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Showing papers by "Junsuk Rho published in 2022"


Journal ArticleDOI
10 Jan 2022-eLight
TL;DR: Hyperbolic metamaterials have an extremely high anisotropy with a hyperbolic dispersion relation and exhibit a high density of states which have been exploited in various applications, such as super-resolution imaging, negative refraction, and enhanced emission control as mentioned in this paper .
Abstract: Abstract Optical metamaterials have presented an innovative method of manipulating light. Hyperbolic metamaterials have an extremely high anisotropy with a hyperbolic dispersion relation. They are able to support high- k modes and exhibit a high density of states which produce distinctive properties that have been exploited in various applications, such as super-resolution imaging, negative refraction, and enhanced emission control. Here, state-of-the-art hyperbolic metamaterials are reviewed, starting from the fundamental principles to applications of artificially structured hyperbolic media to suggest ways to fuse natural two-dimensional hyperbolic materials. The review concludes by indicating the current challenges and our vision for future applications of hyperbolic metamaterials.

147 citations


Journal ArticleDOI
TL;DR: In this paper , a simple asymmetric spin-orbit interaction (SOI)-based technique is realized for multifunctional metaoptics, employing only a single unit cell, breaking the conventional tradeoff between design complexity and efficient asymmetric transmission efficiency.
Abstract: Symmetric spin–orbit interaction (SOI)‐based approaches apply a practical limit on helicity multiplexed metaoptics, i.e., center symmetric information encoding. Contrarily, asymmetric SOI's based on the combination of geometric and propagation phase‐delay approaches can effectively address such limitations for multifunctional multiplexed metaoptics on the cost of design complexities. In this paper, a simple asymmetric SOI‐based technique is realized for multifunctional metaoptics, employing only a single unit cell, breaking the conventional tradeoff between design complexity and efficient asymmetric transmission efficiency. The design approach depends on geometric phase alone, which eases the fabrication challenges and decreases the computational cost associated with previous asymmetric SOI‐based metaoptics. Furthermore, this study utilizes a new, low‐cost CMOS‐compatible material to optimize the proposed single unit cell for low loss and high transmission efficiency over the complete visible domain. On‐axis and off‐axis holographic metasurfaces are designed and integrated with pressure‐sensitive liquid crystal cells to demonstrate actively tunable metaholography with no limitation of center symmetric information encoding. The simple design technique, cost‐effective fabrication, and finger touch‐enabled holographic output switching make this integrated setup a potential candidate for many applications such as smart safety labeling, motion or touch recognition, and interactive displays for impact monitoring of precious artworks and products.

66 citations


Journal ArticleDOI
19 Feb 2022-ACS Nano
TL;DR: In this article , a dual-band vectorial metahologram in the visible and ultraviolet (UV) regimes for optical encryption was proposed. But the proposed scheme is limited to the use of a pixelated metasurface.
Abstract: Metasurface-driven optical encryption devices have attracted much attention. Here, we propose a dual-band vectorial metahologram in the visible and ultraviolet (UV) regimes for optical encryption. Nine polarization-encoded vectorial holograms are observed under UV laser illumination, while another independent hologram appears under visible laser illumination. The proposed engineered silicon nitride, which is transparent in UV, is employed to demonstrate the UV hologram. Nine holographic images for different polarization states are encoded using a pixelated metasurface. The dual-band metahologram is experimentally implemented by stacking the individual metasurfaces that operate in the UV and visible. The visible hologram can be decrypted to provide the first key, a polarization state, which is used to decode the password hidden in the UV vectorial hologram through the use of an analyzer. Considering the property of UV to be invisible to the naked eye, the multiple polarization channels of the vectorial hologram, and the dual-band decoupling, the demonstrated dual-band vectorial hologram device could be applied in various high-security and anticounterfeiting applications.

61 citations


Journal ArticleDOI
TL;DR: In this paper , an electrically tunable metasurface that can represent saturated red, green, and blue pixels that can be dynamically and continuously controlled between on and off states using liquid crystals is presented.
Abstract: Abstract Taking inspiration from beautiful colors in nature, structural colors produced from nanostructured metasurfaces have shown great promise as a platform for bright, highly saturated, and high-resolution colors. Both plasmonic and dielectric materials have been employed to produce static colors that fulfil the required criteria for high-performance color printing, however, for practical applications in dynamic situations, a form of tunability is desirable. Combinations of the additive color palette of red, green, and blue enable the expression of further colors beyond the three primary colors, while the simultaneous intensity modulation allows access to the full color gamut. Here, we demonstrate an electrically tunable metasurface that can represent saturated red, green, and blue pixels that can be dynamically and continuously controlled between on and off states using liquid crystals. We use this to experimentally realize ultrahigh-resolution color printing, active multicolor cryptographic applications, and tunable pixels toward high-performance full-color reflective displays.

