(b) Write out the equations for the time dependence of ρ11, ρ22, ρ12 and ρ21 assuming that a light field interaction V = -μ12Ee iωt + c.c. couples only levels |1> and |2>, and that the excited levels exhibit spontaneous decay. (8 marks) (c) Under steady-state conditions, find the ratio of populations in states |2> and |3>. (3 marks) (d) Find the slowly varying amplitude ̃ ρ 12 of the polarization ρ12 = ̃ ρ 12e iωt . (6 marks) (e) In the limiting case that no decay is possible from intermediate level |3>, what is the ground state population ρ11(∞)? (2 marks) 2. (15 marks total) In a 2-level atom system subjected to a strong field, dressed states are created in the form |D1(n)> = sin θ |1,n> + cos θ |2,n-1> |D2(n)> = cos θ |1,n> sin θ |2,n-1>

The Quantum Theory of Light

In recent years, notions drawn from non-Hermitian physics and parity–time (PT) symmetry have attracted considerable attention. In particular, the realization that the interplay between gain and loss can lead to entirely new and unexpected features has initiated an intense research effort to explore non-Hermitian systems both theoretically and experimentally. Here we review recent progress in this emerging field, and provide an outlook to future directions and developments. This Review Article outlines the exploration of the interplay between parity–time symmetry and non-Hermitian physics in optics, plasmonics and optomechanics.

Non-Hermitian physics and PT symmetry

Sensors play an important part in many aspects of daily life such as infrared sensors in home security systems, particle sensors for environmental monitoring and motion sensors in mobile phones. High-quality optical microcavities are prime candidates for sensing applications because of their ability to enhance light-matter interactions in a very confined volume. Examples of such devices include mechanical transducers, magnetometers, single-particle absorption spectrometers, and microcavity sensors for sizing single particles and detecting nanometre-scale objects such as single nanoparticles and atomic ions. Traditionally, a very small perturbation near an optical microcavity introduces either a change in the linewidth or a frequency shift or splitting of a resonance that is proportional to the strength of the perturbation. Here we demonstrate an alternative sensing scheme, by which the sensitivity of microcavities can be enhanced when operated at non-Hermitian spectral degeneracies known as exceptional points. In our experiments, we use two nanoscale scatterers to tune a whispering-gallery-mode micro-toroid cavity, in which light propagates along a concave surface by continuous total internal reflection, in a precise and controlled manner to exceptional points. A target nanoscale object that subsequently enters the evanescent field of the cavity perturbs the system from its exceptional point, leading to frequency splitting. Owing to the complex-square-root topology near an exceptional point, this frequency splitting scales as the square root of the perturbation strength and is therefore larger (for sufficiently small perturbations) than the splitting observed in traditional non-exceptional-point sensing schemes. Our demonstration of exceptional-point-enhanced sensitivity paves the way for sensors with unprecedented sensitivity.

Exceptional points enhance sensing in an optical microcavity

BACKGROUND Singularities are critical points for which the behavior of a mathematical model governing a physical system is of a fundamentally different nature compared to the neighboring points. Exceptional points are spectral singularities in the parameter space of a system in which two or more eigenvalues, and their corresponding eigenvectors, simultaneously coalesce. Such degeneracies are peculiar features of nonconservative systems that exchange energy with their surrounding environment. In the past two decades, there has been a growing interest in investigating such nonconservative systems, particularly in connection with the quantum mechanics notions of parity-time symmetry, after the realization that some non-Hermitian Hamiltonians exhibit entirely real spectra. Lately, non-Hermitian systems have raised considerable attention in photonics, given that optical gain and loss can be integrated as nonconservative ingredients to create artificial materials and structures with altogether new optical properties. ADVANCES As we introduce gain and loss in a nanophotonic system, the emergence of exceptional point singularities dramatically alters the overall response, leading to a range of exotic functionalities associated with abrupt phase transitions in the eigenvalue spectrum. Even though such a peculiar effect has been known theoretically for several years, its controllable realization has not been made possible until recently and with advances in exploiting gain and loss in guided-wave photonic systems. As shown in a range of recent theoretical and experimental works, this property creates opportunities for ultrasensitive measurements and for manipulating the modal content of multimode lasers. In addition, adiabatic parametric evolution around exceptional points provides interesting schemes for topological energy transfer and designing mode and polarization converters in photonics. Lately, non-Hermitian degeneracies have also been exploited for the design of laser systems, new nonlinear optics phenomena, and exotic scattering features in open systems. OUTLOOK Thus far, non-Hermitian systems have been largely disregarded owing to the dominance of the Hermitian theories in most areas of physics. Recent advances in the theory of non-Hermitian systems in connection with exceptional point singularities has revolutionized our understanding of such complex systems. In the context of optics and photonics, in particular, this topic is highly important because of the ubiquity of nonconservative elements of gain and loss. In this regard, the theoretical developments in the field of non-Hermitian physics have allowed us to revisit some of the well-established platforms with a new angle of utilizing gain and loss as new degrees of freedom, in stark contrast with the traditional approach of avoiding these elements. On the experimental front, progress in fabrication technologies has allowed for harnessing gain and loss in chip-scale photonic systems. These theoretical and experimental developments have put forward new schemes for controlling the functionality of micro- and nanophotonic devices. This is mainly based on the anomalous parameter dependence in the response of non-Hermitian systems when operating around exceptional point singularities. Such effects can have important ramifications in controlling light in new nanophotonic device designs, which are fundamentally based on engineering the interplay of coupling and dissipation and amplification mechanisms in multimode systems. Potential applications of such designs reside in coupled-cavity laser sources with better coherence properties, coupled nonlinear resonators with engineered dispersion, compact polarization and spatial mode converters, and highly efficient reconfigurable diffraction surfaces. In addition, the notion of the exceptional point provides opportunities to take advantage of the inevitable dissipation in environments such as plasmonic and semiconductor materials, which play a key role in optoelectronics. Finally, emerging platforms such as optomechanical cavities provide opportunities to investigate exceptional points and their associated phenomena in multiphysics systems.

