https://escholarship.org/content/qt8mf445sh/qt8mf445sh.pdf?t=nu02or

Atmospheric composition change – global and regional air quality

The recent literature on satellite remote sensing of air quality is reviewed. 2009 is the 50th anniversary of the first satellite atmospheric observations. For the first 40 of those years, atmospheric composition measurements, meteorology, and atmospheric structure and dynamics dominated the missions launched. Since 1995, 42 instruments relevant to air quality measurements have been put into orbit. Trace gases such as ozone, nitric oxide, nitrogen dioxide, water, oxygen/tetraoxygen, bromine oxide, sulfur dioxide, formaldehyde, glyoxal, chlorine dioxide, chlorine monoxide, and nitrate radical have been measured in the stratosphere and troposphere in column measurements. Aerosol optical depth (AOD) is a focus of this review and a significant body of literature exists that shows that ground-level fine particulate matter (PM2.5) can be estimated from columnar AOD. Precision of the measurement of AOD is +/-20% and the prediction of PM2.5 from AOD is order +/-30% in the most careful studies. The air quality needs that can use such predictions are examined. Satellite measurements are important to event detection, transport and model prediction, and emission estimation. It is suggested that ground-based measurements, models, and satellite measurements should be viewed as a system, each component of which is necessary to better understand air quality.

https://www.tandfonline.com/doi/pdf/10.3155/1047-3289.59.6.645

Remote sensing of particulate pollution from space: have we reached the promised land?

The collective representation within global models of aerosol, cloud, precipitation, and their radiative properties remains unsatisfactory. They constitute the largest source of uncertainty in predictions of climatic change and hamper the ability of numerical weather prediction models to forecast high-impact weather events. The joint ESA-JAXA EarthCARE satellite mission, scheduled for launch in 2017, will help to resolve these weaknesses by providing global profiles of cloud, aerosol, precipitation, and associated radiative properties inferred from a combination of measurements made by its collocated active and passive sensors. EarthCARE will improve our understanding of cloud and aerosol processes by extending the invaluable dataset acquired by the A-Train satellites CloudSat, CALIPSO, and Aqua. Specifically, EarthCARE's Cloud Profling Radar, with 7 dB more sensitivity than CloudSat, will detect more thin clouds and its Doppler capability will provide novel information on convection, precipitating ice particle and raindrop fall speeds. EarthCARE's 355-nm High Spectral Resolution Lidar will measure directly and accurately cloud and aerosol extinction and optical depth. Combining this with backscatter and polarization information should lead to an unprecedented ability to identify aerosol type. The Multi-Spectral Imager will provide a context for, and the ability to construct the cloud and aerosol distribution in 3D domains around the narrow 2D retrieved cross-section. The consistency of the retrievals will be assessed to within a target of ±10 W m−2 on the (10 km2) scale by comparing the multi-view Broad-Band Radiometer observations to the top-of-atmosphere fluxes estimated by 3D radiative transfer models acting on retrieved 3D domains.

/pdf/the-earthcare-satellite-the-next-step-forward-in-global-4w19jz39pk.pdf

The EarthCARE Satellite: The Next Step Forward in Global Measurements of Clouds, Aerosols, Precipitation, and Radiation

