A review on thermal and catalytic pyrolysis of plastic solid waste (PSW)

The continuous increase in the generation of waste plastics together with the need for developing more sustainable waste management policies have promoted a great research effort dealing with their valorization routes. In this review, the main thermochemical routes are analyzed for the valorization of waste polyolefins to produce chemicals and fuels. Amongst the different strategies, pyrolysis has received greater attention, but most studies are of preliminary character. Likewise, the studies pursuing the incorporation of waste plastics into refinery units (mainly fluid catalytic cracking and hydrocracking) have been carried out in batch laboratory-scale units. Other promising alternative to which great attention is being paid is the process based on two steps: pyrolysis and in-line intensification for olefin production by means of catalytic cracking or thermal cracking at high temperatures.

Thermochemical routes for the valorization of waste polyolefinic plastics to produce fuels and chemicals. A review

The global energy transition towards a carbon neutral society requires a profound transformation of electricity generation and consumption, as well as of electric power systems. Hydrogen has an important potential to accelerate the process of scaling up clean and renewable energy, however its integration in power systems remains little studied. This paper reviews the current progress and outlook of hydrogen technologies and their application in power systems for hydrogen production, re-electrification and storage. The characteristics of electrolysers and fuel cells are demonstrated with experimental data and the deployments of hydrogen for energy storage, power-to-gas, co- and tri-generation and transportation are investigated using examples from worldwide projects. The current techno-economic status of these technologies and applications is presented, in which cost, efficiency and durability are identified as the main critical aspects. This is also confirmed by the results of a statistical analysis of the literature. Finally, conclusions show that continuous efforts on performance improvements, scale ramp-up, technical prospects and political support are required to enable a cost-competitive hydrogen economy.

Hydrogen energy systems: A critical review of technologies, applications, trends and challenges

Co-pyrolysis of biomass and waste plastics as a thermochemical conversion technology for high-grade biofuel production: Recent progress and future directions elsewhere worldwide

This review gives a worldwide overview on Power-to-Gas projects producing hydrogen or renewable substitute natural gas focusing projects in central Europe. It deepens and completes the content of previous reviews by including hitherto unreviewed projects and by combining project names with details such as plant location. It is based on data from 153 completed, recent and planned projects since 1988 which were evaluated with regards to plant allocation, installed power development, plant size, shares and amounts of hydrogen or substitute natural gas producing examinations and product utilization phases. Cost development for electrolysis and carbon dioxide methanation was analyzed and a projection until 2030 is given with an outlook to 2050. The results show substantial cost reductions for electrolysis as well as for methanation during the recent years and a further price decline to less than 500 euro per kilowatt electric power input for both technologies until 2050 is estimated if cost projection follows the current trend. Most of the projects examined are located in Germany, Denmark, the United States of America and Canada. Following an exponential global trend to increase installed power, today's Power-to-Gas applications are operated at about 39 megawatt. Hydrogen and substitute natural gas were investigated on equal terms concerning the number of projects.

Power-to-Gas: Electrolysis and methanation status review

Optimum biomass drying for combustion - a modeling approach.

Technical, economic and environmental assessments of projected power-to-gas (PtG) deployment scenarios at distributed- to national-scale are reviewed, as well as their extensions to nuclear-assisted renewable hydrogen. Their collective research trends, outcomes, challenges and limitations are highlighted, leading to suggested future work areas. These studies have focused on the conversion of excess wind and solar photovoltaic electricity in European-based energy systems using low-temperature electrolysis technologies. Synthetic natural gas, either solely or with hydrogen, has been the most frequent PtG product. However, the spectrum of possible deployment scenarios has been incompletely explored to date, in terms of geographical/sectorial application environment, electricity generation technology, and PtG processes, products and their end-uses to meet a given energy system demand portfolio. Suggested areas of focus include PtG deployment scenarios: (i) incorporating concentrated solar- and/or hybrid renewable generation technologies; (ii) for energy systems facing high cooling and/or water desalination/treatment demands; (iii) employing high-temperature and/or hybrid hydrogen production processes; and (iv) involving PtG material/energy integrations with other installations/sectors. In terms of PtG deployment simulation, suggested areas include the use of dynamic and load/utilization factor-dependent performance characteristics, dynamic commodity prices, more systematic comparisons between power-to-what potential deployment options and between product end-uses, more holistic performance criteria, and formal optimizations.

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Papers

Optimum biomass drying for combustion - a modeling approach.

A Review of Projected Power-to-Gas Deployment Scenarios

Mixed-waste pyrolysis of biomass and plastics waste – A modelling approach to reduce energy usage

Mechanism and modelling of bamboo pyrolysis

Drying of biomass for power generation: A case study on power generation from empty fruit bunch