laser pulse and describe in detail a technique that completely characterizes a pulse in time: frequency-resolved optical gating.
Journal ArticleDOI

Spectral phase interferometry for direct electric-field reconstruction of ultrashort optical pulses.

TL;DR: In this paper, a self-referencing interferometric technique for measuring the amplitude and phase of ultrashort optical pulses is presented, which uses a collinear geometry that requires no moving components.
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