Exceptional points in optics and photonics.

Squeezed states of the electromagnetic field have been generated by nondegenerate four-wave mixing due to Na atoms in an optical cavity. The optical noise in the cavity, comprised of primarily vacuum fluctuations and a small component of spontaneous emission from the pumped Na atoms, is amplified in one quadrature of the optical field and deamplified in the other quadrature. These quadrature components are measured with a balanced homodyne detector. The total noise level in the deamplified quadrature drops below the vacuum noise level.

Observation of squeezed states generated by four-wave mixing in an optical cavity

We present spectroscopic observation of an exceptional point or the transition point between mode crossing and avoided mode crossing of neighboring quasieigenmodes in a chaotic optical microcavity of a large size parameter. The transition to the avoided mode crossing was impeded until the degree of deformation exceeded a threshold deformation owing to the system's openness also enhanced by the shape deformation. As a result, a singular topology was observed around the exceptional point on the eigenfrequency surfaces, resulting in fundamental inconsistency in mode labeling.

Observation of an exceptional point in a chaotic optical microcavity.

We report observation of lasing in the scarred modes in an asymmetrically deformed microcavity made of liquid jet. The observed scarred modes correspond to morphology-dependent resonance of radial mode order 3 with their $Q$ values in the range of ${10}^{6}$. Emission directionality is also observed, corresponding to a hexagonal unstable periodic orbit.

Observation of scarred modes in asymmetrically deformed microcylinder lasers.

We investigate the dynamics of a novel multiwavelength generator in which cascaded-stimulated Brillouin scattering and Rayleigh scattering are automatically balanced to given an evenly spaced (9.4-GHz), highly flattened (<3-dB) optical frequency comb over a 57.2-nm span. The extended effective length for the relevant nonlinear processes from the distributed Raman gain and the reduced Brillouin threshold from the seeding effect of Rayleigh backscattered waves are considered to be the key factors that explain the operation of this structure.

Dynamics of cascaded Brillouin-Rayleigh scattering in a distributed fiber Raman amplifier.

This work was supported by a National Research Laboratory grant and by KRF Grant No. 2005-070-C00058. J.B.S. and H.W.L. were supported by a grant from KRISS. S.W.K. was supported by KRF Grant No. 2006–005–J02804 and by KOSEF Grant No. R01-2005-000-10678-0.

Universal output directionality of single modes in a deformed microcavity

Epitaxial LiNbO3 films with two orientations were grown on sapphire (1120) substrates using pulsed laser deposition. The film deposited at a low oxygen pressure (i.e., 10−4 Torr) was epitaxially grown along the a axis, and that at a oxygen pressure of 10−1 Torr was epitaxially grown along the c axis. Electro‐optic properties of these films were quite different, demonstrating importance of controlling the epitaxial growth behaviors. The birefringence measurements of the LiNbO3 (1120) film showed a quadratic electro‐optic behavior with an effective quadratic coefficient of 2.38×10−15 m2/V2. This behavior was analyzed in terms of the quadratic electro‐optic tensor for LiNbO3.

Jai-Hyung Lee

Papers

Observation of an exceptional point in a chaotic optical microcavity.

Observation of scarred modes in asymmetrically deformed microcylinder lasers.

Dynamics of cascaded Brillouin-Rayleigh scattering in a distributed fiber Raman amplifier.

Universal output directionality of single modes in a deformed microcavity

Control of epitaxial growth of pulsed laser deposited LiNbO3 films and their electro‐optic effects