Showing papers by "Yaroslav Tserkovnyak published in 2020"

Creating zero-field skyrmions in exchange-biased multilayers through X-ray illumination

Abstract: Skyrmions, magnetic textures with topological stability, hold promises for high-density and energy-efficient information storage devices owing to their small size and low driving-current density. Precise creation of a single nanoscale skyrmion is a prerequisite to further understand the skyrmion physics and tailor skyrmion-based applications. Here, we demonstrate the creation of individual skyrmions at zero-field in an exchange-biased magnetic multilayer with exposure to soft X-rays. In particular, a single skyrmion with 100-nm size can be created at the desired position using a focused X-ray spot of sub-50-nm size. This single skyrmion creation is driven by the X-ray-induced modification of the antiferromagnetic order and the corresponding exchange bias. Furthermore, artificial skyrmion lattices with various arrangements can be patterned using X-ray. These results demonstrate the potential of accurate optical control of single skyrmion at sub-100 nm scale. We envision that X-ray could serve as a versatile tool for local manipulation of magnetic orders. Skyrmions are objects with whirled magnetization protected by their topology that can be created by different means, however, without control of their position. Here, the authors present a method exploiting x-rays to create skyrmions at the beam position allowing for creation of artificial skyrmion lattices.

Tuning entanglement by squeezing magnons in anisotropic magnets

Abstract: There has been much recent interest in coherently preparing and manipulating entanglement in various systems, stimulated by its importance in quantum information science. Here, the authors discuss entanglement between individual spins within anisotropic magnets in thermodynamic equilibrium, suggesting magnetic materials as a natural resource for processing quantum information. Furthermore, they show that entanglement can jump discontinuously by varying an applied magnetic field, which can potentially serve as a switch for quantum information processing tasks.

Observation of Magnon Polarons in a Uniaxial Antiferromagnetic Insulator.

Abstract: Magnon polarons, a type of hybridized excitations between magnons and phonons, were first reported in yttrium iron garnet as anomalies in the spin Seebeck effect responses. Here, we report an observation of antiferromagnetic (AFM) magnon polarons in a uniaxial AFM insulator Cr_{2}O_{3}. Despite the relatively higher energy of magnon than that of the acoustic phonons, near the spin-flop transition of ∼6 T, the left-handed magnon spectrum shifts downward to hybridize with the acoustic phonons to form AFM magnon polarons, which can also be probed by the spin Seebeck effect. The spin Seebeck signal is founded to be enhanced due to the magnon polarons at low temperatures.

Spin Seebeck effect near the antiferromagnetic spin-flop transition

Abstract: Author(s): Reitz, Derek; Li, Junxue; Yuan, Wei; Shi, Jing; Tserkovnyak, Yaroslav | Abstract: We develop a low-temperature, long-wavelength theory for the interfacial spin Seebeck effect (SSE) in easy-axis antiferromagnets. The field-induced spin-flop (SF) transition of N #x27;eel order is associated with a qualitative change in SSE behavior: Below SF, there are two spin carriers with opposite magnetic moments, with the carriers polarized along the field forming a majority magnon band. Above SF, the low-energy, ferromagnetic-like mode has magnetic moment opposite the field. This results in a sign change of the SSE across SF, which agrees with recent measurements on Cr$_2$O$_3$/Pt and Cr$_2$O$_3$/Ta devices [Li $\textit{et al.,}$ $\textit{Nature}$ $\textbf{578,}$ 70 (2020)]. In our theory, SSE is due to a N #x27;eel spin current below SF and a magnetic spin current above SF. Using the ratio of the associated N #x27;eel to magnetic spin-mixing conductances as a single constant fitting parameter, we reproduce the field dependence of the experimental data and partially the temperature dependence of the relative SSE jump across SF.

