Showing papers by "Lucas Alados-Arboledas published in 2015"

A methodology for investigating dust model performance using synergistic EARLINET/AERONET dust concentration retrievals

Abstract: . Systematic measurements of dust concentration profiles at a continental scale were recently made possible by the development of synergistic retrieval algorithms using combined lidar and sun photometer data and the establishment of robust remote-sensing networks in the framework of Aerosols, Clouds, and Trace gases Research InfraStructure Network (ACTRIS)/European Aerosol Research Lidar Network (EARLINET). We present a methodology for using these capabilities as a tool for examining the performance of dust transport models. The methodology includes considerations for the selection of a suitable data set and appropriate metrics for the exploration of the results. The approach is demonstrated for four regional dust transport models (BSC-DREAM8b v2, NMMB/BSC-DUST, DREAMABOL, DREAM8-NMME-MACC) using dust observations performed at 10 ACTRIS/EARLINET stations. The observations, which include coincident multi-wavelength lidar and sun photometer measurements, were processed with the Lidar-Radiometer Inversion Code (LIRIC) to retrieve aerosol concentration profiles. The methodology proposed here shows advantages when compared to traditional evaluation techniques that utilize separately the available measurements such as separating the contribution of dust from other aerosol types on the lidar profiles and avoiding model assumptions related to the conversion of concentration fields to aerosol extinction values. When compared to LIRIC retrievals, the simulated dust vertical structures were found to be in good agreement for all models with correlation values between 0.5 and 0.7 in the 1–6 km range, where most dust is typically observed. The absolute dust concentration was typically underestimated with mean bias values of -40 to -20 μg m−3 at 2 km, the altitude of maximum mean concentration. The reported differences among the models found in this comparison indicate the benefit of the systematic use of the proposed approach in future dust model evaluation studies.

Hygroscopic growth of atmospheric aerosol particles based on active remote sensing and radiosounding measurements: selected cases in southeastern Spain

Abstract: . A new methodology based on combining active and passive remote sensing and simultaneous and collocated radiosounding data to study the aerosol hygroscopic growth effects on the particle optical and microphysical properties is presented. The identification of hygroscopic growth situations combines the analysis of multispectral aerosol particle backscatter coefficient and particle linear depolarization ratio with thermodynamic profiling of the atmospheric column. We analyzed the hygroscopic growth effects on aerosol properties, namely the aerosol particle backscatter coefficient and the volume concentration profiles, using data gathered at Granada EARLINET station. Two study cases, corresponding to different aerosol loads and different aerosol types, are used for illustrating the potential of this methodology. Values of the aerosol particle backscatter coefficient enhancement factors range from 2.1 ± 0.8 to 3.9 ± 1.5, in the ranges of relative humidity 60–90 and 40–83%, being similar to those previously reported in the literature. Differences in the enhancement factor are directly linked to the composition of the atmospheric aerosol. The largest value of the aerosol particle backscatter coefficient enhancement factor corresponds to the presence of sulphate and marine particles that are more affected by hygroscopic growth. On the contrary, the lowest value of the enhancement factor corresponds to an aerosol mixture containing sulphates and slight traces of mineral dust. The Hanel parameterization is applied to these case studies, obtaining results within the range of values reported in previous studies, with values of the γ exponent of 0.56 ± 0.01 (for anthropogenic particles slightly influenced by mineral dust) and 1.07 ± 0.01 (for the situation dominated by anthropogenic particles), showing the convenience of this remote sensing approach for the study of hygroscopic effects of the atmospheric aerosol under ambient unperturbed conditions. For the first time, the retrieval of the volume concentration profiles for these cases using the Lidar Radiometer Inversion Code (LIRIC) allows us to analyze the aerosol hygroscopic growth effects on aerosol volume concentration, observing a stronger increase of the fine mode volume concentration with increasing relative humidity.

EARLINET: potential operationality of a research network

Abstract: . In the framework of ACTRIS (Aerosols, Clouds, and Trace Gases Research Infrastructure Network) summer 2012 measurement campaign (8 June–17 July 2012), EARLINET organized and performed a controlled exercise of feasibility to demonstrate its potential to perform operational, coordinated measurements and deliver products in near-real time. Eleven lidar stations participated in the exercise which started on 9 July 2012 at 06:00 UT and ended 72 h later on 12 July at 06:00 UT. For the first time, the single calculus chain (SCC) – the common calculus chain developed within EARLINET for the automatic evaluation of lidar data from raw signals up to the final products – was used. All stations sent in real-time measurements of a 1 h duration to the SCC server in a predefined netcdf file format. The pre-processing of the data was performed in real time by the SCC, while the optical processing was performed in near-real time after the exercise ended. 98 and 79 % of the files sent to SCC were successfully pre-processed and processed, respectively. Those percentages are quite large taking into account that no cloud screening was performed on the lidar data. The paper draws present and future SCC users' attention to the most critical parameters of the SCC product configuration and their possible optimal value but also to the limitations inherent to the raw data. The continuous use of SCC direct and derived products in heterogeneous conditions is used to demonstrate two potential applications of EARLINET infrastructure: the monitoring of a Saharan dust intrusion event and the evaluation of two dust transport models. The efforts made to define the measurements protocol and to configure properly the SCC pave the way for applying this protocol for specific applications such as the monitoring of special events, atmospheric modeling, climate research and calibration/validation activities of spaceborne observations.

