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Showing papers on "Microphysics published in 2011"


Journal ArticleDOI
TL;DR: In this paper, the authors show that in general, lightning activity is tightly correlated with aerosol loadings at both inter-annual and biweekly time scales, and they estimate that approximately 60% increase in aerosol loading leads to more than 150 percent increase in lightning flashes.
Abstract: Lightning activity over the West Pacific Ocean east of the Philippines is usually much less frequent than over the nearby maritime continents. However, in 2005 the Lightning Imaging Sensor (LIS) aboard the TRMM satellite observed anomalously high lightning activity in that area. In the same year the Moderate resolution Imaging Spectroradiometer (MODIS) measured anomalously high aerosol loading. The high aerosol loading was traced to volcanic activity, and not to any factor linked to meteorology, disentangling the usual convolution between aerosols and meteorology. We show that in general lightning activity is tightly correlated with aerosol loadings at both inter-annual and biweekly time scales. We estimate that a approximately 60% increase in aerosol loading leads to more than 150% increase in lightning flashes. Aerosols increase lightning activity through modification of cloud microphysics. Cloud ice particle sizes are reduced and cloud glaciation is delayed to colder temperature when aerosol loading is increased. TRMM precipitation radar measurements indicate that anomalously high aerosol loading is associated with enhanced cloud mixed phase activity and invigorated convection over the maritime ocean. These observed associations between aerosols, cloud microphysics, morphology and lightning activity are not related to meteorological variables or ENSO events. The results have important implications for understanding the variability of lightning and resulting aerosol-chemistry interactions.

174 citations


Journal ArticleDOI
TL;DR: This paper performed three-dimensional supercell simulations using the two-moment bulk microphysics schemes of Morrison and Milbrandt-Yau in the Weather Research and Forecasting (WRF) model.
Abstract: Idealized three-dimensional supercell simulations were performed using the two-moment bulk microphysics schemes of Morrison and Milbrandt–Yau in the Weather Research and Forecasting (WRF) model. Despite general similarities in these schemes, the simulations were found to produce distinct differences in storm structure, precipitation, and cold pool strength. In particular, the Morrison scheme produced much higher surface precipitation rates and a stronger cold pool, especially in the early stages of storm development. A series of sensitivity experiments was conducted to identify the primary differences between the two schemes that resulted in the large discrepancies in the simulations.Different approaches in treating graupel and hail were found to be responsible for many of the key differences between the baseline simulations. The inclusion of hail in the baseline simulation using the Milbrant–Yau scheme with two rimed-ice categories (graupel and hail) had little impact, and therefore resulted in a...

174 citations


Journal ArticleDOI
TL;DR: The radar observation operator for computation of polarimetric radar variables from the output of numerical cloud models is described in its most generic form in this paper, which is combined with the Hebrew University of Jerusalem cloud model with spectral microphysics.
Abstract: The radar observation operator for computation of polarimetric radar variables from the output of numerical cloud models is described in its most generic form. This operator is combined with the Hebrew University of Jerusalem cloud model with spectral microphysics. The model contains 7 classes of hydrometeors and each class is represented by size distribution functions in 43 size bins. The performance of the cloud model and radar observation operator has been evaluated for the case of a hailstorm in Oklahoma on 2 February 2009. It is shown that the retrieved fields of polarimetric radar variables at C and S microwave bands are generally consistent with results of observations. The relationship between microphysical and polarimetric signatures is illustrated.

158 citations


Journal ArticleDOI
TL;DR: In this paper, a hail storm at Villingen-Schwenningen, southwest Germany, on 28.06.2006 was simulated using the Hebrew University Cloud Model (HUCM) with spectral (bin) microphysics.