Spin-torque oscillation in a magnetic insulator probed by a single-spin sensor

Abstract: We locally probe the magnetic fields generated by a spin-torque oscillator (STO) in a microbar of ferrimagnetic insulator yttrium-iron-garnet using the spin of a single nitrogen-vacancy (NV) center in diamond. The combined spectral resolution and sensitivity of the NV sensor allows us to resolve multiple spin-wave modes and characterize their damping. When damping is decreased sufficiently via spin injection, the modes auto-oscillate, as indicated by a strongly reduced linewidth, a diverging magnetic power spectral density, and synchronization of the STO frequency to an external microwave source. These results open the way for quantitative, nanoscale mapping of the microwave signals generated by STOs, as well as harnessing STOs as local probes of mesoscopic spin systems.

Enhanced antiferromagnetic resonance linewidth in NiO/Pt and NiO/Pd

Abstract: In this paper, we investigate the enhancement of the antiferromagnetic damping in the sintered NiO-HM (where HM is heavy metal) granular systems having NiO/HM interfaces, where $\mathrm{HM}=\mathrm{Pt}$ or Pd. Under the assumption of the spin pumping model, we derive the effective interfacial damping conductance ${g}_{\mathrm{eff}}$, the parameter which characterizes the upper-bound estimate of the spin pumping effect, to be $12\ifmmode\pm\else\textpm\fi{}1\phantom{\rule{0.16em}{0ex}}\mathrm{n}{\mathrm{m}}^{\ensuremath{-}2}$ and $5\ifmmode\pm\else\textpm\fi{}1\phantom{\rule{0.16em}{0ex}}\mathrm{n}{\mathrm{m}}^{\ensuremath{-}2}$ for the NiO/Pt and the NiO/Pd interfaces, respectively, at room temperature. ${g}_{\mathrm{eff}}$ experimentally derived in this study are an important milestone in antiferromagnetic spintronics, giving a guideline for various spin current transfer and spin interaction phenomena with antiferromagnets where the spin mixing conductance is involved.

Quantum Sensing of Spin Transport Properties of an Antiferromagnetic Insulator

Abstract: Antiferromagnetic insulators (AFIs) are of significant interest due to their potential to develop next-generation spintronic devices. One major effort in this emerging field is to harness AFIs for long-range spin information communication and storage. Here, we report a non-invasive method to optically access the intrinsic spin transport properties of an archetypical AFI {\alpha}-Fe2O3 via nitrogen-vacancy (NV) quantum spin sensors. By NV relaxometry measurements, we successfully detect the time-dependent fluctuations of the longitudinal spin density of {\alpha}-Fe2O3. The observed frequency dependence of the NV relaxation rate is in agreement with a theoretical model, from which an intrinsic spin diffusion constant of {\alpha}-Fe2O3 is experimentally measured in the absence of external spin biases. Our results highlight the significant opportunity offered by NV centers in diagnosing the underlying spin transport properties in a broad range of high-frequency magnetic materials, which are challenging to access by more conventional measurement techniques.

Driving a magnetized domain wall in an antiferromagnet by magnons

Abstract: We theoretically study the interaction of magnons, quanta of spin waves, and a domain wall in a one-dimensional easy-axis antiferromagnet in the presence of an external magnetic field applied along the easy axis. To this end, we begin by obtaining the exact solution for spin waves in the background of a domain wall magnetized by an external field. The finite magnetization inside the domain wall is shown to give rise to reflection of magnons scattering off the domain wall, deviating from the well-known result of reflection-free magnons in the absence of a magnetic field. For practical applications of the predicted reflection of magnons, we show that the magnon reflection contributes to the thermally driven domain-wall motion. Our work leads us to envision that inducing a finite magnetization in antiferromagnetic solitons such as vortices and skyrmions can be used to engender phenomena that do not occur in the absence of magnetization.

Antiferromagnetic Switching Driven by the Collective Dynamics of a Coexisting Spin Glass

Abstract: The theory behind the electrical switching of antiferromagnets is premised on the existence of a well defined broken symmetry state that can be rotated to encode information. A spin glass is in many ways the antithesis of this state, characterized by an ergodic landscape of nearly degenerate magnetic configurations, choosing to freeze into a distribution of these in a manner that is seemingly bereft of information. In this study, we show that the coexistence of spin glass and antiferromagnetic order allows a novel mechanism to facilitate the switching of the antiferromagnet Fe$_{1/3+\delta}$NbS$_2$, which is rooted in the electrically-stimulated collective winding of the spin glass. The local texture of the spin glass opens an anisotropic channel of interaction that can be used to rotate the equilibrium orientation of the antiferromagnetic state. The use of a spin glass' collective dynamics to electrically manipulate antiferromagnetic spin textures has never been applied before, opening the field of antiferromagnetic spintronics to many more material platforms with complex magnetic textures.

