Showing papers on "Femtosecond pulse shaping published in 2021"

Extremely regular periodic surface structures in a large area efficiently induced on silicon by temporally shaped femtosecond laser

Abstract: Femtosecond laser-induced periodic surface structures (LIPSS) have several applications in surface structuring and functionalization. Three major challenges exist in the fabrication of regular and uniform LIPSS: enhancing the periodic energy deposition, reducing the residual heat, and avoiding the deposited debris. Herein, we fabricate an extremely regular low-spatial-frequency LIPSS (LSFL) on a silicon surface by a temporally shaped femtosecond laser. Based on a 4f configuration zero-dispersion pulse shaping system, a Fourier transform limit (FTL) pulse is shaped into a pulse train with varying intervals in the range of 0.25–16.2 ps using periodic π-phase step modulation. Under the irradiation of the shaped pulse with an interval of 16.2 ps, extremely regular LSFLs are efficiently fabricated on silicon. The scan velocity for fabricating regular LSFL is 2.3 times faster, while the LSFL depth is 2 times deeper, and the diffraction efficiency is 3 times higher than those of LSFL using the FTL pulse. The formation mechanisms of regular LSFL have been studied experimentally and theoretically. The results show that the temporally shaped pulse enhances the excitation of surface plasmon polaritons and the periodic energy deposition while reducing the residual thermal effects and avoiding the deposition of the ejected debris, eventually resulting in regular and deeper LSFL on the silicon surface.

Calibration of the pixel crosstalk in spatial light modulators for 4f pulse shaping.

Abstract: The targeted shaping of femtosecond pulses in 4f pulse shapers is complicated by, among other factors, the crosstalk between adjacent pixels of a spatial light modulator (SLM). Current methods for the crosstalk evaluation require setting up a different experiment, which is highly inconvenient. Here, we propose a simple procedure to extract the pixel crosstalk within the standard SLM calibration used in pulse shaping. The calibration is based on an analysis of the contrast of a periodic modulation in the spectra induced via SLM. We demonstrate the calibration procedure on a liquid-crystal-based SLM and show that we attain a constant crosstalk effect represented by a Gaussian function with σ=1.0 pix over a broad operational range of the SLM.

Programmable, direct space-to-time picosecond resolution pulse shaper with nanosecond record

Abstract: We demonstrate a novel, to the best of our knowledge, extension of optical arbitrary waveform generation capable of picosecond resolution over nanosecond duration. The method, called space–time induced linearly encoded transcription for temporal optimization, is based on direct space-to-time pulse shaping and is extended here to single-mode output with a programmable temporal profile. We develop the theory of operation and discuss ultimate limits on resolution, record length, and efficiency. We report on the results of an experimental demonstration showing ∼1ps resolution over 600 ps.

Coherent 2D electronic spectroscopy with complete characterization of excitation pulses during all scanning steps

Abstract: Coherent two-dimensional (2D) electronic spectroscopy has become a standard tool in ultrafast science. Thus it is relevant to consider the accuracy of data considering both experimental imperfections and theoretical assumptions about idealized conditions. It is already known that chirped excitation pulses can affect 2D line shapes. In the present work, we demonstrate performance-efficient, automated characterization of the full electric field of each individual multipulse sequence employed during a 2D scanning procedure. Using Fourier-transform spectral interferometry, we analyze how the temporal intensity and phase profile varies from scanning step to scanning step and extract relevant pulse-sequence parameters. This takes into account both random and systematic variations during the scan that may be caused, for example, by femtosecond pulse-shaping artifacts. Using the characterized fields, we simulate and compare 2D spectra obtained with idealized and real shapes obtained from an LCD-based pulse shaper. Exemplarily, we consider fluorescence of a molecular dimer and multiphoton photoemission of a plasmonic nanoslit. The deviations from pulse-shaper artifacts in our specific case do not distort strongly the population-based multidimensional data. The characterization procedure is applicable to other pulses-shaping technologies or excitation geometries, including also pump–probe geometry with multipulse excitation and coherent detection, and allows for accurate consideration of realistic optical excitation fields at all inter-pulse time-delays.

Acousto-optic modulator based dispersion scan for phase characterization and shaping of femtosecond mid-infrared pulses.

Abstract: Compression, shaping and characterization of broadband mid-infrared (MIR) pulses based on an acousto-optic modulator (AOM) pulse shaper is presented. Characterization of the spectral phase is achieved by an AOM-shaper based implementation of a dispersion scan (d-scan). The abilities of the setup are demonstrated by imprinting several test phases with increasing complexity on broadband MIR pulses centered at 3.2 µm and retrieval of the imprinted phases with the presented d-scan method. Phase characterization with d-scan in combination with an evolutionary algorithm allows us to compress the MIR pulses below 50 fs FWHM autocorrelation after the shaper.

Induced modulation of a chirped laser pulse at terahertz frequency with spectral phase shaping

Abstract: The possibility of using harmonic modulation of the spectral phase to generate multiple replicas of the original short laser pulse or controlled periodic intensity modulation at the terahertz frequency of the stretched chirped laser pulse is shown theoretically and experimentally.

Direct reconstruction of two ultrashort pulses based on non-interferometric frequency-resolved optical gating.

