Time-dependent density functional theory for many-electron systems interacting with cavity photons.
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It is shown that the electron-photon wave function is a unique functional of the electronic (current) density and the expectation values of photonic coordinates that naturally leads to time-dependent density functional theory for systems coupled to the Caldeira-Leggett bath.Abstract:
Time-dependent (current) density functional theory for many-electron systems strongly coupled to quantized electromagnetic modes of a microcavity is proposed. It is shown that the electron-photon wave function is a unique functional of the electronic (current) density and the expectation values of photonic coordinates. The Kohn-Sham system is constructed, which allows us to calculate the above basic variables by solving self-consistent equations for noninteracting particles. We suggest possible approximations for the exchange-correlation potentials and discuss implications of this approach for the theory of open quantum systems. In particular we show that it naturally leads to time-dependent density functional theory for systems coupled to the Caldeira-Leggett bath.read more
Citations
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Atoms and molecules in cavities, from weak to strong coupling in quantum-electrodynamics (QED) chemistry
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Polaritonic Chemistry with Organic Molecules
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Cavity-induced modifications of molecular structure in the strong-coupling regime
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References
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Inhomogeneous Electron Gas
P. C. Hohenberg,Walter Kohn +1 more
TL;DR: In this article, the ground state of an interacting electron gas in an external potential was investigated and it was proved that there exists a universal functional of the density, called F[n(mathrm{r})], independent of the potential of the electron gas.
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Density-Functional Theory for Time-Dependent Systems
Erich Runge,E. K. U. Gross +1 more
TL;DR: In this article, a time-dependent version of density functional theory was proposed to deal with the non-perturbative quantum mechanical description of interacting many-body systems moving in a very strong timedependent external field.
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Strong coupling of a single photon to a superconducting qubit using circuit quantum electrodynamics
Andreas Wallraff,David Schuster,Alexandre Blais,Luigi Frunzio,Ren-Shou Huang,Ren-Shou Huang,Johannes Majer,Sushant Kumar,Steven Girvin,Robert Schoelkopf +9 more
TL;DR: It is shown that the strong coupling regime can be attained in a solid-state system, and the concept of circuit quantum electrodynamics opens many new possibilities for studying the strong interaction of light and matter.
Journal ArticleDOI
Cavity quantum electrodynamics for superconducting electrical circuits: An architecture for quantum computation
Alexandre Blais,Ren-Shou Huang,Ren-Shou Huang,Andreas Wallraff,Steven Girvin,Robert Schoelkopf +5 more
TL;DR: In this paper, a realizable architecture using one-dimensional transmission line resonators was proposed to reach the strong coupling limit of cavity quantum electrodynamics in superconducting electrical circuits.