Study of mineral dust entrainment in the planetary boundary layer by lidar depolarisation technique

Abstract: Measurements on 27 June 2011 were performed over the Southern Iberian Peninsula at Granada EARLINET station, using active and passive remote sensing and airborne and surface in-situ data in order to study the entrainment processes between aerosols in the free troposphere and those in the planetary boundary layer (PBL). To this aim the temporal evolution of the lidar depolarisation, backscatter-related Angstrom exponent and potential temperature profiles were used in combination with the PBL contribution to the aerosol optical depth (AOD). Our results show that the mineral dust entrainment in the PBL was caused by the convective processes which ‘trapped’ the lofted mineral dust layer, distributing the mineral dust particles within the PBL. The temporal evolution of ground-based in-situ data evidenced the impact of this process at surface level. Finally, the amount of mineral dust in the atmospheric column available to be dispersed into the PBL was estimated by means of POLIPHON (Polarizing Lidar Photometer Networking). The dust mass concentration derived from POLIPHON was compared with the coarse-mode mass concentration retrieved with airborne in-situ measurements. Comparison shows differences below 50 µg/m 3 (30% relative difference) indicating a relative good agreement between both techniques. Keywords: Saharan mineral dust, atmospheric aerosol, lidar, lidar depolarisation technique, planetary boundary layer (Published: 29 May 2015) Citation: Tellus B 2015, 67, 26180, http://dx.doi.org/10.3402/tellusb.v67.26180

Aerosol properties over the western Mediterranean basin: temporal and spatial variability

Abstract: . This study focuses on the analysis of Aerosol Robotic Network (AERONET) aerosol data obtained over Alboran Island (35.90° N, 3.03° W, 15 m a.s.l.) in the western Mediterranean from July 2011 to January 2012. Additional aerosol data from the three nearest AERONET stations (Malaga, Oujda and Palma de Mallorca) and the Maritime Aerosol Network (MAN) were also analyzed in order to investigate the temporal and spatial variations of aerosol over this scarcely explored region. High aerosol loads over Alboran were mainly associated with desert dust transport from North Africa and occasional advection of anthropogenic fine particles from central European urban-industrial areas. The fine particle load observed over Alboran was surprisingly similar to that obtained over the other three nearest AERONET stations, suggesting homogeneous spatial distribution of fine particle loads over the four studied sites in spite of the large differences in local sources. The results from MAN acquired over the Mediterranean Sea, Black Sea and Atlantic Ocean from July to November 2011 revealed a pronounced predominance of fine particles during the cruise period.

High temporal resolution estimates of columnar aerosol microphysical parameters from spectrum of aerosol optical depth by linear estimation: application to long-term AERONET and star-photometry measurements

Abstract: . This work deals with the applicability of the linear estimation technique (LE) to invert spectral measurements of aerosol optical depth (AOD) provided by AERONET CIMEL sun photometers. The inversion of particle properties using only direct-sun AODs allows the evaluation of parameters such as effective radius (reff) and columnar volume aerosol content (V) with significantly better temporal resolution than the operational AERONET algorithm which requires both direct sun and sky radiance measurements. Sensitivity studies performed demonstrate that the constraints on the range of the inversion are very important to minimize the uncertainties, and therefore estimates of reff can be obtained with uncertainties less than 30 % and of V with uncertainties below 40 %. The LE technique is applied to data acquired at five AERONET sites influenced by different aerosol types and the retrievals are compared with the results of the operational AERONET code. Good agreement between the two techniques is obtained when the fine mode predominates, while for coarse mode cases the LE results systematically underestimate both reff and V. The highest differences are found for cases where no mode predominates. To minimize these biases, correction functions are developed using the multi-year database of observations at selected sites, where the AERONET retrieval is used as the reference. The derived corrections are tested using data from 18 other AERONET stations offering a range of aerosol types. After correction, the LE retrievals provide better agreement with AERONET for all the sites considered. Finally, the LE approach developed here is applied to AERONET and star-photometry measurements in the city of Granada (Spain) to obtain day-to-night time evolution of columnar aerosol microphysical properties.