Abstract: We describe a non-interferometric ultrashort-pulse measurement technique based on frequency-resolved optical gating (FROG) with which pulses can be reconstructed directly, i.e. non-iteratively. Two different FROG spectrograms are measured, which represent the only information required to reconstruct the amplitudes and phases of two independent input pulses. The direct reconstruction method is demonstrated with a single-shot FROG setup used to obtain the spectrograms generated from two synchronized input pulses. To demonstrate and determine the reconstruction quality for complex pulses, a programmable pulse shaper is used to modify the pulses sourced from a Kerr-lens mode-locked Ti:sapphire oscillator.

Phase-only femtosecond optical pulse shaping based on an all-dielectric polarization-insensitive metasurface.

Abstract: Recently, metasurfaces capable of manipulating the amplitude and the phase of an incident wave in a broad frequency band have been employed for femtosecond optical pulse shaping purposes. In this study, we introduce a phase-only pulse shaper based on an all-dielectric CMOS-compatible polarization-insensitive metasurface, composed of Si nano cylinders sitting on a fused silica substrate. The required phase profile of the metasurface for desired waveforms are calculated using an iterative Fourier transform algorithm, and the performance of the pulse shaper metasurface in implementing the phase masks was assessed using full-wave simulations. Such approach for realizing a polarization-insensitive metasurface-based phase-only pulse shaper has never been investigated to the best of our knowledge. It is demonstrated that the simulated results of the proposed metasurface-based pulse shaper is in great agreement with the results of the algorithm, while exhibiting a very high transmission efficiency. This work indicates yet another exciting but not fully examined application of meta-structures that is the optical pulse shaping.

Information transfer from the optical phase to a plasmonic digital encoder composed of a gold nanorod pair.

Abstract: Small all-optical devices are central to the optical computing. Plasmonic digital encoders (PDEs) with a featured dimension of ∼1µm hold the key for transferring information from far field to photonic processing systems. Here we propose a PDE design composed of two gold nanorods (AuNRs), whose pattern represents 2-bit digital information. We implanted information into the spectral phase of a femtosecond pulse by pulse shaping and controlled the two-photon photoluminescence pattern of an AuNR pair. The high contrast ratios were achieved with 13.01 and 6.02 dB for binary codes "1-0" and "0-1", respectively.

Compact vectorial optical field generator using a single phase-only spatial light modulator.

Abstract: In this study, we demonstrate a compact vectorial optical field generator for any coherent light, including femtosecond laser beams. The apparatus utilizes a single Koster prism for both beam splitting and recombining. A phase-only spatial light modulator is used as a diffractive optical element to encode the two complex fields that recombine after being converted to orthogonal polarizations, generating an arbitrary vectorial optical field. We apply this setup to shape focused femtosecond pulses in producing patterned structures.

Independently programmable frequency-multiplexed phase-sensitive optical parametric amplification in the optical telecommunication band.

Abstract: We experimentally demonstrate programmable multimode phase-sensitive amplification multiplexed in the frequency domain for flexible control of parallelly generated squeezed states. We utilize the unique phase-matching condition of a type-II periodically poled potassium titanyl phosphate (PPKTP) crystal and pulse shaping technique to fully control the frequency-domain parallel generation of squeezed states in the optical telecommunication band. We experimentally verify that the independent programmability of phase-sensitive optical parametric amplification (OPA) for the modes corresponding to different frequency bands can be achieved by shaping the pump laser pulse from optical parametric gain measurements using a coherent probe light generated by a degenerate synchronously pumped optical parametric oscillator.

Neural-network-powered pulse reconstruction from one-dimensional interferometric cross-correlation traces.

Abstract: Any ultrafast optical spectroscopy experiment is usually accompanied by the necessary routine of ultrashort-pulse characterisation. The majority of pulse characterisation approaches solve either a one-dimensional (e.g. via interferometry) or a two-dimensional (e.g. via frequency-resolved measurements) problem. Solution of the two-dimensional pulse-retrieval problem is generally more consistent due to problem's over-determined nature. In contrast, the one-dimensional pulse-retrieval problem is impossible to solve unambiguously as ultimately imposed by the fundamental theorem of algebra. In cases where additional constraints are involved, the one-dimensional problem may be possible to solve, however, existing iterative algorithms lack generality, and often stagnate for complicated pulse shapes. Here we use a deep neural network to unambiguously solve a constrained one-dimensional pulse-retrieval problem and show the potential of fast, reliable, and complete pulse characterisation using interferometric cross-correlation time traces (determined by the pulses with partial spectral overlap).

Formation of spiraling infrared emission patterns by controlled interaction of optical filaments.

Abstract: We analyzed the formation of mid-infrared conical emission patterns possessing spiral and half-ring shaped wavelength contours from a beam of a few optical filaments. The complex patterns were generated and modified experimentally by adaptive wavefront shaping of the femtosecond laser pulse. Mutual interactions between co-propagating filaments can induce curvature in their paths, and the spiral and half-ring emissions were shown to be a direct consequence of this angular deflection. Based on our experimental and computational results, the spirals form in the far-field due to self-interference of conical emission from a helically moving filament. The presented findings will advance the tailoring of spatial conical emission patterns potentially beneficial for spectroscopic applications and terahertz generation.

Unlocking coherent control of the extreme ultrafast plasmonic excitation

Abstract: We experimentally coherent control the extreme ultrafast excitation in plasmonic nanostructures within their coherence lifetime. We predict and demonstrate a significant enhancement of the nonlinearity greater than the nonlinearity induced by a maximally compressed pulse.