51 citations


Journal ArticleDOI
TL;DR: In this article , a wideband thermophotovoltaics (STPV) system consisting of an absorber and an emitter pair achieving high absorptance of solar radiation within the range of 400-1500 nm (covering the visible and infrared regions), whereas the emitter achieves an emittance of >95% at a wavelength of 2.3 μm.
Abstract: The efficiency of traditional solar cells is constrained due to the Shockley-Queisser limit, to circumvent this theoretical limit, the concept of solar thermophotovoltaics (STPVs) has been introduced. The typical design of an STPV system consists of a wideband absorber with its front side facing the sun. The back of this absorber is physically attached to the back of a selective emitter facing a low-bandgap photovoltaic (PV) cell. We demonstrate an STPV system consisting of a wideband absorber and emitter pair achieving a high absorptance of solar radiation within the range of 400-1500 nm (covering the visible and infrared regions), whereas the emitter achieves an emittance of >95% at a wavelength of 2.3 μm. This wavelength corresponds to the bandgap energy of InGaAsSb (0.54 eV), which is the targeted PV cell technology for our STPV system design. The material used for both the absorber and the emitter is chromium due to its high melting temperature of 2200 K. An absorber and emitter pair is also fabricated and the measured results are in agreement with the simulated results. The design achieves an overall solar-to-electrical simulated efficiency of 21% at a moderate temperature of 1573 K with a solar concentration of 3000 suns. Furthermore, an efficiency of 15% can be achieved at a low temperature of 873 K with a solar concentration of 500 suns. The designs are also insensitive to polarization and show negligible degradation in solar absorptance and thermal emittance with a change in the angle of incidence.

49 citations


Journal ArticleDOI
TL;DR: In this paper , an electrically tunable metasurface that can represent saturated red, green, and blue pixels that can be dynamically and continuously controlled between on and off states using liquid crystals is presented.
Abstract: Abstract Taking inspiration from beautiful colors in nature, structural colors produced from nanostructured metasurfaces have shown great promise as a platform for bright, highly saturated, and high-resolution colors. Both plasmonic and dielectric materials have been employed to produce static colors that fulfil the required criteria for high-performance color printing, however, for practical applications in dynamic situations, a form of tunability is desirable. Combinations of the additive color palette of red, green, and blue enable the expression of further colors beyond the three primary colors, while the simultaneous intensity modulation allows access to the full color gamut. Here, we demonstrate an electrically tunable metasurface that can represent saturated red, green, and blue pixels that can be dynamically and continuously controlled between on and off states using liquid crystals. We use this to experimentally realize ultrahigh-resolution color printing, active multicolor cryptographic applications, and tunable pixels toward high-performance full-color reflective displays.

45 citations


Journal ArticleDOI
TL;DR: In this paper , the authors proposed an ultrafast and full-color colorimetric humidity sensor that consists of chitosan hydrogel sandwiched by a disordered metal nanoparticle layer and reflecting substrate.
Abstract: The development of real-time and sensitive humidity sensors is in great demand from smart home automation and modern public health. We hereby proposed an ultrafast and full-color colorimetric humidity sensor that consists of chitosan hydrogel sandwiched by a disordered metal nanoparticle layer and reflecting substrate. This hydrogel-based resonator changes its resonant frequency to external humidity conditions because the chitosan hydrogels are swollen under wet state and contracted under dry state. The response time of the sensor is ~104 faster than that of the conventional Fabry-Pérot design. The origins of fast gas permeation are membrane pores created by gaps between the metal nanoparticles. Such instantaneous and tunable response of a new hydrogel resonator is then exploited for colorimetric sensors, anti-counterfeiting applications, and high-resolution displays.

45 citations


Journal ArticleDOI
TL;DR: In this paper , a geometric phase-enabled novel design strategy is proposed to break the conventional trade-off between polarization-insensitivity and bandwidth, which ensures the realization of broad-band polarization sensitivity through a simplified design procedure.
Abstract: The remarkable potential of metasurface holography promises revolutionary advancements for imaging, chip-integrated augmented/virtual reality (AR/VR) technology, and flat optical displays. The choice of constituent element geometry constrains many potential applications purveyed through polarization-independent optical response. The limited capabilities and degree of freedoms in commonly used meta-atoms restrict the design flexibility to break the conventional trade-off between polarization-insensitivity and bandwidth. Here, we propose a geometric phase-enabled novel design strategy to break this conventional trade-off. The proposed strategy ensures the realization of broad-band polarization-insensitivity through a simplified design procedure. An identical output wavefront manipulation is achieved by adjusting the phase delay freedom of geometric phase engineering under different incident polarization conditions. For proof of concept, a metahologram device is fabricated by an optimized complementary metal-oxide-semiconductor (CMOS)-compatible material of hydrogenated amorphous silicon (a-Si:H). This metahologram device reproduces the required hologram with high image fidelity and efficiency under different polarization scenarios of white light incidence. Due to the simple design strategy, low computational cost, and easy fabrication, the proposed technique can be an excellent candidate for realizing polarization-insensitive metahologram devices.

