Journal ArticleDOI
Measurements of Nonlinear Light Scattering
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This article is published in Physical Review Letters.The article was published on 1965-04-26. It has received 531 citations till now. The article focuses on the topics: Biological small-angle scattering & Scattering.read more
Citations
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Theory of nonlinear light scattering from phonons in crystals
Sudhanshu S. Jha,J. W. F. Woo +1 more
TL;DR: In this article, a theory of nonlinear inelastic light scattering in solids involving two incident photons, a phonon of frequency ω(in0), and the scattered photon of frequencyω3=ω1+ω2±ω0 is developed.
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Synthesis, Characterisation and Molecular Hyperpolarisabilities of Pseudo- Octahedral Hydrido(nitrile)iron(II) Complexes for Nonlinear Optics: X-ray Structure of (Fe(H)(dppe)2(4-NCC6H4NO2))(PF6)·CH2Cl2
Maria Paula Robalo,Maria Paula Robalo,António P. S. Teixeira,António P. S. Teixeira,Maria Helena Garcia,Maria Helena Garcia,M. Fátima M. Piedade,M. Fátima M. Piedade,M. Teresa Duarte,Alberto R. Dias,Jochen Campo,Wim Wenseleers,Etienne Goovaerts +12 more
TL;DR: In this article, a series of ionic pseudo-octahedral trans-hydrido(nitrile)iron(II) complexes with the general formula [Fe(H)(dppe)2(4NCR)][PF6] [dppe = 1,2-bis(diphenylphosphanyl)ethane; R = acceptor-substituted conjugated ligand] have been synthesised by chloride abstraction from the starting compound trans-[FeHCl(dppe),2] and fully characterised.
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Time‐dependent density functional theory simulation of hyper‐Raman spectra
TL;DR: In this article, a numerical finite distortion scheme was used to evaluate the first order-derivative of the dynamic first hyperpolarizability with respect to vibrational normal mode coordinates.
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Third-Harmonic Scattering for Fast and Sensitive Screening of the Second Hyperpolarizability in Solution.
TL;DR: Third-harmonic scattering (THS) is developed as an alternative method to measure γ in solution and the second hyperpolarizability |γ| of commonly used solvents is determined, which can be used as an internal calibration standard.
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Observation of Organic Molecules at the Aerosol Surface.
TL;DR: The first successful observations of molecules at the surface of laboratory-generated aerosols suspended in air using the surface-sensitive technique second harmonic light scattering (SHS) are reported.
References
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Journal ArticleDOI
Interactions between light waves in a nonlinear dielectric
TL;DR: In this paper, the induced nonlinear electric dipole and higher moments in an atomic system, irradiated simultaneously by two or three light waves, are calculated by quantum-mechanical perturbation theory.
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A theory of the depolarization of light scattered by a dense medium
A. D. Buckingham,M. J. Stephen +1 more
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Raman effect of multiple radiation process and its applications in spectroscopy
TL;DR: In this article, it was shown that with a beam intensity of 0.1 MW/sq cm, the vibrational Raman spectrum of molecules or crystals may be obtained by the three-photon process.