Showing papers by "Michael Jensen published in 2021"

New particle formation in the remote marine boundary layer.

Abstract: Marine low clouds play an important role in the climate system, and their properties are sensitive to cloud condensation nuclei concentrations. While new particle formation represents a major source of cloud condensation nuclei globally, the prevailing view is that new particle formation rarely occurs in remote marine boundary layer over open oceans. Here we present evidence of the regular and frequent occurrence of new particle formation in the upper part of remote marine boundary layer following cold front passages. The new particle formation is facilitated by a combination of efficient removal of existing particles by precipitation, cold air temperatures, vertical transport of reactive gases from the ocean surface, and high actinic fluxes in a broken cloud field. The newly formed particles subsequently grow and contribute substantially to cloud condensation nuclei in the remote marine boundary layer and thereby impact marine low clouds. Globally, new particle formation represents a major source of cloud condensation nuclei. Here, the authors present evidence of frequent occurrence of new particle formation in the upper part of remote marine boundary layer following cold front passages.

Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA)

Abstract: With their extensive coverage, marine low clouds greatly impact global climate. Presently, marine low clouds are poorly represented in global climate models, and the response of marine low clouds to changes in atmospheric greenhouse gases and aerosols remains the major source of uncertainty in climate simulations. The Eastern North Atlantic (ENA) is a region of persistent but diverse subtropical marine boundary layer clouds, whose albedo and precipitation are highly susceptible to perturbations in aerosol properties. In addition, the ENA is periodically impacted by continental aerosols, making it an excellent location to study the cloud condensation nuclei (CCN) budget in a remote marine region periodically perturbed by anthropogenic emissions, and to investigate the impacts of long-range transport of aerosols on remote marine clouds. The Aerosol and Cloud Experiments in Eastern North Atlantic (ACE-ENA) campaign was motivated by the need of comprehensive in-situ measurements for improving the understanding of marine boundary layer CCN budget, cloud and drizzle microphysics, and the impact of aerosol on marine low cloud and precipitation. The airborne deployments took place from June 21 to July 20, 2017 and January 15 to February 18, 2018 in the Azores. The flights were designed to maximize the synergy between in-situ airborne measurements and ongoing long-term observations at a ground site. Here we present measurements, observation strategy, meteorological conditions during the campaign, and preliminary findings. Finally, we discuss future analyses and modeling studies that improve the understanding and representation of marine boundary layer aerosols, clouds, precipitation, and the interactions among them.

Vertical profiles of trace gas and aerosol properties over the eastern North Atlantic: variations with season and synoptic condition

Abstract: . Because of their extensive coverage, marine low clouds greatly impact the global climate. Presently, the response of marine low clouds to the changes in atmospheric aerosols remains a major source of uncertainty in climate simulations. One key contribution to this large uncertainty derives from the poor understanding of the properties and processes of marine aerosols under natural conditions and the perturbation by anthropogenic emissions. The eastern North Atlantic (ENA) is a region of persistent but diverse subtropical marine boundary layer (MBL) clouds, where cloud albedo and precipitation are highly susceptible to perturbations in aerosol properties. Here we examine the key processes that drive the cloud condensation nuclei (CCN) population in the MBL using comprehensive characterizations of aerosol and trace gas vertical profiles during the Aerosol and Cloud Experiments in the Eastern North Atlantic (ACE-ENA) field campaign. During ACE-ENA, a total of 39 research flights were conducted in the Azores: 20 during summer 2017 and 19 during winter 2018. During summer, long-range-transported aerosol layers were periodically observed in the lower free troposphere (FT), leading to elevated FT CCN concentrations ( NCCN ). Both biomass burning and pollution from North America contribute to submicron aerosol mass in these layers, with pollution likely the dominant contributor. In contrast, long-range transported continental emissions have a much weaker influence on the aerosol properties in the ENA during the winter season. While the entrainment of FT air is a major source of particle number in the MBL for both seasons, on average it does not serve as a direct source of CCN in the MBL because the average FT NCCN is the same or even lower than that in the MBL. The particle number flux due to FT entrainment is dominated by pre-CCN (particles that are too small to form cloud droplets under typical conditions, i.e., particles with sizes below the Hoppel minimum) due to the elevated Npre-CCN in the lower FT. Once these pre-CCN are entrained into the MBL, they can grow and reach CCN size range through condensational growth, representing an indirect and major source of MBL CCN in the ENA. The impact of synoptic conditions on the aerosol properties is examined. Under pre-front and post-front conditions, shallow convective activity often leads to a deep and decoupled boundary layer. Coalescence scavenging and evaporation of drizzle below clouds lead to reduced NCCN and larger accumulation-mode particle sizes in the upper cloud-containing decoupled layer, indicating that surface measurements overestimate the NCCN relevant to the formation of MBL clouds under decoupled conditions.

