Journal ArticleDOI
Quantum Beats in Transmission by Time-Resolved Polarization Spectroscopy
W. Lange,Jürgen Mlynek +1 more
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TLDR
In this paper, the time evolution of a coherent superposition of atomic substates created by a short resonant laser pulse is monitored via changes in polarization of a delayed probe pulse due to stimulated emission.Abstract:
A novel technique is described for high-resolution spectroscopy. The time evolution of a coherent superposition of atomic substates created by a short resonant laser pulse is monitored via changes in polarization of a delayed probe pulse due to stimulated emission. As a demonstration the method was applied to the Zeeman splitting of the $6^{3}P_{1}$ state of ytterbium.read more
Citations
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Journal ArticleDOI
Dynamic effects in nonlinear magneto-optics of atoms and molecules: review
Evgeniy B. Alexandrov,Marcis Auzinsh,Dmitry Budker,Derek F. Jackson Kimball,Simon M. Rochester,Valeriy V. Yashchuk +5 more
TL;DR: In this paper, a brief review is given of topics relating to dynamical processes arising in nonlinear interactions between light and resonant systems (atoms or molecules) in the presence of a magnetic field.
Book ChapterDOI
Chapter 9 – Dynamics
TL;DR: In this article, a short excitation pulse creates a coherent superposition of several nondegenerate eigenstates or quasi-eigenstates (that is, decaying states described in the complex energy formalism).
Journal ArticleDOI
Quantum beat spectroscopy of molecules
Erwin Hack,J. R. Huber +1 more
TL;DR: In this article, a review of the application of quantum beat in high-resolution spectroscopy is presented with special emphasis on the theoretical description of the quantum beat technique and its applications.
Journal ArticleDOI
A simple method of observing coherent ground state transients
Jürgen Mlynek,W. Lange +1 more
TL;DR: In this paper, it was shown that coherence between nondegenerate sublevels of an atomic ground state is efficiently induced by means of a short resonant light pulse, which can sensitively be detected by a polarization technique.
Journal ArticleDOI
Molecular quantum beat spectroscopy
H. Bitto,J. Robert Huber +1 more
TL;DR: In this article, the authors present an account of high-resolution molecular quantum beat spectroscopy and emphasize the versatility of this powerful Doppler-free method, which can be applied to intramolecular relaxation dynamics and the determination of structural parameters such as nuclear hyperfine constants, electric dipole moments, spin-orbit matrix elements and asymmetry splitting.
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