The European Aerosol Research Lidar Network, EARLINET, was founded in 2000 as a research project for establishing a quantitative, comprehensive, and statistically significant database for the horizontal, vertical, and tempo- ral distribution of aerosols on a continental scale. Since then EARLINET has continued to provide the most extensive col- lection of ground-based data for the aerosol vertical distribu- tion over Europe. This paper gives an overview of the network's main de- velopments since 2000 and introduces the dedicated EAR- LINET special issue, which reports on the present innova- tive and comprehensive technical solutions and scientific re- sults related to the use of advanced lidar remote sensing tech- niques for the study of aerosol properties as developed within the network in the last 13 years. Since 2000, EARLINET has developed greatly in terms of number of stations and spatial distribution: from 17 sta- tions in 10 countries in 2000 to 27 stations in 16 countries in 2013. EARLINET has developed greatly also in terms of technological advances with the spread of advanced multi- wavelength Raman lidar stations in Europe. The develop- ments for the quality assurance strategy, the optimization of instruments and data processing, and the dissemination of data have contributed to a significant improvement of the net- work towards a more sustainable observing system, with an increase in the observing capability and a reduction of oper- ational costs. Consequently, EARLINET data have already been ex- tensively used for many climatological studies, long-range transport events, Saharan dust outbreaks, plumes from vol- canic eruptions, and for model evaluation and satellite data validation and integration. Future plans are aimed at continuous measurements and near-real-time data delivery in close cooperation with other ground-based networks, such as in the ACTRIS (Aerosols, Clouds, and Trace gases Research InfraStructure Network) www.actris.net, and with the modeling and satellite commu- nity, linking the research community with the operational world, with the aim of establishing of the atmospheric part of the European component of the integrated global observ- ing system.

https://www.dwd.de/DWD/forschung/projekte/ceilomap/files/amt-7-2389-2014.pdf

EARLINET: towards an advanced sustainable European aerosol lidar network

Stable carbon and oxygen isotopes (δ18O and δ13C values) and trace elements have been applied to the study of diagenesis of carbonate rocks for over 50 years. As valuable as these insights have been, many problems regarding the interpretation of geochemical signals within mature rocks remain. For example, while the δ18O values of carbonate rocks are dependent both upon the temperature and the δ18O value of the fluid, and additional information including trace element composition aids in interpreting such signals, direct evidence of either the temperature or the composition of the fluids is required. Such information can be obtained by analysing the δ18O value of any fluid inclusions or by measuring the temperature using a method such as the ‘clumped’ isotope technique. Such data speak directly to a large number of problems in interpreting the oxygen isotope record including the well-known tendency for δ18O values of carbonate rocks to decrease with increasing age. Unlike the δ18O, δ13C values of carbonates are considered to be less influenced by diagenesis and more a reflection of primary changes in the global carbon cycle through time. However, many studies have not sufficiently emphasized the effects of diagenesis and other post-depositional influences on the eventual carbon isotopic composition of the rock with the classic paradigm that the present is the key to the past being frequently ignored. Finally, many additional proxies are poised to contribute to the interpretation of carbonate diagenesis. Although the study of carbonate diagenesis is at an exciting point with an explosion of new proxies and methods, care should be taken to understand both old and new proxies before applying them to the ancient record.

https://onlinelibrary.wiley.com/doi/pdf/10.1111/sed.12205

The geochemistry of carbonate diagenesis: The past, present and future

The almost six-years long database of aerosol and cloud vertical profiles provided by CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) is at the present the longest database of aerosol optical properties at global scale. This database is a unique tool for the characterization of aerosol 4D distribution at global scale. However, CALIPSO has a small footprint and a revisiting time of 16 days, and therefore how well these measurements represent the atmospheric conditions of a surrounding area over a longer time is a big issue to be investigated. Because of its geographic coverage and the large number of advanced Raman aerosol lidars, EARLINET, the European Aerosol Research Lidar Network, offers a unique opportunity for the validation and full exploitation of the CALIPSO mission. CALIPSO Level 2 and Level 3 data products are investigated in terms of their representativeness by comparison with EARLINET measurements. Comparisons for the Level 2 profiles available in both version 2 (40 km as horizontal resolution) and version 3 (5 km) releases highlight the issue of finding a best compromise between the high resolution and the high signal-to-noise ratio. Representativeness of monthly averages provided in Level 3 data is investigated using EARLINET-CALIPSO correlative measurements. The study will furthermore benefit from the availability of the 12-years long-term database of EARLINET climatological data available from May 2000.

Aleksander Pietruczuk

Papers

Investigation of representativeness of CALIPSO aerosol optical properties products by EARLINET correlative measurements