42 citations


Journal ArticleDOI
TL;DR: In this article , a broad-band polarization-insensitive flexible metasurface for the security of sensitive packages in the transport industry is proposed, which employs both the propagation and the geometric phase of novel TiO2 resin-based anisotropic nanoresonators.
Abstract: Secure packaging and transportation of light-sensitive chemical and biomedical test tubes are crucial for environmental protection and public health. Benefiting from the compact form factor and high efficiency of optical metasurfaces, we propose a broad-band polarization-insensitive flexible metasurface for the security of sensitive packages in the transport industry. We employ both the propagation and the geometric phase of novel TiO2 resin-based anisotropic nanoresonators to demonstrate a flexible and broad-band polarization-insensitive metasurface in the visible domain. The ultraviolet nanoimprint lithographic technique (UV-NIL) is used to fabricate high-index TiO2 nanoparticle-embedded-resin (nano-PER) structures that are patterned on a flexible substrate. This novel approach provides swift single-step fabrication without secondary fabrication steps such as deposition and etching. Moreover, replicating and transforming patterns over flexible substrates make the proposed technique highly suitable for large-throughput commercial manufacturing. As the proposed metahologram manifests high transmission efficiency in the visible domain, such flexible metaholographic platforms could find several exciting applications in bendable/curved displays, wearable devices, and holographic labeling for interactive displays.

40 citations


Journal ArticleDOI
TL;DR: In this paper , a planar all-dielectric metasurface is proposed incorporating extra degrees of freedom to comprehend the conversion of amplitude, polarization, and phase with broadband chiro-optical effects in terms of giant asymmetric transmission with maximum efficiency of ≈77% at the wavelength of 567 nm.
Abstract: Futuristic holographic displays will essentially require broadband chiro‐optical effects for medical imaging, virtual reality, smart security, and optical encryption. However, conventional metasurfaces cannot provide such on‐chip realization of broadband chiro‐optical effects. Moreover, the simultaneous conversion of amplitude, polarization, and phase (APP) at optical wavelengths to introduce giant chirality has not been realized yet. In this paper, a planar all‐dielectric metasurface is proposed incorporating extra degrees of freedom to comprehend the conversion of APP with broadband chiro‐optical effects in terms of giant asymmetric transmission with maximum efficiency of ≈77% at the wavelength of 567 nm. The underlying mechanism behind induced chiro‐optical effects is also investigated using higher‐order multipolar dielectric resonances. Moreover, experimental validation is performed using the reproduced polarization‐encrypted meta‐holograms at broadband visible wavelengths. This work expands the scope of meta‐nanophotonics with potential applications in bioimaging and polarization‐encrypted displays for healthcare and smart security applications.

36 citations


Journal ArticleDOI
TL;DR: In this paper , the authors review the recent progress in optical metasurface-based OVs and provide a comprehensive discussion on the optical manipulation of OVs, including OAM superposition, OAM sorting and OAM multiplexing.
Abstract: Abstract Optical vortices (OVs) carrying orbital angular momentum (OAM) have attracted considerable interest in the field of optics and photonics owing to their peculiar optical features and extra degree of freedom for carrying information. Although there have been significant efforts to realize OVs using conventional optics, it is limited by large volume, high cost, and lack of design flexibility. Optical metasurfaces have recently attracted tremendous interest due to their unprecedented capability in the manipulation of the amplitude, phase, polarization, and frequency of light at a subwavelength scale. Optical metasurfaces have revolutionized design concepts in photonics, providing a new platform to develop ultrathin optical devices for the realization of OVs at subwavelength resolution. In this article, we will review the recent progress in optical metasurface-based OVs. We provide a comprehensive discussion on the optical manipulation of OVs, including OAM superposition, OAM sorting, OAM multiplexing, OAM holography, and nonlinear metasurfaces for OAM generation and manipulation. The rapid development of metasurface for OVs generation and manipulation will play an important role in many relevant research fields. We expect that metasurface will fuel the continuous progress of wearable and portable consumer electronics and optics where low-cost and miniaturized OAM related systems are in high demand.