Topological Transport of Deconfined Hedgehogs in Magnets.

Abstract: We theoretically investigate the dynamics of magnetic hedgehogs, which are three-dimensional topological spin textures that exist in common magnets, focusing on their transport properties and connections to spintronics. We show that fictitious magnetic monopoles carried by hedgehog textures obey a topological conservation law, based on which a hydrodynamic theory is developed. We propose a nonlocal transport measurement in the disordered phase, where the conservation of the hedgehog flow results in a nonlocal signal decaying inversely proportional to the distance. The bulk-edge correspondence between the hedgehog number and skyrmion number, the fictitious electric charges arising from magnetic dynamics, and the analogy between bound states of hedgehogs in ordered phase and the quark confinement in quantum chromodynamics are also discussed. Our study points to a practical potential in utilizing hedgehog flows for long-range neutral signal propagation or manipulation of skyrmion textures in three-dimensional magnetic materials.

Exceptional points in dissipatively coupled spin dynamics

Abstract: Nanoscale or continuum spin systems, including simple ferromagnets and antiferromagnets, can have their spectral properties strongly affected by damping and/or pumping. In particular, dissipation can tune the magnon band structure through a series of exceptional points, which constitute special topological degeneracies with potentially dramatic consequences for response properties of magnetic materials.

Antiferromagnet-Based Neuromorphics Using Dynamics of Topological Charges.

Abstract: We propose a spintronics-based hardware implementation of neuromorphic computing, specifically, the spiking neural network, using topological winding textures in one-dimensional antiferromagnets. The consistency of such a network is emphasized in light of the conservation of topological charges, and the natural spatiotemporal interconversions of magnetic winding. We discuss the realization of the leaky integrate-and-fire behavior of neurons and the spike-timing-dependent plasticity of synapses. Our proposal opens the possibility for an all-spin neuromorphic platform based on antiferromagnetic insulators.

Quantum hydrodynamics of spin winding

Abstract: An easy-plane spin winding in a quantum spin chain can be treated as a transport quantity, which propagates along the chain but has a finite lifetime due to phase slips. In a hydrodynamic formulation for the winding dynamics, the quantum continuity equation acquires a source term due to the transverse vorticity flow. The latter reflects the phase slips and generally compromises the global conservation law. A linear-response formalism for the nonlocal winding transport then reduces to a Kubo response for the winding flow along the spin chain, in conjunction with the parasitic vorticity flow transverse to it. One-dimensional topological hydrodynamics can be recovered when the vorticity flow is asymptotically small. Starting with a microscopic spin-chain formulation, we focus on the asymptotic behavior of the winding transport based on the renormalized sine-Gordon equation, incorporating phase slips as well as Gilbert damping. A generic electrical device is proposed to manifest this physics. We thus suggest winding conductivity as a tangible concept that can characterize low-energy dynamics in a broad class of quantum magnets.

Energy storage in magnetic textures driven by vorticity flow

Abstract: An experimentally feasible energy-storage concept is formulated based on vorticity (hydro)dynamics within an easy-plane insulating magnet. The free energy associated with the magnetic winding texture is built up in a circular easy-plane magnetic structure by injecting a vorticity flow in the radial direction. The latter is accomplished by electrically induced spin-transfer torque, which pumps energy into the magnetic system in proportion to the vortex flux. The resultant magnetic metastable state with a finite winding number can be maintained indefinitely because the process of its relaxation via phase slips is exponentially suppressed when the temperature is brought well below the Curie temperature. We characterize the vorticity-current interaction underlying the energy-loading mechanism through its contribution to the effective electric inductance in the rf response. Our proposal may open an avenue for naturally powering spintronic circuits and nontraditional magnet-based neuromorphic networks.

Edge-State Wave Functions from Momentum-Conserving Tunneling Spectroscopy.

