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Complex Magnetic Behavior of the Heusler Alloy—Cu 2 Mn 0.75 Fe 0.25 Al

TLDR
In this paper, the structural and magnetic properties of alloys were investigated, and the magnetic isotherms were fitted to modified Langevin equation which indicated the presence of clusters with large magnetic moment.
Abstract
We investigated the structural and magnetic properties of Cu 2 Mn 1-x Fe x Al (x = 0.25, 0.5, 0.75) alloys. Among the three compositions, only x = 0.25 composition crystallizes in single phase with L2 1 structure but its magnetic response indicates a complex magnetic structure. The magnetic isotherms were fitted to modified Langevin equation which indicates the presence of clusters with large magnetic moment. The ac susceptibility studies showed the presence of a superparamagnetic phase in the system over and above ferromagnetic order. To determine the nature of the interactions among the clusters, the variation of freezing temperature (T f ) with applied ac frequency was analyzed using different models (Neel-Arrhenius, Vogel-Fulcher, and critical slowing down model).

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Citations
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Coexistence of cluster ferromagnetism and cluster spin-glass like behaviour in melt-quenched Cu2Mn0.5Fe0.5Al Heusler alloy

TL;DR: In this article, the structural stability and magnetic properties of the melt-quenched Heusler alloy-Cu2Mn0.5Al were investigated using X-ray diffraction (XRD), scanning electron microscopy (SEM), dc magnetization and ac susceptibility measurements respectively.
Posted Content

Exotic magnetic behaviour and evidence of cluster glass and Griffiths like phase in Heusler alloys Fe2-xMnxCrAl

TL;DR: A detailed study of structural, magnetic and thermodynamic properties of a series of Heusler alloys Fe2-xMnxCrAl (x=0, 0.25 and 0.75 and 1) was carried out using high resolution synchrotron X-ray diffraction as mentioned in this paper.
Journal ArticleDOI

Griffiths phase and spontaneous magnetization in polycrystalline Co50V34Ga16 alloy

TL;DR: In this paper, the Griffiths phase was found in Co-V-Ga alloy for the first time using the DSC curve and the inverse DC susceptibility (χ−1) in the high temperature region.
Journal ArticleDOI

Effect of partial substitution of iso-valent Mo at Cr-site on electronic structure and physical properties of Fe2CrAl

TL;DR: In this article, the effect of partial substitution of Mo at Cr-site on physical properties of Fe2CrAl was investigated and structural and morphological analysis confirmed the single phase cubic structure of the substituted alloys.
Journal ArticleDOI

Structural, Electronic and Magnetic Properties of the Heusler Alloy Mn 2 VIn: A Combined DFT and Experimental Study

TL;DR: In this paper, the structural, electronic and magnetic properties of the Heusler alloy Mn2VIn have been investigated using the density functional theory and experimental techniques, and the structural properties were determined using X-ray diffraction, revealing the presence of cubic and tetragonal phases in the sample.
References
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Journal ArticleDOI

New Class of Materials: Half-Metallic Ferromagnets

TL;DR: The band structure of Mn-based Heusler alloys of the crystal structure (MgAgAs type) has been calculated with the augmented-spherical-wave method.
Journal ArticleDOI

Formation and coupling of magnetic moments in Heusler alloys

TL;DR: In this article, the microscopic mechanisms responsible for both the formation and coupling of magnetic moments in Heusler alloys were identified, and it was shown that the $X$ atoms (e.g., Cu, Pd) serve primarily to determine the lattice constant, while the $Y$ atoms mediate the interaction between the $\mathrm{Mn}d$ states.
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Magnetic properties and large magnetic-field-induced strains in off-stoichiometric Ni–Mn–Al Heusler alloys

TL;DR: In this article, magnetic properties and magnetic-field-induced strains (MFIS) have been investigated for off-stoichiometric Ni-Mn-Al Heusler alloys with an ordered L21 structure.
Journal ArticleDOI

Heusler Compounds—A Material Class With Exceptional Properties

TL;DR: An overview of Heusler compounds, focusing on their structure, properties, and potential applications, can be found in this article, with a focus on the X2YZ compound.
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