Journal ArticleDOI
TL;DR: In this paper , a 3D achromatic diffractive metalens on the end face of a single-mode fiber was designed and nanoprinted to perform in-focus focusing across the entire near-infrared telecommunication wavelength band ranging from 1.25 to 1.65 µm.
Abstract: Abstract Dispersion engineering is essential to the performance of most modern optical systems including fiber-optic devices. Even though the chromatic dispersion of a meter-scale single-mode fiber used for endoscopic applications is negligible, optical lenses located on the fiber end face for optical focusing and imaging suffer from strong chromatic aberration. Here we present the design and nanoprinting of a 3D achromatic diffractive metalens on the end face of a single-mode fiber, capable of performing achromatic and polarization-insensitive focusing across the entire near-infrared telecommunication wavelength band ranging from 1.25 to 1.65 µm. This represents the whole single-mode domain of commercially used fibers. The unlocked height degree of freedom in a 3D nanopillar meta-atom largely increases the upper bound of the time-bandwidth product of an achromatic metalens up to 21.34, leading to a wide group delay modulation range spanning from −8 to 14 fs. Furthermore, we demonstrate the use of our compact and flexible achromatic metafiber for fiber-optic confocal imaging, capable of creating in-focus sharp images under broadband light illumination. These results may unleash the full potential of fiber meta-optics for widespread applications including hyperspectral endoscopic imaging, femtosecond laser-assisted treatment, deep tissue imaging, wavelength-multiplexing fiber-optic communications, fiber sensing, and fiber lasers.

Peer ReviewDOI
TL;DR: In this paper , the authors present the recent progress on tunable metasurfaces focused on metalenses and metaholograms, including the basic working principles, advantages, and disadvantages of each working mechanism.
Abstract: Abstract. Metasurfaces have attracted great attention due to their ability to manipulate the phase, amplitude, and polarization of light in a compact form. Tunable metasurfaces have been investigated recently through the integration with mechanically moving components and electrically tunable elements. Two interesting applications, in particular, are to vary the focal point of metalenses and to switch between holographic images. We present the recent progress on tunable metasurfaces focused on metalenses and metaholograms, including the basic working principles, advantages, and disadvantages of each working mechanism. We classify the tunable stimuli based on the light source and electrical bias, as well as others such as thermal and mechanical modulation. We conclude by summarizing the recent progress of metalenses and metaholograms, and providing our perspectives for the further development of tunable metasurfaces.

Journal ArticleDOI
TL;DR: In this paper , an approach to attain the large and efficient spin Hall effect of light with high efficiency in the near-infrared was proposed and experimentally demonstrated at 800 nm by using a dielectric metasurface.
Abstract: The spin Hall effect of light refers to a spin-dependent transverse splitting of light at a planar interface. Previous demonstrations to enhance the splitting have suffered from exceedingly low efficiency. Achievements of the large splitting with high efficiency have been reported in the microwave, but those in the optical regime remain elusive. Here, an approach to attain the large splitting with high efficiency in the near-infrared is proposed and experimentally demonstrated at 800 nm by using a dielectric metasurface. Modulation of the complex transmission of the metasurface leads to the shifts that reach 10λ along with efficiencies over 70% under two linear polarizations. Our work extends the recent attempts to achieve the large and efficient spin Hall effect of light, which have been limited only to the microwave, to the optical regime.

Journal ArticleDOI
TL;DR: In this article , an approach to attain the large and efficient spin Hall effect of light with high efficiency in the near-infrared was proposed and experimentally demonstrated at 800 nm by using a dielectric metasurface.
Abstract: The spin Hall effect of light refers to a spin-dependent transverse splitting of light at a planar interface. Previous demonstrations to enhance the splitting have suffered from exceedingly low efficiency. Achievements of the large splitting with high efficiency have been reported in the microwave, but those in the optical regime remain elusive. Here, an approach to attain the large splitting with high efficiency in the near-infrared is proposed and experimentally demonstrated at 800 nm by using a dielectric metasurface. Modulation of the complex transmission of the metasurface leads to the shifts that reach 10λ along with efficiencies over 70% under two linear polarizations. Our work extends the recent attempts to achieve the large and efficient spin Hall effect of light, which have been limited only to the microwave, to the optical regime.

