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Research progress on two-dimensional (2D) halide organic–inorganic hybrid perovskites

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TLDR
In this article, a review mainly describes the development and application of 2D perovskites in recent years and discusses the change in their characteristics and performances with a variation in the number of inorganic layers.
Abstract
Since its discovery, perovskite has experienced tremendous development. Furthermore, due to the outstanding stability of two-dimensional (2D) perovskites, they have been attracting increasing attention. A reduction in the dimensions of perovskites and the introduction of long organic chains yield new structures and properties. As an emerging semiconductor material with high stability, 2D perovskites have many applications in the field of optoelectronics. This review mainly describes the development and application of 2D perovskites in recent years. Firstly, we introduce the basic structure and classification of 2D perovskites. Also, we discuss the change in their characteristics and performances with a variation in the number of inorganic layers. Next, 2D perovskites are classified according to their applications in different fields. Finally, a summary and outlook based on the current development trends of 2D perovskites are presented.

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Citations
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Stability of 2D and quasi-2D perovskite materials and devices

TL;DR: In this article , different 2D and quasi-2D perovskite materials have demonstrated significant improvements in the device stability compared to 3D materials due to their increased hydrophobicity and suppressed ion migration.
Journal ArticleDOI

Progress and challenges in layered two-dimensional hybrid perovskites

TL;DR: In this paper , the authors have given brief insight on structural versatility, synthesis techniques, some of the unique photophysical properties, potential device fabrication, and recent advancements in the 2D structure to stand against degradation.
Journal ArticleDOI

Recent Developments of Optoelectronic Synaptic Devices Based on Metal Halide Perovskites

TL;DR: In this paper , a review of the recent progress on OSDs based on metal halide perovskites (MHPs) including the structures and properties of MHPs, and the architectures and performance characteristics of MHP-OSDs are presented.
Journal ArticleDOI

Accelerated screening of functional atomic impurities in halide perovskites using high-throughput computations and machine learning

TL;DR: In this article , the impurity properties of halide perovskites computed using density functional theory (DFT) can be combined with machine learning (ML) to deliver predictive models and quick identification of optoelectronically active impurity atoms.
Journal ArticleDOI

Impact of Crystal Growth Diversity on Magneto-Photoluminescence and Circular Dichroism in Chiral Lead Halide Perovskites

TL;DR: Chiral-induced magneto-photoluminescence (magneto-PL) is a newly raised magnetooptical phenomenon, where a photolumine intensity can be effectively manipulated by magnetic fields and material helicity as mentioned in this paper .
References
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Journal ArticleDOI

Uniform Permutation of Quasi-2D Perovskites by Vacuum Poling for Efficient, High-Fill-Factor Solar Cells

TL;DR: In this paper, a different strategy of uniformly arranging different n-value nanoplates (PEA2MAn-1PbnI3n+1) by introducing vacuum poling treatment to enforce nucleation during crystallization is reported.
Journal ArticleDOI

Copper-Substituted Lead Perovskite Materials Constructed with Different Halides for Working (CH3NH3)2CuX4-Based Perovskite Solar Cells from Experimental and Theoretical View.

TL;DR: Cu-based perovskite-like materials showed attractive absorbance features extended to the near-infrared range, with appropriate band gaps, and green photoluminescence of these materials was obtained because of Cu+ ions.
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Self-Repairing Tin-Based Perovskite Solar Cells with a Breakthrough Efficiency Over 11%

TL;DR: Phenylhydrazine hydrochloride (PHCl) is introduced into FASnI3 (FA = NH2 CH =NH2 + ) perovskite films to reduce the existing Sn4+ and prevent the further degradation of FAS nI3 , since PHCl has a reductive hydrazino group and a hydrophobic phenyl group.
Journal ArticleDOI

High-performance quasi-2D perovskite light-emitting diodes: from materials to devices.

TL;DR: In this article, the inherent properties of quasi-2D perovskite materials, the corresponding energy transfer and spectral tunability methodologies for thin films, as well as their application in high-performance LEDs are summarized.
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What is the basic concepts and structural characteristics of two-dimensional organic halide perovskite materials?

The paper discusses the basic structure and classification of two-dimensional (2D) organic halide perovskite materials and their characteristics and performances with a variation in the number of inorganic layers.