Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering.
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TLDR
A unique outlook on the paths toward commercialization of PVKSCs from the interfacial engineering perspective is offered, relevant to both specialists and nonspecialists in the field through a brief introduction of the background of the field, current state-of-the-art evolution, and future research prospects.Abstract:
High-efficiency and low-cost perovskite solar cells (PVKSCs) are an ideal candidate for addressing the scalability challenge of solar-based renewable energy. The dynamically evolving research field of PVKSCs has made immense progress in solving inherent challenges and capitalizing on their unique structure-property-processing-performance traits. This review offers a unique outlook on the paths toward commercialization of PVKSCs from the interfacial engineering perspective, relevant to both specialists and nonspecialists in the field through a brief introduction of the background of the field, current state-of-the-art evolution, and future research prospects. The multifaceted role of interfaces in facilitating PVKSC development is explained. Beneficial impacts of diverse charge-transporting materials and interfacial modifications are summarized. In addition, the role of interfaces in improving efficiency and stability for all emerging areas of PVKSC design are also evaluated. The authors' integral contributions in this area are highlighted on all fronts. Finally, future research opportunities for interfacial material development and applications along with scalability-durability-sustainability considerations pivotal for facilitating laboratory to industry translation are presented.read more
Citations
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Journal ArticleDOI
Regulating Surface Termination for Efficient Inverted Perovskite Solar Cells with Greater Than 23% Efficiency
Fengzhu Li,Xiang Deng,Feng Qi,Zhen Li,Danjun Liu,Dong Shen,Minchao Qin,Shengfan Wu,Francis Lin,Sei-Hum Jang,Jie Zhang,Xinhui Lu,Dangyuan Lei,Chun-Sing Lee,Zonglong Zhu,Alex K.-Y. Jen +15 more
TL;DR: A rationally designed bifunctional molecule, piperazinium iodide (PI), containing both R2NH and R2 NH2+ groups on the same six-membered ring, behaving both as an electron donor and an electron acceptor to react with different surface-terminating ends on perovskite films is reported.
Journal ArticleDOI
Reduction of lead leakage from damaged lead halide perovskite solar modules using self-healing polymer-based encapsulation
Yan Jiang,Yan Jiang,Longbin Qiu,Emilio J. Juarez-Perez,Luis K. Ono,Zhanhao Hu,Zonghao Liu,Zhifang Wu,Lingqiang Meng,Qijing Wang,Yabing Qi +10 more
TL;DR: In this article, Jiang et al. demonstrate that the encapsulation method based on an epoxy resin reduces the Pb leakage rate by a factor of 375 compared with the one based on a glass cover with an ultraviolet-cured resin at the module edges.
Journal ArticleDOI
Interface and Defect Engineering for Metal Halide Perovskite Optoelectronic Devices.
TL;DR: A comprehensive review of various strategies that attempt to modify the interfacial characteristics, control the crystal growth, and understand the defect physics in metal halide perovskites, for both solar cell and LED applications, is presented.
Journal ArticleDOI
Materials and Methods for Interface Engineering toward Stable and Efficient Perovskite Solar Cells
Jiangzhao Chen,Nam-Gyu Park +1 more
TL;DR: In this article, the minimization of interfacial nonradiative recombination (NRR) losses through interface engineering especially for perovovision devices is discussed. But this work is restricted to the perovision case.
Journal ArticleDOI
Low dimensional metal halide perovskites and hybrids
Chenkun Zhou,Haoran Lin,Qingquan He,Liang-Jin Xu,Michael Worku,Maya Chaaban,Sujin Lee,Xiaoqin Shi,Xiaoqin Shi,Mao-Hua Du,Biwu Ma,Biwu Ma +11 more
TL;DR: In this article, the authors discuss the synthesis, characterization, application, and computational studies of low dimensional metal halide perovskites and hybrid structures at the molecular level using appropriate organic and inorganic components.
References
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Organometal Halide Perovskites as Visible-Light Sensitizers for Photovoltaic Cells
TL;DR: Two organolead halide perovskite nanocrystals were found to efficiently sensitize TiO(2) for visible-light conversion in photoelectrochemical cells, which exhibit strong band-gap absorptions as semiconductors.
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TL;DR: A low-cost, solution-processable solar cell, based on a highly crystalline perovskite absorber with intense visible to near-infrared absorptivity, that has a power conversion efficiency of 10.9% in a single-junction device under simulated full sunlight is reported.
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Interface engineering of highly efficient perovskite solar cells
Huanping Zhou,Qi Chen,Gang Li,Song Luo,Tze Bing Song,Hsin Sheng Duan,Ziruo Hong,Jingbi You,Yongsheng Liu,Yang Yang +9 more
TL;DR: Perovskite films received a boost in photovoltaic efficiency through controlled formation of charge-generating films and improved current transfer to the electrodes and low-temperature processing steps allowed the use of materials that draw current out of the perovskites layer more efficiently.
Journal ArticleDOI
Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
TL;DR: A bilayer architecture comprising the key features of mesoscopic and planar structures obtained by a fully solution-based process is reported, providing important progress towards the understanding of the role of solution-processing in the realization of low-cost and highly efficient perovskite solar cells.
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High-performance photovoltaic perovskite layers fabricated through intramolecular exchange
Woon Seok Yang,Jun Hong Noh,Nam Joong Jeon,Young Chan Kim,Seungchan Ryu,Jangwon Seo,Sang Il Seok +6 more
TL;DR: An approach for depositing high-quality FAPbI3 films, involving FAP bI3 crystallization by the direct intramolecular exchange of dimethylsulfoxide (DMSO) molecules intercalated in PbI2 with formamidinium iodide is reported.