Journal ArticleDOI
TL;DR: A single meta-nanoresonator-based tri-functional metasurface is proposed by combining the geometric phase-based spin-decoupling and Malus's law intensity modulation to improve information capacity and opens new avenues in multi-functional meta-devices design.
Abstract: Multi‐functional metasurfaces have attracted great attention due to the significant possibilities to realize highly integrated and ultra‐compact meta‐devices. Merging nano‐printing and holographic information multiplexing is one of the effective ways to achieve multi‐functionality, and such a merger can increase the information encoding capacity. However, the current approaches rely on stacking layers and interleaving, where multiple resonators effectively combine different functionalities on the cost of efficiency, design complexity, and challenging fabrication. To address such challenges, a single meta‐nanoresonator‐based tri‐functional metasurface is proposed by combining the geometric phase‐based spin‐decoupling and Malus's law intensity modulation. The proposed strategy effectively improves information capacity owing to the orientation degeneracy of spin‐decoupling rather than layer stacking or super‐cell designs. To validate the proposed strategy, a metasurface demonstrating two helicity‐dependent holographic outputs is presented in far‐field, whereas a continuous nano‐printing image is in near‐field. It is also employed on CMOS‐compatible and cost‐effective hydrogen amorphous silicon providing transparent responses for the whole visible band. As a result, the proposed metasurface has high transmission efficiency in the visible regime and verifies the design strategy without adding extra complexities to conventional nano‐pillar geometry. Therefore, the proposed metasurface opens new avenues in multi‐functional meta‐devices design and has promising applications in anti‐counterfeiting, optical storage and displays.

Journal ArticleDOI
TL;DR: In this article , the authors describe novel metasurfaces-based nanophotonic platforms that have shown exceptional control of electromagnetic waves at the subwavelength scale as promising candidates to overcome existing restrictions, while realizing flat optical devices.
Abstract: The holographic display, one of the most realistic ways to reconstruct optical images in three-dimensional (3D) space, has gained a lot of attention as a next-generation display platform for providing deeper immersive experiences to users. So far, diffractive optical elements (DOEs) and spatial light modulators (SLMs) have been used to generate holographic images by modulating electromagnetic waves at each pixel. However, such architectures suffer from limitations in terms of having a resolution of only a few microns and the bulkiness of the entire optical system. In this review, we describe novel metasurfaces-based nanophotonic platforms that have shown exceptional control of electromagnetic waves at the subwavelength scale as promising candidates to overcome existing restrictions, while realizing flat optical devices. After introducing the fundamentals of metasurfaces in terms of spatial and spectral wavefront modulation, we present a variety of multiplexing approaches for high-capacity and full-color metaholograms exploiting the multiple properties of light as an information carrier. We then review tunable metaholograms using active materials modulated by several external stimuli. Afterward, we discuss the integration of metasurfaces with other optical elements required for future 3D display platforms in augmented/virtual reality (AR/VR) displays such as lenses, beam splitters, diffusers, and eye-tracking sensors. Finally, we address the challenges of conventional nanofabrication methods and introduce scalable preparation techniques that can be applied to metasurface-based nanophotonic technologies towards commercially and ergonomically viable future holographic displays.

Journal ArticleDOI
TL;DR: In this article , the authors proposed a metasurface-enhanced SL-based depth-sensing platform that scatters high-density ~10 K dot array over the 180° FOV by manipulating light at subwavelength-scale.
Abstract: Abstract Structured light (SL)-based depth-sensing technology illuminates the objects with an array of dots, and backscattered light is monitored to extract three-dimensional information. Conventionally, diffractive optical elements have been used to form laser dot array, however, the field-of-view (FOV) and diffraction efficiency are limited due to their micron-scale pixel size. Here, we propose a metasurface-enhanced SL-based depth-sensing platform that scatters high-density ~10 K dot array over the 180° FOV by manipulating light at subwavelength-scale. As a proof-of-concept, we place face masks one on the beam axis and the other 50° apart from axis within distance of 1 m and estimate the depth information using a stereo matching algorithm. Furthermore, we demonstrate the replication of the metasurface using the nanoparticle-embedded-resin (nano-PER) imprinting method which enables high-throughput manufacturing of the metasurfaces on any arbitrary substrates. Such a full-space diffractive metasurface may afford ultra-compact depth perception platform for face recognition and automotive robot vision applications.

Journal ArticleDOI
TL;DR: In this paper , an explicit analytic formula for the spin Hall shift is derived under arbitrarily polarized incidence, and it is shown that the spin-hall shift can be enhanced at any incident angle by using polarization degree of freedom and independent of the Fresnel coefficients of an interface under circularly polarized light.
Abstract: Abstract The spin Hall effect of light (SHEL) is the microscopic spin-dependent splitting of light at an optical interface. Whereas the spin Hall shift under linearly polarized light is well-formulated, studies on the SHEL under elliptically or circularly polarized light have primarily relied on numerical computation. In this work, an explicit analytic formula for the spin Hall shift is derived under arbitrarily polarized incidence. Furthermore, from this explicit expression, we demonstrate that the spin Hall shift can be enhanced at any incident angle by using polarization degree of freedom and is independent of the Fresnel coefficients of an interface under circularly polarized light. The analytic formula will help us understand the SHEL under general polarization intuitively and realize unprecedented modulation of the SHEL.