Abstract: We perform momentum-conserving tunneling spectroscopy using a GaAs cleaved-edge overgrowth quantum wire to investigate adjacent quantum Hall edge states. We use the lowest five wire modes with their distinct wave functions to probe each edge state and apply magnetic fields to modify the wave functions and their overlap. This reveals an intricate and rich tunneling conductance fan structure which is succinctly different for each of the wire modes. We self-consistently solve the Poisson-Schr\"odinger equations to simulate the spectroscopy, reproducing the striking fans in great detail, thus, confirming the calculations. Further, the model predicts hybridization between wire states and Landau levels, which is also confirmed experimentally. This establishes momentum-conserving tunneling spectroscopy as a powerful technique to probe edge state wave functions.

Coupled spin-charge dynamics in magnetic van der Waals heterostructures

Abstract: We present a phenomenological theory for coupled spin-charge dynamics in magnetic van der Waals (vdW) heterostructures. The system studied consists of a layered antiferromagnet inserted into a capacitive vdW heterostructure. It has been recently demonstrated that charge doping in such layered antiferromagnets can modulate the strength, and even the sign, of exchange coupling between the layer magnetizations. This provides a mechanism for electrically generating magnetization dynamics. The central result we predict here is that the magnetization dynamics reciprocally results in inducing charge flows. Such dynamics makes magnetic van der Waals heterostructures interesting candidates for spintronics applications. To this end, we also show that these systems can be used to convert subterahertz-radiation-induced magnetization dynamics into electrical signals.

Driving a magnetized domain wall in an antiferromagnet by magnons

Abstract: We theoretically study the interaction of magnons, quanta of spin waves, and a domain wall in a one-dimensional easy-axis antiferromagnet in the presence of an external magnetic field applied along the easy axis. To this end, we begin by obtaining the exact solution for spin waves in the background of a domain wall magnetized by an external field. The finite magnetization inside the domain wall is shown to give rise to reflection of magnons scattering off the domain wall, deviating from the well-known result of reflection-free magnons in the absence of a magnetic field. For practical applications of the predicted reflection of magnons, we show that the magnon reflection contributes to the thermally-driven domain-wall motion. Our work leads us to envision that inducing a finite magnetization in antiferromagnetic solitons such as vortices and skyrmions can be used to engender phenomena that do not occur in the absence of magnetization.

Superconductivity-enhanced spin pumping: The role of Andreev bound-state resonances

Abstract: We describe a simple hybrid superconductor$|$ferromagnetic-insulator structure manifesting spin-resolved Andreev bound states in which dynamic magnetization is employed to probe spin related physics. We show that, at low bias and below $T_c$, the transfer of spin angular momentum pumped by an externally driven ferromagnetic insulator is greatly affected by the formation of spin-resolved Andreev bound states. Our results indicate that these bound states capture the essential physics of condensate-facilitated spin flow. For finite thicknesses of the superconducting layer, comparable to the coherence length, resonant Andreev bound states render highly transmitting subgap spin transport channels. We point out that the resonant enhancement of the subgap transport channels establishes a prototype Fabry-Perot resonator for spin pumping.

Collective spin dynamics under dissipative spin Hall torque.

Abstract: Current-induced spin torques in layered magnetic heterostructures have many commonalities across broad classes of magnetic materials. These include not only collinear ferromagnets, ferrimagnets, and antiferromagnets, but also more complex noncollinear spin systems. We develop a general Lagrangian-Rayleigh approach for studying the role of dissipative torques, which can pump energy into long-wavelength magnetic dynamics, causing dynamic instabilities. While the Rayleigh structure of such torques is similar for different magnetic materials, their consequences depend sensitively on the nature of the order and, in particular, on whether there is a net magnetic moment. The latter endows the system with a unipolar switching capability, while magnetically compensated materials tend to evolve towards limit cycles, at large torques, with chirality dependent on the torque sign. Apart from the ferromagnetic and antiferromagnetic cases, we discuss ferrimagnets, which display an intricate competition between switching and limit cycles. As a simple case for compensated noncollinear order, we consider isotropic spin glasses, as well as a scenario of their coexistence with a collinear magnetic order.