Journal•ISSN: 0278-6826
Aerosol Science and Technology
Taylor & Francis
About: Aerosol Science and Technology is an academic journal published by Taylor & Francis. The journal publishes majorly in the area(s): Aerosol & Particle. It has an ISSN identifier of 0278-6826. Over the lifetime, 3866 publications have been published receiving 156221 citations.
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TL;DR: The optical properties of light-absorbing, carbonaceous substance often called "soot", "black carbon", or "carbon black" have been the subject of some debate as discussed by the authors.
Abstract: The optical properties of the light-absorbing, carbonaceous substance often called “soot,” “black carbon,” or “carbon black" have been the subject of some debate. These properties are necessary to model how aerosols affect climate, and our review is targeted specifically for that application. We recommend the term light-absorbing carbon to avoid conflict with operationally based definitions. Absorptive properties depend on molecular form, particularly the size of sp 2-bonded clusters. Freshly-generated particles should be represented as aggregates, and their absorption is like that of particles small relative to the wavelength. Previous compendia have yielded a wide range of values for both refractive indices and absorption cross section. The absorptive properties of light-absorbing carbon are not as variable as is commonly believed. Our tabulation suggests a mass-normalized absorption cross section of 7.5 ± 1.2 m2/g at 550 nm for uncoated particles. We recommend a narrow range of refractive indices for s...
2,312 citations
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TL;DR: The authors revisited common assumptions for estimating PM2.5 mass concentration and found that these assumptions can be used to estimate organic mass in a wide range of scenarios, such as PM1.5.
Abstract: (2001). Species Contributions to PM2.5 Mass Concentrations: Revisiting Common Assumptions for Estimating Organic Mass. Aerosol Science and Technology: Vol. 35, No. 1, pp. 602-610.
1,842 citations
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1,809 citations
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TL;DR: In this article, a thermal-optical technique for analysis of the carbonaceous fraction of particulate diesel exhaust is reported, and the speciation of organic and elemental carbon is accomplished through temperature and atmosphere control, and by an optical feature that corrects for pyrolytically generated carbon.
Abstract: Diesel exhaust has been classified a probable human carcinogen, and the National Institute for Occupational Safety and Health (NIOSH) has recommended that employers reduce workers' exposures. Because diesel exhaust is a chemically complex mixture containing thousands of compounds, some measure of exposure must be selected. Previously used methods involving gravimetry or analysis of the soluble organic fraction of diesel soot lack adequate sensitivity and selectivity for low-level determination of particulate diesel exhaust; a new analytical approach was therefore needed. In this paper, results of investigation of a thermal-optical technique for analysis of the carbonaceous fraction of particulate diesel exhaust are reported. With this technique, speciation of organic and elemental carbon is accomplished through temperature and atmosphere control, and by an optical feature that corrects for pyrolytically generated carbon, or “char,” which is formed during the analysis of some materials. The therma...
1,749 citations
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TL;DR: In this article, the authors describe an aerosol mass spectrometer (AMS) which has been developed in response to these aerosol sampling needs and demonstrate quantitative mea surement capability for a laboratory-generated pure component NH4 NO3 aerosol.
Abstract: The importance of atmospheric aerosols in regulating the Earth's climate and their potential detrimental impact on air quality and human health has stimulated the need for instrumentation which can provide real-time analysis of size resolved aerosol, mass, and chemical composition We describe here an aerosol mass spectrometer (AMS) which has been developed in response to these aerosol sampling needs and present results which demonstrate quantitative mea surement capability for a laboratory-generated pure component NH4 NO3 aerosol The instrument combines standard vacuum and mass spectrometric technologies with recently developed aerosol sampling techniques A unique aerodynamic aerosol inlet (developed at the University of Minnesota) focuses particles into a narrow beam and efficiently transports them into vacuum where aerodynamic particle size is determined via a particle time-of-flight (TOF) measurement Time-resolved particle mass detection is performed mass spectrometrically following particle flash
1,357 citations