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Research progress on two-dimensional (2D) halide organic–inorganic hybrid perovskites

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TLDR
In this article, a review mainly describes the development and application of 2D perovskites in recent years and discusses the change in their characteristics and performances with a variation in the number of inorganic layers.
Abstract
Since its discovery, perovskite has experienced tremendous development. Furthermore, due to the outstanding stability of two-dimensional (2D) perovskites, they have been attracting increasing attention. A reduction in the dimensions of perovskites and the introduction of long organic chains yield new structures and properties. As an emerging semiconductor material with high stability, 2D perovskites have many applications in the field of optoelectronics. This review mainly describes the development and application of 2D perovskites in recent years. Firstly, we introduce the basic structure and classification of 2D perovskites. Also, we discuss the change in their characteristics and performances with a variation in the number of inorganic layers. Next, 2D perovskites are classified according to their applications in different fields. Finally, a summary and outlook based on the current development trends of 2D perovskites are presented.

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Stability of 2D and quasi-2D perovskite materials and devices

TL;DR: In this article , different 2D and quasi-2D perovskite materials have demonstrated significant improvements in the device stability compared to 3D materials due to their increased hydrophobicity and suppressed ion migration.
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Progress and challenges in layered two-dimensional hybrid perovskites

TL;DR: In this paper , the authors have given brief insight on structural versatility, synthesis techniques, some of the unique photophysical properties, potential device fabrication, and recent advancements in the 2D structure to stand against degradation.
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Recent Developments of Optoelectronic Synaptic Devices Based on Metal Halide Perovskites

TL;DR: In this paper , a review of the recent progress on OSDs based on metal halide perovskites (MHPs) including the structures and properties of MHPs, and the architectures and performance characteristics of MHP-OSDs are presented.
Journal ArticleDOI

Accelerated screening of functional atomic impurities in halide perovskites using high-throughput computations and machine learning

TL;DR: In this article , the impurity properties of halide perovskites computed using density functional theory (DFT) can be combined with machine learning (ML) to deliver predictive models and quick identification of optoelectronically active impurity atoms.
Journal ArticleDOI

Impact of Crystal Growth Diversity on Magneto-Photoluminescence and Circular Dichroism in Chiral Lead Halide Perovskites

TL;DR: Chiral-induced magneto-photoluminescence (magneto-PL) is a newly raised magnetooptical phenomenon, where a photolumine intensity can be effectively manipulated by magnetic fields and material helicity as mentioned in this paper .
References
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Journal ArticleDOI

Low-Dimensional Perovskites with Diammonium and Monoammonium Alternant Cations for High-Performance Photovoltaics.

TL;DR: Ultrafast transient absorption indicates that B-ACI perovskites exhibit a narrow distribution of quantum well widths, leading to a barrier-free and balanced carrier transport pathway with enhanced carrier diffusion (electron and hole) length over 350 nm.
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Field-Effect Transistors Based on van-der-Waals-Grown and Dry-Transferred All-Inorganic Perovskite Ultrathin Platelets

TL;DR: This work reports on high-performance all-inorganic perovskite FETs profiting from both van der Waals epitaxial boundary-free ultrathin single crystals and completely dry-processed transfer technique without chemical contaminant, which could open the door for the FET applications based on perovSKite single crystals.
Journal ArticleDOI

Lead and HTM Free Stable Two-Dimensional Tin Perovskites with Suitable Band Gap for Solar Cell Applications.

TL;DR: It is found that the use of symmetrical imidazolium-based cations allow the formation of 2D perovskites with relatively narrow band gaps compared to traditional -NH3 + amino groups, with optical band gap values of 1.81”eV and 1.79 eV for Bn2 SnI4 and BdiSnI4 respectively.
Journal ArticleDOI

Highly Enhanced Third-Harmonic Generation in 2D Perovskites at Excitonic Resonances

TL;DR: In this article, the authors performed parametric nonlinear optical characterization of 2D perovskite nanosheets mechanically exfoliated from four different lead halide RPP single crystals.
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What is the basic concepts and structural characteristics of two-dimensional organic halide perovskite materials?

The paper discusses the basic structure and classification of two-dimensional (2D) organic halide perovskite materials and their characteristics and performances with a variation in the number of inorganic layers.