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Luminescent Ce(III) Complexes as Stoichiometric and Catalytic Photoreductants for Halogen Atom Abstraction Reactions.

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TLDR
The strongly reducing metalloradical character of 1, 1-(i)Pr, and 1-Cy in their (2)A1 excited states afforded photochemical halogen atom abstraction reactions from sp(3) and sp(2) C-X (X = Cl, Br, I) bonds for the first time with a lanthanide cation.
Abstract
Luminescent Ce(III) complexes, Ce[N(SiMe3)2]3 (1) and [(Me3Si)2NC(RN)2]Ce[N(SiMe3)2]2 (R = iPr, 1-iPr; R = Cy, 1-Cy), with C3v and C2v solution symmetries display absorptive 4f → 5d electronic transitions in the visible region. Emission bands are observed at 553, 518, and 523 nm for 1, 1-iPr, and 1-Cy with lifetimes of 24, 67, and 61 ns, respectively. Time-dependent density functional theory (TD-DFT) studies on 1 and 1-iPr revealed the 2A1 excited states corresponded to singly occupied 5dz2 orbitals. The strongly reducing metalloradical character of 1, 1-iPr, and 1-Cy in their 2A1 excited states afforded photochemical halogen atom abstraction reactions from sp3 and sp2 C–X (X = Cl, Br, I) bonds for the first time with a lanthanide cation. The dehalogenation reactions could be turned over with catalytic amounts of photosensitizers by coupling salt metathesis and reduction to the photopromoted atom abstraction reactions.

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Patent

Organic Electroluminescent Materials and Devices

TL;DR: In this paper, novel tricarbazole compounds with appropriate HOMO and LUMO energies can be obtained for use as materials in a secondary hole transport layer, by appropriately selecting the nature of the tricarazole substituents.
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Selective functionalization of methane, ethane, and higher alkanes by cerium photocatalysis

TL;DR: The development of photocatalytic C–H amination, alkylation, and arylation of methane, ethane, and higher alkanes under visible light irradiation at ambient temperature is reported.
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Photoactive Complexes with Earth-Abundant Metals

TL;DR: The focus is on conceptually new, structurally well-characterized complexes with excited-state lifetimes between 10 ps and 1 ms in fluid solution for possible applications in photosensitizing, light-harvesting, luminescence and catalysis.
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δ-Selective Functionalization of Alkanols Enabled by Visible-Light-Induced Ligand-to-Metal Charge Transfer.

TL;DR: Under mild redox-neutral conditions without the need for prefunctionalization, this method provides a versatile platform to access molecular complexity from simple and abundant alcohols.
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Photocatalytic C−C Bond Cleavage and Amination of Cycloalkanols by Cerium(III) Chloride Complex

TL;DR: This work presents the first example of catalytic C-C bond cleavage and functionalization of unstrained secondary cycloalkanols through visible-light-induced photoredox catalysis utilizing a cerium(III) chloride complex.
References
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Book

Principles of fluorescence spectroscopy

TL;DR: This book describes the fundamental aspects of fluorescence, the biochemical applications of this methodology, and the instrumentation used in fluorescence spectroscopy.
Journal ArticleDOI

Visible Light Photoredox Catalysis with Transition Metal Complexes: Applications in Organic Synthesis

TL;DR: The conversion of these bench stable, benign catalysts to redox-active species upon irradiation with simple household lightbulbs represents a remarkably chemoselective trigger to induce unique and valuable catalytic processes.
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Kinetics of Fluorescence Quenching by Electron and H‐Atom Transfer

TL;DR: In this article, the rate constants of 60 typical electron donor-acceptor systems have been measured in de-oxygenated acetonitrile and are shown to be correlated with the free enthalpy change, ΔG23, involved in the actual electron transfer process.
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Visible light photoredox catalysis: applications in organic synthesis

TL;DR: This tutorial review provides a historical overview of visible light photoredox catalysis in organic synthesis along with recent examples which underscore its vast potential to initiate organic transformations.
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Visible light photocatalysis as a greener approach to photochemical synthesis

TL;DR: Transition metal photocatalysis represents a promising strategy towards the development of practical, scalable industrial processes with great environmental benefits.
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