Fundamentals of Plasmonics.- Electromagnetics of Metals.- Surface Plasmon Polaritons at Metal / Insulator Interfaces.- Excitation of Surface Plasmon Polaritons at Planar Interfaces.- Imaging Surface Plasmon Polariton Propagation.- Localized Surface Plasmons.- Electromagnetic Surface Modes at Low Frequencies.- Applications.- Plasmon Waveguides.- Transmission of Radiation Through Apertures and Films.- Enhancement of Emissive Processes and Nonlinearities.- Spectroscopy and Sensing.- Metamaterials and Imaging with Surface Plasmon Polaritons.- Concluding Remarks.

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Plasmonics: Fundamentals and Applications

Over the past three decades a new spectroscopic technique with unique possibilities has emerged. Based on coherent and time-resolved detection of the electric field of ultrashort radiation bursts in the far-infrared, this technique has become known as terahertz time-domain spectroscopy (THz-TDS). In this review article the authors describe the technique in its various implementations for static and time-resolved spectroscopy, and illustrate the performance of the technique with recent examples from solid-state physics and physical chemistry as well as aqueous chemistry. Examples from other fields of research, where THz spectroscopic techniques have proven to be useful research tools, and the potential for industrial applications of THz spectroscopic and imaging techniques are discussed.

Terahertz spectroscopy and imaging – Modern techniques and applications

Adsorption of organic molecules on silica surface.

Metamaterials are artificial materials with subwavelength structure1 that enable the translation of magnetic2 and electric responses3 into spectral regions not accessible through naturally occurring materials. Here, we report direct measurements of the propagation and confinement of terahertz electromagnetic surface modes tightly bound to flat plasmonic metamaterials that consist of metal surfaces decorated with two-dimensional arrays of subwavelength-periodicity pits. These modes are surface plasmon polaritons with an effective plasma frequency controlled entirely by the surface geometry4. The mode spectrum and penetration depth into air demonstrate strong wavelength-scale energy confinement to the surface below the electromagnetic band edge; this is in stark contrast to the very weak confinement found at flat metal surfaces in this spectral regime. The results are in good agreement with analytical and numerical models of surface plasmon polaritons propagating on structured perfect-conductor surfaces, and imply that plasmonic metamaterials could help miniaturize optical components or lead to improved chemical or biochemical sensors.

Highly confined guiding of terahertz surface plasmon polaritons on structured metal surfaces

We review photonic applications of dielectric whispering-gallery mode (WGM) resonators-tracing the growth of the technology from experiments with levitating droplets of aerosols to ultrahigh-Q solid state crystalline and integrated on-chip microresonators.

Optical resonators with whispering-gallery modes-part II: applications

The far-infrared absorption and index of refraction of high-resistivity, float-zone, crystalline silicon has been measured by terahertz time-domain spectroscopy. The measured new upper limit for the absorption of this most transparent dielectric material in the far infrared shows unprecedented transparency over the range from 0.5 to 2.5 THz and a well-resolved absorption feature at 3.6 THz. The index of refraction shows remarkably little dispersion, changing by only 0.0001 over the range from 0.5 to 4.5 THz.

Terahertz time-domain spectroscopy characterization of the far-infrared absorption and index of refraction of high-resistivity, float-zone silicon

We report an experimental and theoretical study of THz Sommerfeld wave propagation on a single copper wire. THz pulses are optoelectronically generated and launched onto 0.52-mm-diam copper wire, and the guided THz pulses are detected at the end of the wire by a standard photoconductive antenna. Very low attenuation and group velocity dispersion are observed, and the measured radial field amplitude of the Sommerfeld wave is inversely proportional to the radial distance. These results are consistent with theoretical predictions. Experimental results from curved wires show the weakly guiding property of the THz Sommerfeld wave, which will limit its applications.

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THz Sommerfeld wave propagation on a single metal wire

Via THz time-domain spectroscopy, we have measured the absorption and index of refraction of single-crystal 〈110〉 ZnTe from 0.3 to 4.5 THz. We find that the absorption is dominated by two lower-frequency phonon lines at 1.6 and 3.7 THz and not by the transverse-optical (TO) -phonon line at 5.3 THz as previously assumed. However, the index of refraction is determined mainly by the TO-phonon line. Using these data, we discuss a frequency-domain picture of electro-optic detection of THz radiation below the TO-phonon resonance and compare with the photoconductive THz receiver over the same frequency range.

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Measurements of the thz absorption and dispersion of znte and their relevance to the electro-optic detection of thz radiation

Waveguide terahertz time-domain spectroscopy is demonstrated to have the sensitivity to characterize nanometer-thick water layers on the surfaces of a parallel-plate metal waveguide. The measured far-infrared absorption and index of refraction of the 20-nm water layers are in reasonable self-consistent agreement with those of bulk water.

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Waveguide terahertz time-domain spectroscopy of nanometer water layers.

We demonstrate the efficient coupling of THz pulses into and out of an adiabatically compressed parallel-plate metal waveguide. The plate separation of the 63.5-mm long, compressed waveguide was fixed at 103μm at the entrance and exit ends for efficient coupling, but could be reduced in the middle. The experimental results show strong transmission of the THz signal through the compressed waveguide for a minimum midpoint separation of only 8μm. This technique can be used to achieve efficient coupling together with higher sensitivity for waveguide THz-TDS.

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Jiangquan Zhang

Papers

Terahertz time-domain spectroscopy characterization of the far-infrared absorption and index of refraction of high-resistivity, float-zone silicon

THz Sommerfeld wave propagation on a single metal wire

Measurements of the thz absorption and dispersion of znte and their relevance to the electro-optic detection of thz radiation

Waveguide terahertz time-domain spectroscopy of nanometer water layers.

Adiabatic compression of parallel-plate metal waveguides for sensitivity enhancement of waveguide THz time-domain spectroscopy