126 citations


Journal ArticleDOI
TL;DR: In this paper, the authors evaluated the Weather Research and Forecasting model (WRF) sensitivity to eight different combinations of cumulus, microphysics, and planetary boundary layer (PBL) parameterization schemes over a topographically complex region in southern Spain (Andalusia) for the period 1990-99.
Abstract: This paper evaluates the Weather Research and Forecasting model (WRF) sensitivity to eight different combinations of cumulus, microphysics, and planetary boundary layer (PBL) parameterization schemes over a topographically complex region in southern Spain (Andalusia) for the period 1990–99. The WRF configuration consisted of a 10-km-resolution domain nested in a coarser domain driven by 40-yr European Centre for Medium-Range Weather Forecasts Re-Analysis (ERA-40) data, with spectral nudging above the PBL employed over the latter domain. The model outputs have been compared at different time scales with an observational dataset that comprises 438 rain gauges and 152 temperature stations with records of both daily maximum and minimum temperatures. To reduce the ‘‘representation error,’’ the validation with observations has been performed using a multistep regionalization that distinguishes five precipitation regions and four temperature regions. The analysis proves that both cumulus and PBL schemes have a crucial impact on the description of precipitation in Andalusia, whereas no noticeable differences between microphysics options were appreciated. Temperature is described similarly by all the configurations, except for the PBL choice affecting minimum values. WRF provides a definite improvement over ERA-40 in the climate description in terms of frequency, spatial distribution, and intensity of extreme events. It also captures more accurately the annual cycle and reduces the biases and the RMSE for monthly precipitation, whereas only a minor enhancement of these features was obtained for monthly-mean maximum and minimum temperatures. The results indicate that WRF is able to correctly reproduce Andalusian climate and produces useful added-value information for climate studies.

112 citations


Journal ArticleDOI
TL;DR: In this paper, the potential effects of increased aerosol loading on the development of deep convective clouds and resulting precipitation amounts are studied by employing the Weather Research and Forecasting (WRF) model as a detailed high-resolution cloud resolving model (CRM) with both detailed bulk and bin microphysics schemes.
Abstract: . The potential effects of increased aerosol loading on the development of deep convective clouds and resulting precipitation amounts are studied by employing the Weather Research and Forecasting (WRF) model as a detailed high-resolution cloud resolving model (CRM) with both detailed bulk and bin microphysics schemes. Both models include a physically-based activation scheme that incorporates a size-resolved aerosol population. We demonstrate that the aerosol-induced effect is controlled by the balance between latent heating and the increase in condensed water aloft, each having opposing effects on buoyancy. It is also shown that under polluted conditions, increases in the CCN number concentration reduce the cumulative precipitation due to the competition between the sedimentation and evaporation/sublimation timescales. The effect of an increase in the IN number concentration on the dynamics of deep convective clouds is small and the resulting decrease in domain-averaged cumulative precipitation is shown not to be statistically significant, but may act to suppress precipitation. It is also shown that even in the presence of a decrease in the domain-averaged cumulative precipitation, an increase in the precipitation variance, or in other words, andincrease in rainfall intensity, may be expected in more polluted environments, especially in moist environments. A significant difference exists between the predictions based on the bin and bulk microphysics schemes of precipitation and the influence of aerosol perturbations on updraft velocity within the convective core. The bulk microphysics scheme shows little change in the latent heating rates due to an increase in the CCN number concentration, while the bin microphysics scheme demonstrates significant increases in the latent heating aloft with increasing CCN number concentration. This suggests that even a detailed two-bulk microphysics scheme, coupled to a detailed activation scheme, may not be sufficient to predict small changes that result from perturbations in aerosol loading.

111 citations


Journal ArticleDOI
TL;DR: The manifestation of predator-prey behavior in the aerosol–cloud–precipitation system is a further example of the self-organizing properties of the system and suggests that exploiting principles of population dynamics may help reduce complex aerosol-cloud–rain interactions to a more tractable problem.
Abstract: We show that the aerosol–cloud–precipitation system exhibits characteristics of the predator-prey problem in the field of population dynamics. Both a detailed large eddy simulation of the dynamics and microphysics of a precipitating shallow boundary layer cloud system and a simpler model built upon basic physical principles, reproduce predator-prey behavior with rain acting as the predator and cloud as the prey. The aerosol is shown to modulate the predator-prey response. Steady-state solution to the proposed model shows the known existence of bistability in cloudiness. Three regimes are identified in the time-dependent solutions: (i) the weakly precipitating regime where cloud and rain coexist in a quasi steady state; (ii) the moderately drizzling regime where limit-cycle behavior in the cloud and rain fields is produced; and (iii) the heavily precipitating clouds where collapse of the boundary layer is predicted. The manifestation of predator-prey behavior in the aerosol–cloud–precipitation system is a further example of the self-organizing properties of the system and suggests that exploiting principles of population dynamics may help reduce complex aerosol–cloud–rain interactions to a more tractable problem.

