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Journal ArticleDOI

Single-Beam Coherent Anti-Stokes Raman Scattering Spectroscopy Using Both Pump and Soliton Stokes Pulses from a Photonic Crystal Fiber

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TLDR
In this paper, a single-beam coherent anti-Stokes Raman scattering (CARS) spectroscopy using the combination of a pulse shaper and a photonic crystal fiber (PCF) was demonstrated.
Abstract
Novel single-beam coherent anti-Stokes Raman scattering (CARS) spectroscopy using the combination of a pulse shaper and a photonic crystal fiber (PCF) was demonstrated successfully, where a fundamental soliton Stokes pulse and a spectrally compressed pump pulse were generated in the same PCF. Unlike previous single-beam CARS setups, it can probe C–H stretching vibrations from 2800 to 3100 cm-1 and the resonant Raman C–H stretching vibrations of polystyrene were successfully observed with the single-beam CARS technique.

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Citations
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Journal ArticleDOI

Compact light source for ultrabroadband coherent anti-Stoke Raman scattering (CARS) microscopy.

TL;DR: By using an assembled module, an ultrabroadband CARS spectrum and a CARS image of a murine adipocyte are observed and the module is expected to greatly spread the CARS microscopy to various fields by its extreme easiness to handle.
Journal ArticleDOI

Soliton dynamics in photonic-crystal fibers for coherent Raman microspectroscopy and microscopy

TL;DR: In this article, the authors describe various generation schemes that employ soliton dynamics in photonic-crystal fibers to generate a red-shifted femtosecond pulse with high efficiency.
Journal ArticleDOI

Compact and fully collinear light source for broadband multiplex CARS microscopy covering the fingerprint region.

TL;DR: Compact and fully collinear light source for multiplex coherent anti-Stokes Raman scattering (CARS) microscopy was proposed and demonstrated and has great potential to expand the utility of CARS microscopy to a wide variety of fields such as endoscopy.
Book ChapterDOI

Optical Solitons from a Photonic Crystal Fiber and Their Applications

TL;DR: In this paper, a photonic crystal fiber (PCF) is used to generate ultrabroadband optical pulses by propagating femtosecond optical pulses in these fibers, and the properties of the fundamental solitons from a PCF and its applications studied in our laboratory.
Patent

Optical analysis device and biomolecular analysis device

TL;DR: In this paper, a multicolumn CARS light is generated from, a sample by using a residual component of the pump light introduced to an optical waveguide and the Stokes light generated in an OWG.
References
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Genetic Algorithms

Journal ArticleDOI

Theory of the soliton self-frequency shift.

TL;DR: The theory of Raman effects, which causes a continuous downshift of the mean frequency of pulses propagating in optical fibers, agrees well with recent measurements.
Journal ArticleDOI

Coherent Anti-Stokes Raman Scattering Microscopy: Instrumentation, Theory, and Applications

TL;DR: Coherent anti-Stokes Raman scattering (CARS) microscopy permits vibrational imaging with high-sensitivity, high speed, and three-dimensional spatial resolution as discussed by the authors, and the development of multiplex CARS microspectroscopy, which allows high-speed characterization of microscopic samples.
Journal ArticleDOI

Single-pulse coherently controlled nonlinear Raman spectroscopy and microscopy

TL;DR: This work performs single-pulse vibrational spectroscopy on several molecules in the liquid phase, where both the excitation and the readout processes are performed by the same pulse, using a single broadband laser source.
Journal ArticleDOI

Coherent anti-Stokes Raman Scattering Microscopy

TL;DR: Results show that CARS microscopy has the potential to become an important complementary technique that can be used with other well-established microscopic methods, and it can be expected that the impressive growth of the field will continue.
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