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Theory for nonlinear Mie-scattering from spherical metal clusters

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TLDR
In this paper, the angular dependence of light intensities radiated in second and third harmonic generation by spherical metal clusters is analyzed in detail, and resonance effects in the integrated intensities are studied.
Abstract
Using classical electrodynamics we determine the angular dependence of the light intensities radiated in second and third harmonic generation by spherical metal clusters. Forward and backward scattering is analyzed in detail. Also resonance effects in the integrated intensities are studied. By treating intermediate cluster sizes, we complete the scattering theory for spherical clusters between Rayleigh-type analysis for small spheres and geometrical optics for spheres much larger than the wavelength for nonlinear optics. The particle size sensitivity of Mie-scattering is increased by nonlinearity. The results suggest that small particle sizes can be extracted more easily from nonlinear optics.

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Journal ArticleDOI

Multipolar nonlinear nanophotonics

TL;DR: In this paper, the authors review the advances in the recently emerged field of multipolar nonlinear nanophotonics, starting from earlier relevant studies of metallic and metal-dielectric structures supporting localized plasmonic resonances, and then discussing the latest results for all- dielectric nanostructures driven by Mie-type multipolar resonances and optically induced magnetic response.
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Theory of optical second-harmonic generation from a sphere of centrosymmetric material: Small-particle limit

TL;DR: In this paper, the electromagnetic theory of optical second-harmonic generation from small spherical particles comprised of centrosymmetric material is presented, where the interfacial region where the inversion symmetry is broken provides a source of the nonlinearity.
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Nonlinear Light Scattering and Spectroscopy of Particles and Droplets in Liquids

TL;DR: Recent developments of nonlinear light scattering techniques have resulted in a deeper insight of the underlying light-matter interactions and shed new light on the molecular mechanism of surface kinetics in solution, properties of interfacial water in contact with hydrophilic and hydrophobic particles and droplets, and vesicle structure and transport properties.
Journal ArticleDOI

Boundary element method for surface nonlinear optics of nanoparticles

TL;DR: The frequency-domain boundary element formulation for solving surface second-harmonic generation from nanoparticles of virtually arbitrary shape and material uses the Rao-Wilton-Glisson basis functions and Galerkin's testing, which leads to very accurate solutions for both near and far fields.
Journal ArticleDOI

Free-electron Optical Nonlinearities in Plasmonic Nanostructures: A Review of the Hydrodynamic Description

TL;DR: In this paper, a review of free-carrier nonlinearities in the hydrodynamic description in both perturbative and non-perturbative regimes, considering also contribution of nonlocal effects is presented.
References
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Book

Classical Electrodynamics

Book

Principles of Optics

Max Born, +1 more
TL;DR: In this paper, the authors discuss various topics about optics, such as geometrical theories, image forming instruments, and optics of metals and crystals, including interference, interferometers, and diffraction.
Book

Absorption and Scattering of Light by Small Particles

TL;DR: In this paper, a Potpourri of Particles is used to describe surface modes in small Particles and the Angular Dependence of Scattering is shown to be a function of the size of the particles.
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