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Model for Brillouin Scattering in Amorphous Solids

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TLDR
In this paper, an elastic continuum model for Brillouin scattering by an amorphous solid is presented, where light scatters on distorted plane wave acoustic phonons leads to the prediction that the scattered intensity plotted as a function of the frequency transfer Ωo consists of the usual BrillouIN peaks plus a background which, a t room temperature, goes like Ω; for small Ω o, but rises less steeply for larger Ω O, and may even bend over within the range of the validity of the model, depending on the correlation lengths for spatial fluctuations due
Abstract
An elastic continuum model is presented for Brillouin scattering by an amorphous solid. The assumption that light scatters on distorted plane wave acoustic phonons leads to the prediction that the scattered intensity plotted as a function of the frequency transfer Ωo consists of the usual Brillouin peaks plus a background which, a t room temperature, goes like Ωo; for small Ωo, but rises less steeply for larger Ωo, and may even bend over within the range of the validity of the model, depending on the correlation lengths for spatial fluctuations due to disorder and on the speeds of sound. For the case of a-Si, additional results are obtained with the help of existing experimental measurements. Es wird die Brillouinstreuung in a morphen Snbstanzen an einem elastischen Kontinuums-modell diskutiert. Die Annahme, das Licht an durch deformierte ebene Wellen beschriebenen akustischen Phononen gestreut wird, fiihrt zu folgenden Aussagen. Die Streuintensitiit als Funktion der Frequenzverschiebung besteht aus den ublichen Brillouin-Peaks und einem Hintergrund, der, bei Raumtemperaturen, fur kleine Ωo proportional zu Ω 2o ist. Mit wachsendem Ω o wachst der Hintergrund dam schwacher als Ω2o. Jc nach den Werten der Korrelationslangen fur raumliche Fluktuationen und der Schallgeschwindigkeiten kanner im Giiltigkeitsbereich des Modells sogar nach Erreichen eines Maximums wieder abfallen. ZusaItzliche Aussagen werden fur den Fall von a-Si unter Ausnutzung existierender Messungen gemacht.

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Citations
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Formation of glasses from liquids and biopolymers.

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Relaxation in glassforming liquids and amorphous solids

TL;DR: The field of viscous liquid and glassy solid dynamics is reviewed by a process of posing the key questions that need to be answered, and then providing the best answers available to the authors and their advisors at this time as mentioned in this paper.
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Raman Spectroscopy of Nanomaterials: How Spectra Relate to Disorder, Particle Size and Mechanical Properties

TL;DR: In this article, the authors provide a basic understanding of the information micro-Raman Spectroscopy (mRS) may yield when applied to nanomaterials, a generic term for describing nano-sized crystals and bulk homogeneous materials with a structural disorder at the nanoscale.
Journal ArticleDOI

The nature of boson peak in Raman scattering in glasses

TL;DR: In this article, it has been shown that the form of a low-frequency boson peak in Raman scattering is universal for glasses of different chemical compositions and that from this form one can determine the structural correlation function, i.e. the character of violations of ordered arrangement of atoms within several coordination spheres in non-crystalline solids.
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Vibrational dynamics and the structure of glasses

TL;DR: In this article, a model assuming a non-continuous structure of glasses is established to interpret the inelastic neutron scattering and Raman scattering, and size distributions of the blobs are deduced from neutron and raman scatterings.
References
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Journal ArticleDOI

Raman-Scattering Selection-Rule Breaking and the Density of States in Amorphous Materials

TL;DR: In this article, the dielectric correlation function in glasses is calculated and the assumption of short correlation length for normal modes breaks the momentum selection rules and leads to expressions for the first-order Raman-scattering intensity in terms of the density-of-state functions and known frequency-dependent amplitudes.
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Measurement of Elastic Constants at Low Temperatures by Means of Ultrasonic Waves–Data for Silicon and Germanium Single Crystals, and for Fused Silica

TL;DR: In this article, the authors measured velocities of propagation and elastic constants in the 10-30 cm range of a fused silica rod, through polystyrene or silicone one-quarter wavelength seal, and into the solid specimen.
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Brillouin Scattering in Cubic Crystals

TL;DR: In this paper, the authors used a helium-neon laser light source and a high-resolution grating spectrograph to study the Brillouin spectrum of light scattered from three alkali halide crystals: KCl, RbCl, and KI.
Journal ArticleDOI

Optical Spectra of Orientationally Disordered Crystals. I. Theory for Translational Lattice Vibrations

TL;DR: In this article, the authors considered a class of crystals in which the molecules are arranged on or near regular positions in space, but are irregularly oriented, and the irregular orientation of the molecules frequently perturbs only slightly the translational lattice vibrations of the crystal.
Journal ArticleDOI

Brillouin-Scattering Measurements on Silicon and Germanium

TL;DR: The first Brillouin scattering measurements on silicon and germanium were reported in this paper, where the optical absorption lies in the range of 10.4 to 6.5 GHz.
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