108 citations


Journal ArticleDOI
TL;DR: In this article, the authors assess the ability of the recent chemistry version (v3.3) of the Weather Research and Forecasting (WRF-Chem) model to simulate boundary layer structure, aerosols, stratocumulus clouds, and energy fluxes over the Southeast Pacific Ocean.
Abstract: . This study assesses the ability of the recent chemistry version (v3.3) of the Weather Research and Forecasting (WRF-Chem) model to simulate boundary layer structure, aerosols, stratocumulus clouds, and energy fluxes over the Southeast Pacific Ocean. Measurements from the VAMOS Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx) and satellite retrievals (i.e., products from the MODerate resolution Imaging Spectroradiometer (MODIS), Clouds and Earth's Radiant Energy System (CERES), and GOES-10) are used for this assessment. The Morrison double-moment microphysics scheme is newly coupled with interactive aerosols in the model. The 31-day (15 October–16 November 2008) WRF-Chem simulation with aerosol-cloud interactions (AERO hereafter) is also compared to a simulation (MET hereafter) with fixed cloud droplet number concentrations in the microphysics scheme and simplified cloud and aerosol treatments in the radiation scheme. The well-simulated aerosol quantities (aerosol number, mass composition and optical properties), and the inclusion of full aerosol-cloud couplings lead to significant improvements in many features of the simulated stratocumulus clouds: cloud optical properties and microphysical properties such as cloud top effective radius, cloud water path, and cloud optical thickness. In addition to accounting for the aerosol direct and semi-direct effects, these improvements feed back to the simulation of boundary-layer characteristics and energy budgets. Particularly, inclusion of interactive aerosols in AERO strengthens the temperature and humidity gradients within the capping inversion layer and lowers the marine boundary layer (MBL) depth by 130 m from that of the MET simulation. These differences are associated with weaker entrainment and stronger mean subsidence at the top of the MBL in AERO. Mean top-of-atmosphere outgoing shortwave fluxes, surface latent heat, and surface downwelling longwave fluxes are in better agreement with observations in AERO, compared to the MET simulation. Nevertheless, biases in some of the simulated meteorological quantities (e.g., MBL temperature and humidity) and aerosol quantities (e.g., underestimations of accumulation mode aerosol number) might affect simulated stratocumulus and energy fluxes over the Southeastern Pacific, and require further investigation. The well-simulated timing and outflow patterns of polluted and clean episodes demonstrate the model's ability to capture daily/synoptic scale variations of aerosol and cloud properties, and suggest that the model is suitable for studying atmospheric processes associated with pollution outflow over the ocean. The overall performance of the regional model in simulating mesoscale clouds and boundary layer properties is encouraging and suggests that reproducing gradients of aerosol and cloud droplet concentrations and coupling cloud-aerosol-radiation processes are important when simulating marine stratocumulus over the Southeast Pacific.

108 citations


Journal ArticleDOI
TL;DR: In this paper, the International Cloud Experiment (TWP ]ICE) provided extensive observational data sets designed to initialize, force, and constrain atmospheric model simulations, including radar reflectivity and satellite infrared brightness temperature observations.
Abstract: The Tropical Warm Pool.International Cloud Experiment (TWP ]ICE) provided extensive observational data sets designed to initialize, force, and constrain atmospheric model simulations. In this first of a two ]part study, precipitation and cloud structures within nine cloud ]resolving model simulations are compared with scanning radar reflectivity and satellite infrared brightness temperature observations during an active monsoon period from 19 to 25 January 2006. Seven of nine simulations overestimate convective area by 20% or more leading to general overestimation of convective rainfall. This is balanced by underestimation of stratiform rainfall by 5% to 50% despite overestimation of stratiform area by up to 65% because of a preponderance of very low stratiform rain rates in all simulations. All simulations fail to reproduce observed radar reflectivity distributions above the melting level in convective regions and throughout the troposphere in stratiform regions. Observed precipitation ]sized ice reaches higher altitudes than simulated precipitation ]sized ice despite some simulations that predict lower than observed top ]of ]atmosphere infrared brightness temperatures. For the simulations that overestimate radar reflectivity aloft, graupel is the cause with one ]moment microphysics schemes whereas snow is the cause with two ]moment microphysics schemes. Differences in simulated radar reflectivity are more highly correlated with differences in mass mean melted diameter (Dm) than differences in ice water content. Dm is largely dependent on the mass ]dimension relationship and gamma size distribution parameters such as size intercept (N0) and shape parameter (m). Having variable density, variable N0, or m greater than zero produces radar reflectivities closest to those observed.

