Pure dephasing and phonon dynamics in GaAs- and GaN-based quantum dot structures: Interplay between material parameters and geometry

TLDR: In this article, the pure dephasing of excitons in quantum dot structures due to their interaction with acoustic phonons as well as the spatiotemporal dynamics of the created nonequilibrium phonon population is studied theoretically.

Abstract: The pure dephasing of excitons in quantum dot structures due to their interaction with acoustic phonons as well as the spatiotemporal dynamics of the created nonequilibrium phonon population is studied theoretically. The theory is applied to GaAs- as well as GaN-based heterostructures. A detailed analysis of the interplay between different material parameters, different quantum dot geometries, and different electric fields is presented. The optical polarization induced by an ultrashort laser pulse exhibits a characteristic nonexponential behavior: it decays on a pico- or subpicosecond time scale to a value that strongly depends on temperature, structure, and material parameters and is then retained until, on a typically much longer time scale, it finally decays because of electron-hole recombination or transitions to other states. We find that, in general, the remnant optical polarization is much higher in the GaAs-based structures than in the GaN-based structure mainly because of the strongly enhanced piezoelectric coupling in GaN quantum dots. The optical excitation also leads to the buildup of a phonon population consisting of a polaron part that remains localized in the region of the quantum dot and a traveling part that leaves the dot region at the speed of sound. This traveling part exhibits characteristic anisotropies reflecting both the anisotropy of the quantum dot structure and of the coupling matrix elements.