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Perovskite solar cells: An integrated hybrid lifecycle assessment and review in comparison with other photovoltaic technologies

TLDR
In this paper, a critical review of some existing photovoltaic (PV) technologies in comparison with perovskite-structured solar cells (PSCs), including material and performance parameters, production processes and manufacturing complexity, economics, key technological challenges for further developments and current research efforts is presented.
Abstract
Solar cells are considered as one of the prominent sources of renewable energy suitable for large-scale adoption in a carbon-constrained world and can contribute to reduced reliance on energy imports, whilst improving the security of energy supply. A new arrival in the family of solar cells technologies is the organic-inorganic halide perovskite. The major thrust for endorsing these new solar cells pertains to their potential as an economically and environmentally viable option to traditional silicon-based technology. To verify this assertion, this paper presents a critical review of some existing photovoltaic (PV) technologies in comparison with perovskite-structured solar cells (PSCs), including material and performance parameters, production processes and manufacturing complexity, economics, key technological challenges for further developments and current research efforts. At present, there is limited environmental assessment of PSCs and consequently, a methodologically robust and environmentally expansive lifecycle supply chain assessment of two types of PSC modules A and B is also undertaken within the context of other PV technologies, to assess their potential for environmentally friendly innovation in the energy sector. Module A is based on MAPbX3 perovskite structure while module B is based on CsFAPbX3 with improved stability, reproducibility and high performance efficiency. The main outcomes, presented along with sensitivity analysis, show that PSCs offer more environmentally friendly and sustainable option, with the least energy payback period, as compared to other PV technologies. The review and analysis presented provide valuable insight and guidance in identifying pathways and windows of opportunity for future PV designs towards cleaner and sustainable energy production.

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Journal ArticleDOI

How to Make over 20% Efficient Perovskite Solar Cells in Regular (n-i-p) and Inverted (p-i-n) Architectures

TL;DR: This work presents detailed protocols for preparing PSCs in regular (n–i–p) and inverted (p–i-n) architectures with ≥20% PCE and encourages the practice of reporting detailed and transparent protocols that can be more easily reproduced by other laboratories.
Journal ArticleDOI

Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering.

TL;DR: A unique outlook on the paths toward commercialization of PVKSCs from the interfacial engineering perspective is offered, relevant to both specialists and nonspecialists in the field through a brief introduction of the background of the field, current state-of-the-art evolution, and future research prospects.
Journal ArticleDOI

Enhanced solar cell stability by hygroscopic polymer passivation of metal halide perovskite thin film

TL;DR: In this paper, a functional hygroscopic polymer, poly(ethylene oxide), was applied to perovskite solar cells to make them more stable in a humid environment.
Journal ArticleDOI

Electron and hole transport layers optimization by numerical simulation of a perovskite solar cell

TL;DR: In this paper, an n-i-p perovskite solar cell was studied using SCAPS simulator and the primary solar cell's structure is FTO/ITO/PERVskite/PEDOT:PSS/Au which has achieved a power conversion efficiency of η∼ 13.94%.
References
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Journal ArticleDOI

A low-cost, high-efficiency solar cell based on dye-sensitized colloidal TiO2 films

TL;DR: In this article, the authors describe a photovoltaic cell, created from low-to medium-purity materials through low-cost processes, which exhibits a commercially realistic energy-conversion efficiency.
Journal ArticleDOI

Organometal Halide Perovskites as Visible-Light Sensitizers for Photovoltaic Cells

TL;DR: Two organolead halide perovskite nanocrystals were found to efficiently sensitize TiO(2) for visible-light conversion in photoelectrochemical cells, which exhibit strong band-gap absorptions as semiconductors.
Journal ArticleDOI

Efficient Hybrid Solar Cells Based on Meso-Superstructured Organometal Halide Perovskites

TL;DR: A low-cost, solution-processable solar cell, based on a highly crystalline perovskite absorber with intense visible to near-infrared absorptivity, that has a power conversion efficiency of 10.9% in a single-junction device under simulated full sunlight is reported.
Journal ArticleDOI

Sequential deposition as a route to high-performance perovskite-sensitized solar cells

TL;DR: A sequential deposition method for the formation of the perovskite pigment within the porous metal oxide film that greatly increases the reproducibility of their performance and allows the fabrication of solid-state mesoscopic solar cells with unprecedented power conversion efficiencies and high stability.
Journal ArticleDOI

Electron-hole diffusion lengths exceeding 1 micrometer in an organometal trihalide perovskite absorber.

TL;DR: In this article, transient absorption and photoluminescence-quenching measurements were performed to determine the electron-hole diffusion lengths, diffusion constants, and lifetimes in mixed halide and triiodide perovskite absorbers.
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