Intercomparisons of Mobility Size Spectrometers and Condensation Particle Counters in the Frame of the Spanish Atmospheric Observational Aerosol Network

Abstract: Red Espanola de DMAs Ambientales (REDMAAS), the Spanish network of environmental differential mobility analyzers (DMAs), currently comprises six research groups involved in the measurement of atmospheric aerosol size distributions by means of DMAs. The aim of this network is to guarantee the good quality and comparability of the routine measurements carried out at each location and in diverse environments across Spain. In order to achieve this objective, one of its main activities is the annual intercomparison of mobility size spectrometers used within the network (five units of scanning mobility particle sizers [SMPS] and one ultrafine particle monitor [UFPM]). Here we report the 2main results obtained during the 2010–2012 campaigns, including a study on particle deposition in dryers used in ambient air sampling systems. In general, all instruments showed good performance with deviations in accepted tolerance. The intercomparisons have been proved to be a useful exercise to detect instrument problems, su...

Role of spheroidal particles in closure studies for aerosol microphysical–optical properties

Abstract: A study has been carried out to assess the discrepancies between computed and observed aerosol scattering and backscattering properties in the atmosphere. The goals were: (i) to analyse the uncertainty associated with computed optical properties when spherical and spheroidal approximations are used, and (ii) to estimate nephelometry errors due to angular truncation and non-Lambertian illumination of the light source in terms of size range, particle shape and aerosol chemical compounds. Mie and T-matrix theories were used for computing light optical properties for spherical and spheroidal particles, respectively, from observed particle size distributions. The scattering coefficient of the fine mode was not much influenced by the particle shape. However, computed backscattering values underestimated the observed values by ∼15%. For the coarse mode, the spheroidal approximation yielded better results than that for spherical particles, especially for backscattering properties. Even after applying the spheroidal approximation, computed scattering and backscattering values within the coarse mode underestimated the observed values by ∼49% and ∼11%, respectively. The angular correction most widely used to correct the nephelometer data was discussed to explore its uncertainty. In the case of the scattering properties within the coarse mode, the change of the computed optical parameter is ∼+8% and for the scattering and backscattering values within the fine mode it is lower than ∼±4% for spherical and spheroidal particles. Additionally, if the spheroidal particles are used to evaluate the aerosol optical properties, the correction must be reconsidered with the aim of reducing the uncertainty found for scattering within the coarse mode. This is recommended for sites with desert dust influence; then the deviation of the computed scattering can be up to 13%.

Assessment of African desert dust episodes over the southwest Spain at sea level using in situ aerosol optical and microphysical properties

Abstract: Desert dust (DD) aerosols reach the El Arenosillo observatory (southwest Spain) following two characteristic pathways at sea level, each showing significant differences in its aerosol microphysical and optical properties. These differences, in turn, determine the influence on the radiative forcing over the region. For these events, the meteorological scenarios show a depression located over North Africa at ground level. A Mediterranean pathway occurs when: (1) the depression is located over North Africa and the Mediterranean Basin or (2) it is coupled to a high pressure in higher latitudes. A North Africa pathway is observed when the depression is located only over North Africa. In our inventory, there are clear DD episodes under the Mediterranean flow, whereas other specific DD events take place under a mixture of Mediterranean and North African flows. The pure Mediterranean flow is associated with a higher increase of particle volume and scattering coefficient within the sub-micron than the super-micron size ranges. This result indicates that the contribution to the radiative forcing through the scattering processes over the region for particles with D 1 µm. In contrast, the episodes with a mixture of Mediterranean and North African flows show a similar effect of sub- and super-micron size ranges on radiative forcing. The size range with the largest impact on the scattering processes is 0.3 µm

Study of aerosol microphysical properties profiles retrieved from ground-based remote sensing and aircraft in-situ measurements during a Saharan dust event

Abstract: Introduction Conclusions References

Characterization of Saharan dust ageing over the western Mediterranean Basin during a multi-intrusion event in June 2013 in the framework of the ADRIMED/ChArMEx campaign

