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Improvement of spectral resolution by using the excitation dependence of dipole–dipole interaction in a dense atomic gas

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TLDR
In this article, the authors studied the selective reflection from the interface between a dense rubidium (Rb) atomic vapor and a transparent dielectric, which can be used to improve the resolution of spectroscopy of dense media.
Abstract
We have studied the selective reflection from the interface between a dense rubidium (Rb) atomic vapor and a transparent dielectric. A remarkable narrowing of the spectrum, which can be used to improve the resolution of spectroscopy of dense media, has been demonstrated. This narrowing results from the reduction of the dipole–dipole interaction between atoms when the Rb vapor is excited by a strong pump laser. By using this technique, we have resolved the hyperfine structure of the Rb D2 line, which is hidden by collisional broadening.

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Citations
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Journal ArticleDOI

Probing dipole-dipole interaction in a rubidium gas via double-quantum 2D spectroscopy.

TL;DR: This technique provides sensitive and background-free detection of the dipole-dipole interaction and a theoretical model based on the optical Bloch equations is used to reproduce the experimental spectrum and confirm the origin of doublequantum signals.
Journal ArticleDOI

Long range dipole-dipole interaction in low-density atomic vapors probed by double-quantum two-dimensional coherent spectroscopy.

TL;DR: The experimental results confirm the long range nature of the dipole-dipole interaction, which is critical for understanding many-body physics in atoms/molecules and can open a new avenue to study long-range interactions in solid state systems such as quantum dots and color centers in diamonds.
Journal ArticleDOI

Observation of narrow Autler-Townes components in the resonant response of a dense atomic gas

TL;DR: In this article, the reflection of a weak probe beam from a dense atomic potassium vapor in the presence of a strong laser field tuned to the atomic resonance transition was studied under the Autler-Townes doublet condition.
Journal ArticleDOI

Line shapes of atomic transitions in excited dense gas

TL;DR: In this article, the authors discussed the results of experimental studies of dipole-dipole broadened line shapes in excited atomic vapors and the Lorentz local field shift and self-broadened width were measured in optically excited potassium and rubidium vapors.
Journal ArticleDOI

Excitation dependence of resonance line self-broadening at different atomic densities

TL;DR: In this article, the authors studied the dipole?dipole spectral broadening of a resonance line at high atomic densities when the self-broadening dominates, and found that the selfbroadening reduction dependence on the pump power is atomic density independent.
References
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Principles of Optics

Max Born, +1 more
TL;DR: In this article, the authors discuss various topics about optics, such as geometrical theories, image forming instruments, and optics of metals and crystals, including interference, interferometers, and diffraction.
Book

Principles of Nonlinear Optical Spectroscopy

Shaul Mukamel
TL;DR: In this article, the authors present a simulation of the optical response functions of a multilevel system with relaxation in a multimode Brownian Oscillator Model and a wavepacket analysis of nonimpulsive measurements.
Journal ArticleDOI

Electromagnetically Induced Transparency

TL;DR: Electromagnetic induced transparency is a technique for eliminating the effect of a medium on a propagating beam of electromagnetic radiation EIT may also be used, but under more limited conditions, to eliminate optical self-focusing and defocusing and to improve the transmission of laser beams through inhomogeneous refracting gases and metal vapors, as figure 1 illustrates.
Journal ArticleDOI

Superluminal and Slow Light Propagation in a Room-Temperature Solid

TL;DR: It is observed that ions in mirror sites are inversely saturable and cause superluminal light propagation, whereas ions in inversion sites experience conventional saturable absorption and produce slow light.
Journal ArticleDOI

Enhancement of the index of refraction via quantum coherence.

TL;DR: Atoms prepared in a coherent superposition of a ground- (or excited-) state doublet can produce a large resonant index of refraction with vanishing absorption.
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