102 citations


Journal ArticleDOI
TL;DR: A review of previous modeling studies on the impact of micro-physical schemes and processes on the intensity and track of hurricanes is presented and compared against the current Katrina study in this article.
Abstract: During the past decade, both research and operational numerical weather prediction models [e.g. the Weather Research and Forecasting Model (WRF)] have started using more complex microphysical schemes originally developed for high-resolution cloud resolving models (CRMs) with 1-2 km or less horizontal resolutions. WRF is a next-generation meso-scale forecast model and assimilation system. It incorporates a modern software framework, advanced dynamics, numerics and data assimilation techniques, a multiple moveable nesting capability, and improved physical packages. WRF can be used for a wide range of applications, from idealized research to operational forecasting, with an emphasis on horizontal grid sizes in the range of 1-10 km. The current WRF includes several different microphysics options. At NASA Goddard, four different cloud microphysics options have been implemented into WRF. The performance of these schemes is compared to those of the other microphysics schemes available in WRF for an Atlantic hurricane case (Katrina). In addition, a brief review of previous modeling studies on the impact of microphysics schemes and processes on the intensity and track of hurricanes is presented and compared against the current Katrina study. In general, all of the studies show that microphysics schemes do not have a major impact on track forecasts but do have more of an effect on the simulated intensity. Also, nearly all of the previous studies found that simulated hurricanes had the strongest deepening or intensification when using only warm rain physics. This is because all of the simulated precipitating hydrometeors are large raindrops that quickly fall out near the eye-wall region, which would hydrostatically produce the lowest pressure. In addition, these studies suggested that intensities become unrealistically strong when evaporative cooling from cloud droplets and melting from ice particles are removed as this results in much weaker downdrafts in the simulated storms. However, there are many differences between the different modeling studies, which are identified and discussed.

101 citations


Journal ArticleDOI
TL;DR: In this paper, an efficient two-moment microphysics parameterization scheme for convective clouds is developed to improve the representation of convective cloud and its interactions with stratiform clouds and aerosol in global climate models.
Abstract: [1] An efficient two-moment microphysics parameterization scheme for convective clouds is developed to improve the representation of convective clouds and its interactions with stratiform clouds and aerosol in global climate models (GCMs). The scheme explicitly treats mass mixing ratio and number concentration of four hydrometeor species (cloud water, cloud ice, rain, and snow) and describes several microphysical processes, including autoconversion, self-collection, collection between hydrometeor species, freezing, cloud ice nucleation, droplet activation, and sedimentation. Thus this physically based scheme is suitable for investigating the interaction between convection and aerosol and the indirect aerosol effect on climate. An evaluation of the scheme in the single-column version of NCAR Community Atmospheric Model version 3.5 (CAM3.5) with the Tropical Warm Pool–International Cloud Experiment (TWP-ICE) data shows that the simulation of cloud microphysical properties in convective core is significantly improved, indicating that the new parameterization describes the microphysical processes in convection reasonably well. The contribution from convective detrainment to large-scale cloud ice and liquid water budgets is enhanced greatly. With more realistic convective cloud microphysical properties and their detrainment, the surface stratiform precipitation, which is seriously underestimated in the model, is increased by a factor of roughly 2.5, and therefore is much closer to the observations. In addition, the simulations of net surface shortwave radiation flux, OLR, specific humidity, and temperature are also improved to some extent. Sensitivity experiments show that the microphysics scheme is moderately sensitive to model vertical resolution, updraft vertical velocity, and numerics, but less so to the lower boundary conditions of hydrometeor budget equations. The experiments with climatological aerosol distribution show that convective precipitation is suppressed with increasing aerosol amount, consistent with some available observations.

