Journal ArticleDOI
Ru-based multifunctional mesoporous catalyst for low-pressure and non-thermal plasma synthesis of ammonia
Peng Peng,Yanling Cheng,Raymond Hatzenbeller,Min Addy,Nan Zhou,Charles Schiappacasse,Dongjie Chen,Yaning Zhang,Yaning Zhang,Erik Anderson,Yuhuan Liu,Paul Chen,Roger Ruan,Roger Ruan +13 more
TLDR
In this article, the synthesis of ammonia using NTP and a Ru-based, multifunctional catalytic system deposited on mesoporous Si-MCM-41 was reported.About:
This article is published in International Journal of Hydrogen Energy.The article was published on 2017-07-27. It has received 73 citations till now. The article focuses on the topics: Ammonia production & Nonthermal plasma.read more
Citations
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Journal ArticleDOI
Greening Ammonia toward the Solar Ammonia Refinery
Lu Wang,Meikun Xia,Hong Wang,Kefeng Huang,Chenxi Qian,Christos T. Maravelias,Geoffrey A. Ozin +6 more
TL;DR: In light of the targets set out by the Paris Climate Agreement and the global energy sector's ongoing transition from fossil fuels to renewables, the chemical industry is searching for innovative ways of reducing greenhouse gas emissions associated with the production of ammonia as discussed by the authors.
Journal ArticleDOI
Catalysis Enabled by Plasma Activation of Strong Chemical Bonds: A Review
TL;DR: It is highlighted how plasma activation of reactants can provide access to overall reaction rates, conversions, product yields, and/or product distributions unattainable by thermal catalysis at similar temperatures and pressures.
Journal ArticleDOI
Photocatalytic Fixation of Nitrogen to Ammonia by Single Ru Atom Decorated TiO2 Nanosheets
Shizhen Liu,Yajun Wang,Shaobin Wang,Mingmu You,Song Hong,Tai-Sing Wu,Yun-Liang Soo,Zhenqing Zhao,Guiyuan Jiang,Jieshan Qiu,Baojun Wang,Zhenyu Sun +11 more
TL;DR: In this paper, single Ru decorated TiO2 nanosheets rich in oxygen vacancies were synthesized, which greatly promoted photoreduction of aqueous N2 to NH3, affording an NH3 formation rate of 56.3 μg/h/gcat.
Journal ArticleDOI
A review on the non-thermal plasma-assisted ammonia synthesis technologies
Peng Peng,Paul Chen,Charles Schiappacasse,Nan Zhou,Erik Anderson,Dongjie Chen,Juer Liu,Yanling Cheng,Raymond Hatzenbeller,Min Addy,Yaning Zhang,Yaning Zhang,Yuhuan Liu,Roger Ruan +13 more
TL;DR: In this article, a systematic review of the plasma-assisted ammonia synthesis under low temperature and pressure conditions is presented, which represents a promising alternative method of clean ammonia synthesis, as it circumvents the volatile operating conditions, fossil fuel use, and high capital costs of the Haber-Bosch process.
Journal ArticleDOI
Plasma-driven catalysis: green ammonia synthesis with intermittent electricity
Kevin Hendrik Reindert Rouwenhorst,Yannick Engelmann,Kevin van ’t Veer,Kevin van ’t Veer,Rolf Sybren Postma,Annemie Bogaerts,Leon Lefferts +6 more
TL;DR: A review of the literature on plasma-driven ammonia synthesis is presented in this article, where the authors distinguish between mechanisms for ammonia synthesis in the presence of a plasma, with and without a catalyst, for different plasma conditions.
References
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Book
Infrared and Raman Spectra of Inorganic and Coordination Compounds
TL;DR: In this article, the normal modes of vibration are illustrated and corresponding vibrational frequencies are listed for each type, including diatomic, triatomic, fouratomic, five-atomic, six-atomic and seven-atomic types.
Journal ArticleDOI
A new family of mesoporous molecular sieves prepared with liquid crystal templates
Jeffrey S. Beck,James C. Vartuli,Wieslaw J. Roth,M. E. Leonowicz,Charles T. Kresge,Kirk D. Schmitt,Cynthia Ting-Wah Chu,David H. Olson,E. W. Sheppard,S. B. McCullen,J. B. Higgins,J.L. Schlenker +11 more
TL;DR: In this paper, the synthesis, characterization, and proposed mechanism of formation of a new family of silicatelaluminosilicate mesoporous molecular sieves designated as M41S is described.
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How a century of ammonia synthesis changed the world
TL;DR: On 13 October 1908, Fritz Haber filed his patent on the "synthesis of ammonia from its elements" for which he was later awarded the 1918 Nobel Prize in Chemistry as mentioned in this paper.
Journal ArticleDOI
Ammonia synthesis using a stable electride as an electron donor and reversible hydrogen store
Masaaki Kitano,Yasunori Inoue,Youhei Yamazaki,Fumitaka Hayashi,Shinji Kanbara,Satoru Matsuishi,Toshiharu Yokoyama,Sung Wng Kim,Sung Wng Kim,Michikazu Hara,Hideo Hosono +10 more
TL;DR: Kinetic analysis with infrared spectroscopy reveals that C12A7:e(-) markedly enhances N(2) dissociation on Ru by the back donation of electrons and that the poisoning of ruthenium surfaces by hydrogen adatoms can be suppressed effectively because of the ability of C12 a7: e(-) to store hydrogen reversibly.