Exciting advancements have been made in the field of flexible electronic devices in the last two decades and will certainly lead to a revolution in peoples’ lives in the future. However, because of the poor sustainability of the active materials in complex stress environments, new requirements have been adopted for the construction of flexible devices. Thus, hierarchical architectures in natural materials, which have developed various environment-adapted structures and materials through natural selection, can serve as guides to solve the limitations of materials and engineering techniques. This review covers the smart designs of structural materials inspired by natural materials and their utility in the construction of flexible devices. First, we summarize structural materials that accommodate mechanical deformations, which is the fundamental requirement for flexible devices to work properly in complex environments. Second, we discuss the functionalities of flexible devices induced by nature-inspired stru...

/pdf/nature-inspired-structural-materials-for-flexible-electronic-3pusz1g5tt.pdf

Nature-Inspired Structural Materials for Flexible Electronic Devices

Soft electronics are intensively studied as the integration of electronics with dynamic nonplanar surfaces has become necessary. Here, a discussion of the strategies in materials innovation and structural design to build soft electronic devices and systems is provided. For each strategy, the presentation focuses on the fundamental materials science and mechanics, and example device applications are highlighted where possible. Finally, perspectives on the key challenges and future directions of this field are presented.

Materials and Structures toward Soft Electronics.

Origami has been employed to build deployable mechanical metamaterials through folding and unfolding along the crease lines. Deployable metamaterials are usually flexible, particularly along their deploying and collapsing directions, which unfortunately in many cases leads to an unstable deployed state, i.e., small perturbations may collapse the structure along the same deployment path. Here we create an origami-inspired mechanical metamaterial with on-demand deployability and selective collapsibility through energy analysis. This metamaterial has autonomous deployability from the collapsed state and can be selectively collapsed along two different paths, embodying low stiffness for one path and substantially high stiffness for another path. The created mechanical metamaterial yields load-bearing capability in the deployed direction while possessing great deployability and collapsibility. The principle in this work can be utilized to design and create versatile origami-inspired mechanical metamaterials that can find many applications.

https://www.pnas.org/content/pnas/115/9/2032.full.pdf

Origami-inspired, on-demand deployable and collapsible mechanical metamaterials with tunable stiffness

Developing mechanical metamaterials with programmable properties is an emerging topic receiving wide attention. While the programmability mainly originates from structural multistability in previously designed metamaterials, here it is shown that nonflat-foldable origami provides a new platform to achieve programmability via its intrinsic self-locking and reconfiguration capabilities. Working with the single-collinear degree-4 vertex origami tessellation, it is found that each unit cell can self-lock at a nonflat configuration and, therefore, possesses wide design space to program its foldability and relative density. Experiments and numerical analyses are combined to demonstrate that by switching the deformation modes of the constituent cell from prelocking folding to postlocking pressing, its stiffness experiences a sudden jump, implying a limiting-stopper effect. Such a stiffness jump is generalized to a multisegment piecewise stiffness profile in a multilayer model. Furthermore, it is revealed that via strategically switching the constituent cells' deformation modes through passive or active means, the n-layer metamaterial's stiffness is controllable among 2n target stiffness values. Additionally, the piecewise stiffness can also trigger bistable responses dynamically under harmonic excitations, highlighting the metamaterial's rich dynamic performance. These unique characteristics of self-locking origami present new paths for creating programmable mechanical metamaterials with in situ controllable mechanical properties.

Programmable Self-Locking Origami Mechanical Metamaterials.

DOI: 10.1002/admi.201800284 expand the range of accessible 3D geometries.[5–8] Due to their shape-adaptive nature, origami and kirigami, originally applied only to paper, can serve as routes to large-scale structural systems that require packaging and deployment, such as foldable solar panels,[9,10] retractable roofs,[11] deployable sunshields,[12] and many others.[13] More recent work demonstrates that these and related methods for assembling planar materials into complex 3D structures can exploit sophisticated 2D fabrication technologies and thin film materials from the electronics/optoelectronics industries, to yield functional systems in 3D designs that were previously unachievable.[14–18] In this way, the techniques of origami/kirigami can enable many classes of nontraditional devices not only at the macroscale but also at the micro/ nanoscale, with the potential to open up opportunities for unusual engineering designs in microsystems technologies.[19–22] Much research in origami/kirigami assembly aims to extend the range of length scales and the scope of functional materials that can be realized in 3D systems, and to transfer those ideas and Origami and kirigami, the ancient techniques for making paper works of art, also provide inspiration for routes to structural platforms in engineering applications, including foldable solar panels, retractable roofs, deployable sunshields, and many others. Recent work demonstrates the utility of the methods of origami/kirigami and conceptually related schemes in cutting, folding, and buckling in the construction of devices for emerging classes of technologies, with examples in mechanical/optical metamaterials, stretchable/ conformable electronics, micro/nanoscale biosensors, and large-amplitude actuators. Specific notable progress is in the deployment of functional materials such as single-crystal silicon, shape memory polymers, energy-storage materials, and graphene into elaborate 3D micro and nanoscale architectures. This review highlights some of the most important developments in this field, with a focus on routes to assembly that apply across a range of length scales and with advanced materials of relevance to practical applications. Hall of Fame Article