Journal ArticleDOI
TL;DR: In this paper, two additional morphological parameters of the radar Doppler spectrum, the skewness and kurtosis, were introduced to reduce the retrieval uncertainties of cloud microphysical and dynamical properties.
Abstract: [1] Several aspects of spectral broadening and drizzle growth in shallow liquid clouds remain not well understood. Detailed, cloud-scale observations of microphysics and dynamics are essential to guide and evaluate corresponding modeling efforts. Profiling, millimeter-wavelength (cloud) radars can provide such observations. In particular, the first three moments of the recorded cloud radar Doppler spectra, the radar reflectivity, mean Doppler velocity, and spectrum width, are often used to retrieve cloud microphysical and dynamical properties. Such retrievals are subject to errors introduced by the assumptions made in the inversion process. Here, we introduce two additional morphological parameters of the radar Doppler spectrum, the skewness and kurtosis, in an effort to reduce the retrieval uncertainties. A forward model that emulates observed radar Doppler spectra is constructed and used to investigate these relationships. General, analytical relationships that relate the five radar observables to cloud and drizzle microphysical parameters and cloud turbulence are presented. The relationships are valid for cloud-only, cloud mixed with drizzle, and drizzle-only particles in the radar sampling volume and provide a seamless link between observations and cloud microphysics and dynamics. The sensitivity of the five observed parameters to the radar operational parameters such as signal-to-noise ratio and Doppler spectra velocity resolution are presented. The predicted values of the five observed radar parameters agree well with the output of the forward model. The novel use of the skewness of the radar Doppler spectrum as an early qualitative predictor of drizzle onset in clouds is introduced. It is found that skewness is a parameter very sensitive to early drizzle generation. In addition, the significance of the five parameters of the cloud radar Doppler spectrum for constraining drizzle microphysical retrievals is discussed.

Journal ArticleDOI
TL;DR: In this article, the authors used a three-dimensional general circulation model with sulfur chemistry and sectional aerosol microphysics (WACCM/CARMA) to study aerosol formation and micro-physics in the upper troposphere and lower stratosphere, as well as the middle and upper stratosphere.
Abstract: . Using a three-dimensional general circulation model with sulfur chemistry and sectional aerosol microphysics (WACCM/CARMA), we studied aerosol formation and microphysics in the upper troposphere and lower stratosphere (UTLS) as well as the middle and upper stratosphere based on three nucleation schemes (two binary homogeneous schemes and an ion-mediated scheme related to one of the binary schemes). Simulations suggest that ion-mediated nucleation rates in the UTLS are 25 % higher than its related binary scheme, but that the rates predicted by the two binary schemes vary by two orders of magnitude. None of the nucleation schemes is superior at matching the limited observations available at the smallest sizes. However, it is found that coagulation, not nucleation, controls number concentration at sizes greater than approximately 10 nm. Therefore, based on this study, processes relevant to atmospheric chemistry and radiative forcing in the UTLS are not sensitive to the choice of nucleation schemes. The dominance of coagulation over other microphysical processes in the UTLS is consistent with other recent work using microphysical models. Simulations using all three nucleation schemes compare reasonably well to observations of size distributions, number concentration across latitude, and vertical profiles of particle mixing ratio in the UTLS. Interestingly, we find that we need to include Van der Waals forces in our coagulation scheme to match the UTLS aerosol concentrations. We conclude that this model can reasonably represent sulfate microphysical processes in the UTLS, and that the properties of particles at atmospherically relevant sizes appear to be insensitive to the details of the nucleation scheme. We also suggest that micrometeorites, which are not included in this model, dominate the aerosol properties in the upper stratosphere above about 30 km.

Journal ArticleDOI
TL;DR: In this paper, the effects of clouds on aerosols are treated by using an explicit cloud parameterized-pollutant (ECPP) approach that links aerosol and chemical processes on the large-scale grid with statistics of cloud properties and processes resolved by the CRM.
Abstract: . Anthropogenic aerosol effects on climate produce one of the largest uncertainties in estimates of radiative forcing of past and future climate change. Much of this uncertainty arises from the multi-scale nature of the interactions between aerosols, clouds and large-scale dynamics, which are difficult to represent in conventional general circulation models (GCMs). In this study, we develop a multi-scale aerosol-climate model that treats aerosols and clouds across different scales, and evaluate the model performance, with a focus on aerosol treatment. This new model is an extension of a multi-scale modeling framework (MMF) model that embeds a cloud-resolving model (CRM) within each grid column of a GCM. In this extension, the effects of clouds on aerosols are treated by using an explicit-cloud parameterized-pollutant (ECPP) approach that links aerosol and chemical processes on the large-scale grid with statistics of cloud properties and processes resolved by the CRM. A two-moment cloud microphysics scheme replaces the simple bulk microphysics scheme in the CRM, and a modal aerosol treatment is included in the GCM. With these extensions, this multi-scale aerosol-climate model allows the explicit simulation of aerosol and chemical processes in both stratiform and convective clouds on a global scale. Simulated aerosol budgets in this new model are in the ranges of other model studies. Simulated gas and aerosol concentrations are in reasonable agreement with observations (within a factor of 2 in most cases), although the model underestimates black carbon concentrations at the surface by a factor of 2–4. Simulated aerosol size distributions are in reasonable agreement with observations in the marine boundary layer and in the free troposphere, while the model underestimates the accumulation mode number concentrations near the surface, and overestimates the accumulation mode number concentrations in the middle and upper free troposphere by a factor of about 2. The overestimation of accumulation model number concentrations in the middle and upper free troposphere is consistent with large aerosol mass fraction above 5 km in the MMF model compared with other models. Simulated cloud condensation nuclei (CCN) concentrations are within the observational variations. Simulated aerosol optical depths (AOD) are in reasonable agreement with observations (within a factor of 2), and the spatial distribution of AOD is consistent with observations, while the model underestimates AOD over regions with strong fossil fuel and biomass burning emissions. Overall, this multi-scale aerosol-climate model simulates aerosol fields as well as conventional aerosol models.