Abstract: In the framework of the ChArMEx (Chemistry-Aerosol Mediterranean Experiment, http://charmex.lsce.ipsl.fr/) initiative, a field campaign took place in the western Mediterranean Basin between 10 June and 5 July 2013 within the ADRIMED (Aerosol Direct Radiative Impact on the regional climate in the MEDiterranean region) project. The scientific objectives of the campaign were the characterization of the different aerosol types found over the Mediterranean Sea and the calculation of their direct radiative forcing (column closure and regional scale). Two super-sites (Ersa, Corsica Island, France, and Lampedusa Island, Italy) were equipped with a complete set of instruments to measure in-situ aerosol physical, chemical and optical properties, as well as aerosol mixing state and vertical distribution and radiative fluxes. Four secondary sites were operated in Granada (Spain), Menorca Island (Spain), Rome (Italy) and Lecce (Italy). All sites were equipped with AERONET sunphotometers. The ground observations were supported by airborne measurements including 2 SAFIRE aircraft (ATR-42 equipped with in situ measurements (10 June – 5 July) and Falcon-20 (17 June – 5 July) with the LNG aerosol lidar) and sounding and drifting balloons launched by CNES from Menorca Island and carrying the LOAC particle counter/sizer (16 June – 4 July). Satellite products from MODIS, MSG/SEVIRI and CALIOP provided additional observations. In several occasions corresponding to aerosol loads of different types, the aircraft flew near EARLINET/ACTRIS (European Aerosol Research Lidar Network / Aerosols, Clouds, and Trace gases Research InfraStructure Network, http://www.actris.net/) lidar stations. This work is focused on a moderate multi-intrusion Saharan dust event occurred over the western Mediterranean Basin (WMB) during the period 14 – 27 June. The dust plumes were detected by the EARLINET stations of Granada, Barcelona, Naples, Potenza, Lecce and Serra la Nave (Sicily) and by the ChArMEx lidar stations of Menorca, Ersa and Lampedusa. The dust origin is chronologically identified from northern Morocco, center Algeria and center Tunisia. The multi-intrusion aspect of the event results in aerosol optical depth peaks higher in the eastern part of the WMB (maximum of 0.45 at 440 nm detected in Lecce) than in the western part of the WMB where the event starts (maximum of 0.29 at 440 nm detected in Granada). The spatio-temporal evolution of the plumes during their transport and the differences due to the different dust origins are investigated with multi-wavelength ground-based lidars, sun-photometers, the airborne lidar and balloon-borne aerosol counters.

Atmospheric Particle Size Distributions in the Spanish Network of Environmental DMAs (REDMAAS)

Abstract: The present work is a first approach to the study of the spatio-temporal variability of the submicrometer atmospheric aerosol in Spain. The aerosol measurements have been obtained simultaneously at seven monitoring stations that compose the REDMAAS network during two measurement campaigns corresponding to summer and winter seasons.In both summer and winter periods those measurement stations with a direct influence of anthropogenic emissions recorded the highest concentrations of particle number. In the summer campaign, the average daily pattern of the aerosol size distribution in the traffic and background urban stations was conditioned by the traffic emissions and secondary aerosol formation through photochemical reactions (new particle formation events, NPF). However, the secondary aerosol had a higher contribution to the aerosol total number concentration in the rural background and high-altitude stations. In the winter campaign, in all sampling sites with the exception of Izana station, the traffic and domestic activity emissions had a greater contribution than secondary aerosol formation on particle number total concentration.New particle formation events were identified at all sites during the summer period, and at sites without direct influence of anthropogenic emissions during the winter campaign. Some aerosol shrinkage processes were also observed at the Madrid and El Arenosillo stations.

Aerosol cloud interaction: a multiplatform-scenario-based methodology

Abstract: Suspended atmospheric particles i.e. aerosol particles go through many chemical and physical processes and those interactions and transformations may cause particle change in size, structure and composition regulated by mechanisms, which are also present in clouds. These interactions play a great role in the radiation transfer in the atmosphere and are not completely understood as competing effects might occur which are known as indirect aerosol effects. Performing measurements and experiments in remote sensing to improve the knowledge of these processes are also a challenge. In face of that we propose a multi-platform approach based lidar, sun photometry and satellite observations which should be characterized under a scenario perspective in which given the cloud height, geometric and optical geometries in a diurnal/nocturnal basis will make possible to apply different analytical tools in each a set of product that specify the aerosol present in the vicinity of clouds, their optical and physical properties. These scenarios are meant to aid in tagging the expected products and help in creating a robust database to systematically study the aerosol-cloud interaction.In total we will present 6 scenarios: 3 under daylight conditions, 3 under at nighttime. Each scenario and their counterpart should be able to provide the cloud base/top height, aerosol backscattering profile and cloud optical/geometric thickness. In each instance we should count on a 5 wavelength Raman lidar system measurement, a collocated sun photometer and CALIPSO/MODIS observation from AQUA/TERRA platforms. To further improve the aerosol cloud interaction the Raman lidar system should have a water vapor channel or moreover a liquid water channel. In our study we will present a two-day case study to show the methodology feasibility and its potential application.