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Research progress on two-dimensional (2D) halide organic–inorganic hybrid perovskites

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TLDR
In this article, a review mainly describes the development and application of 2D perovskites in recent years and discusses the change in their characteristics and performances with a variation in the number of inorganic layers.
Abstract
Since its discovery, perovskite has experienced tremendous development. Furthermore, due to the outstanding stability of two-dimensional (2D) perovskites, they have been attracting increasing attention. A reduction in the dimensions of perovskites and the introduction of long organic chains yield new structures and properties. As an emerging semiconductor material with high stability, 2D perovskites have many applications in the field of optoelectronics. This review mainly describes the development and application of 2D perovskites in recent years. Firstly, we introduce the basic structure and classification of 2D perovskites. Also, we discuss the change in their characteristics and performances with a variation in the number of inorganic layers. Next, 2D perovskites are classified according to their applications in different fields. Finally, a summary and outlook based on the current development trends of 2D perovskites are presented.

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Stability of 2D and quasi-2D perovskite materials and devices

TL;DR: In this article , different 2D and quasi-2D perovskite materials have demonstrated significant improvements in the device stability compared to 3D materials due to their increased hydrophobicity and suppressed ion migration.
Journal ArticleDOI

Progress and challenges in layered two-dimensional hybrid perovskites

TL;DR: In this paper , the authors have given brief insight on structural versatility, synthesis techniques, some of the unique photophysical properties, potential device fabrication, and recent advancements in the 2D structure to stand against degradation.
Journal ArticleDOI

Recent Developments of Optoelectronic Synaptic Devices Based on Metal Halide Perovskites

TL;DR: In this paper , a review of the recent progress on OSDs based on metal halide perovskites (MHPs) including the structures and properties of MHPs, and the architectures and performance characteristics of MHP-OSDs are presented.
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Accelerated screening of functional atomic impurities in halide perovskites using high-throughput computations and machine learning

TL;DR: In this article , the impurity properties of halide perovskites computed using density functional theory (DFT) can be combined with machine learning (ML) to deliver predictive models and quick identification of optoelectronically active impurity atoms.
Journal ArticleDOI

Impact of Crystal Growth Diversity on Magneto-Photoluminescence and Circular Dichroism in Chiral Lead Halide Perovskites

TL;DR: Chiral-induced magneto-photoluminescence (magneto-PL) is a newly raised magnetooptical phenomenon, where a photolumine intensity can be effectively manipulated by magnetic fields and material helicity as mentioned in this paper .
References
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Journal ArticleDOI

Orange to Red, Emission-Tunable Mn-Doped Two-Dimensional Perovskites with High Luminescence and Stability.

TL;DR: A facile and convenient hot-injection strategy to synthesize Mn doped two-dimensional (2D) perovskite nanosheets is reported, which achieves a QY as high as 97% and possesses excellent stability, whose emission property can be maintained for almost one year.
Journal ArticleDOI

Regulating Second-Harmonic Generation by van der Waals Interactions in Two-dimensional Lead Halide Perovskite Nanosheets.

TL;DR: Combined first-principles calculations and Monte Carlo simulations reveal that the induced second-order polarization arises primarily from the (C6H5CH2NH3)+ cations; and these organic amine cations form significantly reorganized conformations with decreasing nanosheet thickness due to weakened van der Waals interactions.
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High Performance Quasi-2D Perovskite Sky-Blue Light-Emitting Diodes Using a Dual-Ligand Strategy

TL;DR: By adjusting the proportion of the two ligands, sky-blue perovskite light-emitting diodes (PeLEDs) with electroluminescence (EL) peak located 485 nm are achieved with a maximum luminance up to 1130 cd m-2 and a maximum external quantum efficiency (EQE) up to 7.84%.
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What is the basic concepts and structural characteristics of two-dimensional organic halide perovskite materials?

The paper discusses the basic structure and classification of two-dimensional (2D) organic halide perovskite materials and their characteristics and performances with a variation in the number of inorganic layers.