Journal ArticleDOI
TL;DR: In this paper , the fundamental principles and practical design procedures to exploit the abilities of metalenses, including achromaticity, high numerical aperture, and tunability, are presented, along with a practical guide for the design, fabrication, and critical considerations of metalense with examples of early works to more recent developments.
Abstract: Metalenses comprised of artificial subwavelength structures known as meta-atoms have demonstrated abilities beyond conventional bulky optical components by modulating the phase, amplitude, and polarization of light in an ultrathin planar form factor. In this Tutorial, we present the fundamental principles and practical design procedures to exploit the abilities of metalenses, including achromaticity, high numerical aperture, and tunability. The fundamental principles include both plasmonic and dielectric meta-atoms, which require different physics to describe their light–matter interactions. In the phase modulation section, we compare the methods of physically implementing phase via meta-atoms including both the propagation and geometric phase methods. Next, we cover the recent progress of nanofabrication procedures from the perspective of the metalenses using materials such as titanium dioxide, gallium nitride, and hydrogenated amorphous silicon. We further compare the various fabrication methods with regard to the resolution, size, cost, and optical properties of fabricated metalenses. Then, we describe the critical considerations of metalenses including aberration-correction, numerical aperture, and tunability for advanced flat optics. Herein, we provide a practical guide for the design, fabrication, and critical considerations of metalenses with examples of research from early works to more recent developments.

Journal ArticleDOI
TL;DR: In this article , humidity-tunable nano pixels are investigated with a 700 nm resolution that demonstrates full standard RGB (sRGB) gamut coverage with a millisecond response time.
Abstract: Humidity‐responsive structural coloration is actively investigated to realize real‐time humidity sensors for applications in smart farming, food storage, and healthcare management. Here, humidity‐tunable nano pixels are investigated with a 700 nm resolution that demonstrates full standard RGB (sRGB) gamut coverage with a millisecond‐response time. The color pixels are designed as Fabry–Pérot (F–P) etalons which consist of an aluminum mirror substrate, humidity‐responsive polyvinyl alcohol (PVA) spacer, and a top layer of disordered silver nanoparticles (NPs). The measured volume change of the PVA reaches up to 62.5% when the relative humidity (RH) is manipulated from 20 to 90%. The disordered silver NP layer permits the penetration of water molecules into the PVA layer, enhancing the speed of absorption and swelling down to the millisecond level. Based on the real‐time response of the hydrogel‐based F–P etalons with a high‐throughput 3D nanoimprint technique, a high‐resolution multicolored color print that can have potential applications in display technologies and optical encryption, is demonstrated.

Journal ArticleDOI
TL;DR: In this article , various metasurface design strategies are reviewed thoroughly, including phase map retrieval and meta-atom unit-cell design for light modulation with subwavelength thickness.
Abstract: Over the last two decades, the capabilities of metasurfaces in light modulation with subwavelength thickness have been proven, and metasurfaces are expected to miniaturize conventional optical components and add various functionalities. In this review article, various metasurface design strategies are reviewed thoroughly. First, we revisit the scalar diffraction theory to provide the basic principle of light propagation. Then, we discuss widely used design methods based on the unit-cell approach. The methods include a set of simplified steps, including the phase map retrieval and meta-atom unit-cell design. Then, we introduce recently emerging metasurfaces that may not be accurately designed using unit-cell approach. We examine unconventional metasurfaces where the conventional design methods fail and finally discuss potential design methods for such metasurfaces. This article is protected by copyright. All rights reserved.

Journal ArticleDOI
TL;DR: In this article , the chirality of chiral L-handed helicoid-III nanoparticles is quantified by means of an asymmetric factor, the so-called g-factor.
Abstract: While plasmonic particles can provide optical resonances in a wide spectral range from the lower visible up to the near-infrared, often, symmetry effects are utilized to obtain particular optical responses. By breaking certain spatial symmetries, chiral structures arise and provide robust chiroptical responses to these plasmonic resonances. Here, we observe strong chiroptical responses in the linear and nonlinear optical regime for chiral L-handed helicoid-III nanoparticles and quantify them by means of an asymmetric factor, the so-called g-factor. We calculate the linear optical g-factors for two distinct chiroptical resonances to −0.12 and –0.43 and the nonlinear optical g-factors to −1.45 and −1.63. The results demonstrate that the chirality of the helicoid-III nanoparticles is strongly enhanced in the nonlinear regime.