Contrasting characteristics of open- and closed-cellular stratocumulus cloud in the eastern North Atlantic

Abstract: . Extensive regions of marine boundary layer cloud impact the radiative balance through their significant shortwave albedo while having little impact on outgoing longwave radiation. Despite this importance, these cloud systems remain poorly represented in large-scale models due to difficulty in representing the processes that drive their life cycle and coverage. In particular, the mesoscale organization and cellular structure of marine boundary clouds have important implications for the subsequent cloud feedbacks. In this study, we use long-term (2013–2018) observations from the Atmospheric Radiation Measurement (ARM) Facility's Eastern North Atlantic (ENA) site on Graciosa Island, Azores, Portugal, to identify cloud cases with open- or closed-cellular organization. More than 500 h of each organization type are identified. The ARM observations are combined with reanalysis and satellite products to quantify the cloud, precipitation, aerosol, thermodynamic, and large-scale synoptic characteristics associated with these cloud types. Our analysis shows that both cloud organization populations occur during similar sea surface temperature conditions, but the open-cell cases are distinguished by stronger cold-air advection and large-scale subsidence compared to the closed-cell cases, consistent with their formation during cold-air outbreaks. We also find that the open-cell cases were associated with deeper boundary layers, stronger low-level winds, and higher rain rates compared to their closed-cell counterparts. Finally, raindrops with diameters larger than 1 mm were routinely recorded at the surface during both populations, with a higher number of large drops during the open-cellular cases. The similarities and differences noted herein provide important insights into the environmental and cloud characteristics during varying marine boundary layer cloud mesoscale organization and will be useful for the evaluation of model simulations for ENA marine clouds.

What drives daily precipitation over the central Amazon? Differences observed between wet and dry seasons

Abstract: . This study offers an alternative presentation regarding how diurnal precipitation is modulated by convective events that developed over the central Amazon during the preceding nighttime period. We use data collected during the Observations and Modelling of the Green Ocean Amazon (GoAmazon 2014/2015) field campaign that took place from 1 January 2014 to 30 November 2015 in the central Amazon. Local surface-based observations of cloud occurrence, soil temperature, surface fluxes, and planetary boundary layer characteristics are coupled with satellite data to identify the physical mechanisms that control the diurnal rainfall in central Amazon during the wet and dry seasons. This is accomplished through evaluation of the atmospheric properties during the nocturnal periods preceding raining and non-raining events. Comparisons between these non-raining and raining transitions are presented for the wet (January to April) and dry (June to September) seasons. The results suggest that wet-season diurnal precipitation is modulated by nighttime cloud coverage and local influences such as heating induced turbulence, whereas the dry-season rain events are controlled by large-scale circulations.

Factors Governing Cloud Growth and Entrainment Rates in Shallow Cumulus and Cumulus Congestus During GoAmazon2014/5

Abstract: Convective clouds are formed from rising air parcels, to first order driven by buoyancy and modulated by environmental stability and mixing with environmental air. Both shallow cumulus and congestus cloud types play an important role in tropical climate dynamics by distributing heat and moisture vertically (Riehl et al., 1951), and in the case of congestus providing a contribution to the net diabatic heating term proportional to their precipitation (Schumacher et al., 2008; Stachnik et al., 2013). They also can act as a precursor for deeper convection (Neggers et al., 2007) by moistening and destabilizing the stable layers that inhibit them (Mechem & Oberthaler, 2013; Riehl et al., 1951; Stevens, 2007). Despite their importance, some aspects of these clouds are not fully understood, and their contribution to tropical dynamics is not correctly represented in global climate models (GCMs) (Nam et al., 2012; Williams & Tselioudis, 2007). GCMs underestimate the sensitivity of convection to the tropospheric humidity (Derbyshire et al., 2004), including over the Amazon region (Lintner et al., 2017). As a result, shallow cumulus and congestus cloud fractions tend to be underestimated (Nam et al., 2012; Williams & Tselioudis, 2007). While there have been recent improvements (Xie et al., 2019), GCMs struggle to represent the diurnal cycle of convective precipitation correctly, by initializing and deepening convection too quickly (Del Genio & Wu, 2010; Stirling & Stratton, 2012).