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Spinon Fermi surface in a triangular lattice quantum spin liquid YbMgGaO4

TLDR
In this article, the authors reported neutron scattering measurements that reveal broad spin excitations covering a wide region of the Brillouin zone in an extremely clean antiferromagnet YbMgGaO4.
Abstract
Quantum spin liquid (QSL) is an exotic quantum state of matter in which spins are highly entangled and remain disordered down to zero temperature. In addition to its relevance to high-temperature superconductivity and quantum-information applications, experimental identification of this new state of matter in its own right is of fundamental importance for our understanding of quantum matter. Theoretical studies have proposed various QSL ground states, most of which are characterized by exotic spin excitations with fractional quantum numbers (termed `spinon'). However, a conclusive experimental confirmation of any QSL and spinon excitations remains outstanding. Here, we report neutron scattering measurements that reveal broad spin excitations covering a wide region of the Brillouin zone in an extremely clean antiferromagnet YbMgGaO4. The observed diffusive spin excitation persists at the lowest measured energy and shows a clear upper excitation edge, which is naturally accounted by the particle-hole excitation of a spinon Fermi surface. Combining this with the low-temperature heat capacity results we propose that YbMgGaO4 is a gapless U(1) QSL with a spinon Fermi surface. Our results therefore identify a QSL in a perfect spin-1/2 triangular lattice occurring in the original proposal by Anderson.

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Journal ArticleDOI

Quantum spin liquids.

TL;DR: An overview of an exotic type of liquid Materials with interacting quantum spins that nevertheless do not order magnetically down to the lowest temperatures are candidates for a materials class called quantum spin liquids (QSLs), characterized by long-range quantum entanglement and are tricky to study theoretically.
Journal ArticleDOI

Quantum Spin Liquids

TL;DR: In the past few years, increasing evidence has accumulated for a number of materials suggesting that they have characteristics strongly reminiscent of those expected for a quantum spin liquid as mentioned in this paper, although there is not yet entirely convincing experimental evidence that any particular material has a spin liquid ground state.
Journal ArticleDOI

Valence Bonds in Random Quantum Magnets: Theory and Application to YbMgGaO 4

TL;DR: In this article, the effect of quenched disorder on spin-1/2 quantum magnets was analyzed and a theory for 2D valence-bond solids subject to weak bond randomness, as well as extensions to stronger disorder regimes where we make connections with quantum spin liquids was proposed.
Journal ArticleDOI

Crystalline Electric-Field Randomness in the Triangular Lattice Spin-Liquid YbMgGaO4

TL;DR: The CEF randomness gives rise to a distribution of the effective spin-1/2 g factors and explains the unprecedented broadening of low-energy magnetic excitations in the fully polarized ferromagnetic phase of YbMgGaO_{4}, although a distributionof magnetic couplings due to the Mg/Ga disorder may be important as well.
Journal ArticleDOI

A high-temperature quantum spin liquid with polaron spins

TL;DR: The existence of a quantum spin liquid in which quantum fluctuations of spins are sufficiently strong to preclude spin ordering down to zero temperature was originally proposed theoretically more than 40 years ago, but its experimental realization turned out to be very elusive as discussed by the authors.
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