Journal ArticleDOI
TL;DR: The spin Hall effect of light (SHEL) as mentioned in this paper is the microscopic splitting of light into two circular polarizations at the optical interface along the perpendicular direction, and it has been garnering significant scientific interest.
Abstract: The spin Hall effect of light (SHEL) is the microscopic splitting of light into two circular polarizations at the optical interface along the perpendicular direction. With the advent of metamaterials/metasurfaces and their fast‐developing applications, the SHEL has been garnering significant scientific interest. Here, the principle and recent developments in SHEL research is reviewed. A theoretical description of the SHEL is provided, including the formalism and general techniques. Also, recent studies on and applications of the SHEL are extensively reviewed, including the enhancement of the spin Hall shift and efficiency, implementation of dynamic tunability, elimination of polarization dependence, and precision measurements. The review is concluded with a discussion on the future direction and prospects of the SHEL.

Journal ArticleDOI
TL;DR: Large-scale multilevel tunable absorbers realized with nanoparticle-based solution fabrication techniques are expected to open the way for advanced thermo-optical cryptographic devices based on tunable reflective coloration and near-infrared absorption.
Abstract: Reconfigurable light absorbers have attracted much attention by providing additional optical responses and expanding the number of degrees of freedom in security applications. Fabry-Pèrot absorbers based on phase change materials with tunable properties can be implemented over large scales without the need for additional steps such as lithography, while exhibiting reconfigurable optical responses. However, a fundamental limitation of widely used phase change materials such as vanadium dioxide and germanium-antimony-tellurium-based chalcogenide glasses is that they have only two distinct phases; therefore, only two different states of optical properties are available. Here, we experimentally demonstrate active multilevel absorbers that are tuned by controlling the external temperature. This is produced by creating large-scale lithography-free multilayer structures with both undoped and tungsten-doped solution-processed monoclinic-phase vanadium dioxide thin films. The doping of vanadium dioxide with tungsten allows for the modulation of the phase-transition temperature, which results in an extra degree of freedom and therefore an additional step for the tunable properties. The proposed multilevel absorber is designed and characterized both numerically and experimentally. Such large-scale multilevel tunable absorbers realized with nanoparticle-based solution fabrication techniques are expected to open the way for advanced thermo-optical cryptographic devices based on tunable reflective coloration and near-infrared absorption.

Journal ArticleDOI
TL;DR: In this article , a metahologram is designed and fabricated using a nanocomposite, which exhibits conversion efficiencies of 48% and 35% at wavelengths of 532 and 635 nm, respectively.
Abstract: Metasurfaces consisting of artificially designed meta-atoms have been popularized recently due to their advantages of amplitude and phase of light control. However, the electron beam lithography method for metasurface fabrication has high cost and low throughput, which results in a limitation for the fabrication of metasurfaces. In this study, nanocomposite printing technology is used to fabricate high-efficiency metasurfaces with low cost. To demonstrate the efficiency of the proposed fabrication method, a metahologram is designed and fabricated using a nanocomposite. The metahologram exhibits conversion efficiencies of 48% and 35% at wavelengths of 532 and 635 nm, respectively. The nanocomposite is composed of polymers with nanoparticles, so durability tests are also performed to evaluate the effects of temperature and humidity on the metasurfaces. The test verifies that at temperatures below the glass transition temperature of the base resin, the nanostructures do not collapse, so the efficiency of the metasurfaces remains almost the same. The surrounding humidity does not affect the nanostructures at all. Hence, the durability of the nanocomposite metasurfaces can be further enhanced by replacing the base resin, and this nanocomposite printing method will facilitate practical metasurface use at low cost.

Journal ArticleDOI
TL;DR: In this article , an inverse design method based on gradient-descent optimization is presented to encode multiple pieces of holographic information into a single metasurface, which allows the inverse design of singlecell meta-atom design strategies, facilitating high-throughput fabrication using broadband low-loss materials.
Abstract: Metasurface‐generated holography has emerged as a promising route for fully reproducing vivid scenes by manipulating the optical properties of light using ultra‐compact devices. However, achieving multiple holographic images using a single metasurface is still difficult due to the capacity limit of a single meta‐atom. In this work, an inverse design method based on gradient‐descent optimization is presented to encode multiple pieces of holographic information into a single metasurface. The proposed method allows the inverse design of single‐cell metasurfaces without the need for complex meta‐atom design strategies, facilitating high‐throughput fabrication using broadband low‐loss materials. By exploiting the proposed design method, both multiplane red‐green‐blue (RGB) color and three‐dimensional (3D) holograms are designed and experimentally demonstrated. Multiplane RGB color holograms with nine distinct holograms are achieved, which demonstrate the state‐of‐the‐art data capacity of a phase‐only metasurface. The first experimental demonstration of metasurface‐generated 3D holograms with completely independent and distinct images in each plane is also presented. The current research findings provide a viable route for practical metasurface‐generated holography by demonstrating the high‐density holography produced by a single metasurface. It is expected to ultimately lead to optical storage, display, and full‐color imaging applications.