Journal ArticleDOI
TL;DR: In this paper, the Rutledge and Hobbs-based bulk microphysics scheme in the Goddard Cumulus Ensemble model is modified to reduce the bias of reflectivity values in the middle and upper troposphere in simulated convective systems.
Abstract: A well-known bias common to many bulk microphysics schemes currently being used in cloud-resolving models is the tendency to produce excessively large reflectivity values (e.g., 40 dBZ) in the middle and upper troposphere in simulated convective systems. The Rutledge and Hobbs–based bulk microphysics scheme in the Goddard Cumulus Ensemble model is modified to reduce this bias and improve realistic aspects. Modifications include lowering the efficiencies for snow/graupel riming and snow accreting cloud ice; converting less rimed snow to graupel; allowing snow/graupel sublimation; adding rime splintering, immersion freezing, and contact nucleation; replacing the Fletcher formulation for activated ice nuclei with that of Meyers et al.; allowing for ice supersaturation in the saturation adjustment; accounting for ambient RH in the growth of cloud ice to snow; and adding/accounting for cloud ice fall speeds. In addition, size-mapping schemes for snow/graupel were added as functions of temperature and m...

Journal ArticleDOI
TL;DR: In this article, a technique that allows for the discrimination between low stratus and (ground) fog on the basis of geostationary satellite imagery is introduced. But the performance of this technique is shown to be good in a comparison with METeorological Aerodrome Report data comprising 1030 satellite scenes.
Abstract: The detection of ground fog from satellite data is of interest in operational nowcasting applications, as well as in studies of the climate system. A discrimination between fog at the ground and other low-stratus situations from satellite data requires information on cloud vertical geometry to establish whether the cloud touches the ground. This article introduces a technique that allows for the discrimination between low stratus and (ground) fog on the basis of geostationary satellite imagery. The cloud-base height is derived using a subadiabatic model of cloud microphysics. In this model, the cloud base is varied until model liquid-water path matches that retrieved from satellite data. The performance of this technique is shown to be good in a comparison with METeorological Aerodrome Report data comprising 1030 satellite scenes. With a hit rate of 81% and a threat score of 0.62, the skill is satisfactory.

Journal ArticleDOI
TL;DR: The CLAIM-3D (3Dimensional Cloud Aerosol Interaction Mission) satellite concept proposed by as mentioned in this paper combines several techniques to simultaneously measure the vertical profile of cloud microphysics, thermodynamic phase, brightness temperature, and aerosol amount and type in the neighborhood of the clouds.
Abstract: . Cloud-aerosol interaction is a key issue in the climate system, affecting the water cycle, the weather, and the total energy balance including the spatial and temporal distribution of latent heat release. Information on the vertical distribution of cloud droplet microphysics and thermodynamic phase as a function of temperature or height, can be correlated with details of the aerosol field to provide insight on how these particles are affecting cloud properties and their consequences to cloud lifetime, precipitation, water cycle, and general energy balance. Unfortunately, today's experimental methods still lack the observational tools that can characterize the true evolution of the cloud microphysical, spatial and temporal structure in the cloud droplet scale, and then link these characteristics to environmental factors and properties of the cloud condensation nuclei. Here we propose and demonstrate a new experimental approach (the cloud scanner instrument) that provides the microphysical information missed in current experiments and remote sensing options. Cloud scanner measurements can be performed from aircraft, ground, or satellite by scanning the side of the clouds from the base to the top, providing us with the unique opportunity of obtaining snapshots of the cloud droplet microphysical and thermodynamic states as a function of height and brightness temperature in clouds at several development stages. The brightness temperature profile of the cloud side can be directly associated with the thermodynamic phase of the droplets to provide information on the glaciation temperature as a function of different ambient conditions, aerosol concentration, and type. An aircraft prototype of the cloud scanner was built and flew in a field campaign in Brazil. The CLAIM-3D (3-Dimensional Cloud Aerosol Interaction Mission) satellite concept proposed here combines several techniques to simultaneously measure the vertical profile of cloud microphysics, thermodynamic phase, brightness temperature, and aerosol amount and type in the neighborhood of the clouds. The wide wavelength range, and the use of multi-angle polarization measurements proposed for this mission allow us to estimate the availability and characteristics of aerosol particles acting as cloud condensation nuclei, and their effects on the cloud microphysical structure. These results can provide unprecedented details on the response of cloud droplet microphysics to natural and anthropogenic aerosols in the size scale where the interaction really happens.