/pdf/assembly-of-advanced-materials-into-3d-functional-structures-406a74gx8i.pdf

Assembly of Advanced Materials into 3D Functional Structures by Methods Inspired by Origami and Kirigami: A Review

The manipulation and characterization of light polarization states are essential for many applications in quantum communication and computing, spectroscopy, bioinspired navigation, and imaging. Chiral metamaterials and metasurfaces facilitate ultracompact devices for circularly polarized light generation, manipulation, and detection. Herein, we report bioinspired chiral metasurfaces with both strong chiral optical effects and low insertion loss. We experimentally demonstrated submicron-thick circularly polarized light filters with peak extinction ratios up to 35 and maximum transmission efficiencies close to 80% at near-infrared wavelengths (the best operational wavelengths can be engineered in the range of 1.3–1.6 µm). We also monolithically integrated the microscale circular polarization filters with linear polarization filters to perform full-Stokes polarimetric measurements of light with arbitrary polarization states. With the advantages of easy on-chip integration, ultracompact footprints, scalability, and broad wavelength coverage, our designs hold great promise for facilitating chip-integrated polarimeters and polarimetric imaging systems for quantum-based optical computing and information processing, circular dichroism spectroscopy, biomedical diagnosis, and remote sensing applications. Inspired by the polarization-sensitive vision of the compound eyes in a marine crustacean called the Mantis Shrimp, researchers from Arizona State University, US have designed a chiral metasurface for manipulating the polarization of light. The metasurface design consists of a thin nanostructured silicon layer, a dielectric spacer layer and a gold nanowire polarizer, and has a total thickness of less than 1 micrometer. This thin planar surface offers low optical loss with a transmission as high as 80% in the near-infrared wavelength range, and acts as a circular polarization filter with an extinction ratio as high as 35. The circular polarization filters, in combination with linear polarization filters, can enable chip-scale polarimeters for sensing the polarization state of light. This on-chip integrated approach could prove useful in ultra-compact devices for advanced imaging and sensing applications.

/pdf/nature-inspired-chiral-metasurfaces-for-circular-57icc6njmy.pdf

Nature-inspired chiral metasurfaces for circular polarization detection and full-Stokes polarimetric measurements.

Flat optics presents a new path to control the phase, amplitude, and polarization state of light with ultracompact devices. Here we demonstrate chip-integrated metasurface devices for polarization detection of mid-infrared light with arbitrary polarization states. Six high-performance microscale linear and circular polarization filters based on vertically stacked plasmonic metasurfaces (with total thickness <600  nm) are integrated on the same chip to obtain all four Stokes parameters of light with high accuracy. The device designs can be tailored to operate at any wavelength in the mid-infrared spectral region and are feasible for on-chip integration with mid-infrared (mid-IR) photodetectors and imager arrays. Our work will enable on-chip mid-IR polarimeters and polarimetric imaging systems, which are highly desirable for many applications, such as clinical diagnosis, target detection, and space exploration.

Chip-integrated plasmonic flat optics for mid-infrared full-Stokes polarization detection

A new methodology to create 3D origami patterns out of Si nanomembranes using pre-stretched and pre-patterned polydimethylsiloxane substrates is reported. It is shown this approach is able to mimic paper-based origami patterns. The combination of origami-based microscale 3D architectures and stretchable devices will lead to a breakthrough on reconfigurable systems.

Microscale Silicon Origami

Plasmonic chiral metamaterials have attracted broad research interest because of their potential applications in optical communication, biomedical diagnosis, polarization imaging, and circular dichroism spectroscopy. However, optical losses in plasmonic structures severely limit practical applications. Here, we present the design concept and experimental demonstration for highly efficient subwavelength-thick plasmonic chiral metamaterials with strong chirality. The proposed designs utilize plasmonic metasurfaces to control the phase and polarization of light and exploit anisotropic thin-film interference effects to enhance optical chirality while minimizing optical loss. Based on such design concepts, we demonstrated experimentally optical devices such as circular polarization filters with transmission efficiency up to 90% and extinction ratio >180, polarization converters with conversion efficiency up to 90%, as well as on-chip integrated microfilter arrays for full Stokes polarization detection with high accuracy over a broad wavelength range (3.5-5 μm). The proposed design concepts are applicable from near-infrared to Terahertz regions via structural engineering.

Jing Bai

Papers

Nature-inspired chiral metasurfaces for circular polarization detection and full-Stokes polarimetric measurements.

Chip-integrated plasmonic flat optics for mid-infrared full-Stokes polarization detection

Microscale Silicon Origami

Highly Efficient Anisotropic Chiral Plasmonic Metamaterials for Polarization Conversion and Detection.

Printing continuous metal structures via polymer-assisted photochemical deposition