Journal ArticleDOI
TL;DR: In this paper , the authors presented a novel strategy for realizing heterogeneous structures that enable efficient near-field coupling between the plasmonic modes of gold nanoparticles and various other nanomaterials via a simple three-dimensional coassembly process.
Abstract: Plasmonic nanoparticle clusters promise to support unique engineered electromagnetic responses at optical frequencies, realizing a new concept of devices for nanophotonic applications. However, the technological challenges associated with the fabrication of three-dimensional nanoparticle clusters with programmed compositions remain unresolved. Here, we present a novel strategy for realizing heterogeneous structures that enable efficient near-field coupling between the plasmonic modes of gold nanoparticles and various other nanomaterials via a simple three-dimensional coassembly process. Quantum dots embedded in the plasmonic structures display ∼56 meV of a blue shift in the emission spectrum. The decay enhancement factor increases as the total contribution of radiative and nonradiative plasmonic modes increases. Furthermore, we demonstrate an ultracompact diagnostic platform to detect M13 viruses and their mutations from femtoliter volume, sub-100 pM analytes. This platform could pave the way toward an effective diagnosis of diverse pathogens, which is in high demand for handling pandemic situations.

Journal ArticleDOI
TL;DR: In this article , a metahologram is designed and fabricated using a nanocomposite, which exhibits conversion efficiencies of 48% and 35% at wavelengths of 532 and 635 nm, respectively.
Abstract: Metasurfaces consisting of artificially designed meta-atoms have been popularized recently due to their advantages of amplitude and phase of light control. However, the electron beam lithography method for metasurface fabrication has high cost and low throughput, which results in a limitation for the fabrication of metasurfaces. In this study, nanocomposite printing technology is used to fabricate high-efficiency metasurfaces with low cost. To demonstrate the efficiency of the proposed fabrication method, a metahologram is designed and fabricated using a nanocomposite. The metahologram exhibits conversion efficiencies of 48% and 35% at wavelengths of 532 and 635 nm, respectively. The nanocomposite is composed of polymers with nanoparticles, so durability tests are also performed to evaluate the effects of temperature and humidity on the metasurfaces. The test verifies that at temperatures below the glass transition temperature of the base resin, the nanostructures do not collapse, so the efficiency of the metasurfaces remains almost the same. The surrounding humidity does not affect the nanostructures at all. Hence, the durability of the nanocomposite metasurfaces can be further enhanced by replacing the base resin, and this nanocomposite printing method will facilitate practical metasurface use at low cost.

Journal ArticleDOI
TL;DR: In this article , a gap-shifted split ring resonator (SRR) was used to achieve spin angular momentum selection and achieved the maximum calculated circular dichroism in reflection (CDR) of 0.91.
Abstract: Abstract Tunable metasurfaces can replace conventional bulky active optical modules to realize practical flat optical devices such as lenses, LiDAR, holography, and augmented reality. However, tunable metasurfaces have generally been limited to switching between two distinct states. Here, we present liquid crystal (LC) integrated chiral metasurfaces, of which the metahologram intensity can be adjusted continuously between fully ‘on’ and ‘off’ states. The chiral metasurface consists of a gap-shifted split ring resonator (SRR), and exhibits spin angular momentum selection that reflects left-circularly-polarized light but perfectly absorbs right-circularly-polarized light (99.9%). The gap-shifted SRR realizes spin angular momentum selection using a metal–dielectric–metal multilayer structure and thereby induces a strong gap-plasmonic response, achieving the maximum calculated circular dichroism in reflection (CDR) of 0.99 at the wavelength of 635 nm. With the chiral metasurface, metaholograms are demonstrated with tunable intensities using LCs that change the polarization state of the output light using an applied voltage. With the LC integrated chiral metasurfaces, 23 steps of polarization are demonstrated for the continuous tuning of the holographic image intensity, achieving measured CDR of 0.91. The proposed LC integrated spin-selective chiral metasurface provides a new resource for development of compact active optical modules with continuously-tunable intensity.