Journal ArticleDOI
TL;DR: In this paper, the authors introduce the new aerosol microphysics submodel MADE-in, implemented within the ECHAM/MESSy Atmospheric Chemistry global model (EMAC).
Abstract: . Black carbon (BC) and mineral dust are among the most abundant insoluble aerosol components in the atmosphere. When released, most BC and dust particles are externally mixed with other aerosol species. Through coagulation with particles containing soluble material and condensation of gases, the externally mixed particles may obtain a liquid coating and be transferred into an internal mixture. The mixing state of BC and dust aerosol particles influences their radiative and hygroscopic properties, as well as their ability of forming ice crystals. We introduce the new aerosol microphysics submodel MADE-in, implemented within the ECHAM/MESSy Atmospheric Chemistry global model (EMAC). MADE-in is able to track mass and number concentrations of BC and dust particles in their different mixing states, as well as particles free of BC and dust. MADE-in describes these three classes of particles through a superposition of seven log-normally distributed modes, and predicts the evolution of their size distribution and chemical composition. Six out of the seven modes are mutually interacting, allowing for the transfer of mass and number among them. Separate modes for the different mixing states of BC and dust particles in EMAC/MADE-in allow for explicit simulations of the relevant aging processes, i.e. condensation, coagulation and cloud processing. EMAC/MADE-in has been evaluated with surface and airborne measurements and mostly performs well both in the planetary boundary layer and in the upper troposphere and lowermost stratosphere.

Journal ArticleDOI
TL;DR: In this article, the authors focused on low-level, liquid-dominated clouds in two separate regimes with respect to cloud and aerosol properties: single-layer stratocumulus with below-cloud aerosol concentrations (Na) less than 250 cm−3 (clean cases); and layered stratocummulus with Na > 500 cm−1 below cloud base, associated with a biomass burning aerosol (polluted cases).
Abstract: [1] Aircraft measurements during the Indirect and Semi-Direct Aerosol Campaign (ISDAC) in April 2008 are used to investigate factors influencing the microphysics and radiative properties of springtime Arctic clouds. The analysis is focused on low-level, liquid-dominated clouds in two separate regimes with respect to cloud and aerosol properties: single-layer stratocumulus with below-cloud aerosol concentrations (Na) less than 250 cm−3 (clean cases); and layered stratocumulus with Na > 500 cm−3 below cloud base, associated with a biomass burning aerosol (polluted cases). For each regime, vertical profiles through cloud are used to determine cloud microphysical and radiative properties. The polluted cases were correlated with warmer, geometrically thicker clouds, with higher droplet number concentrations (Nd), liquid water paths (LWP), optical depths (τ), and albedo (A) relative to clean cases. The mean cloud droplet effective radii (reff), however, were similar (5.7 μm) for both aerosol-cloud regimes. This discrepancy resulted mainly from the higher LWP of clouds in polluted cases, which can be explained by both meteorological (temperature, dynamics) and microphysical (precipitation inhibition) factors. Adiabatic parcel model simulations demonstrate that differences in droplet activation between the aerosol-cloud regimes may play a role, as the higher Na in polluted cases limits activation to larger and/or more hygroscopic particles. The observations and analysis presented here demonstrate the complex interactions among environmental conditions, aerosol, and the microphysics and radiative properties of Arctic clouds.

Journal ArticleDOI
TL;DR: In this article, a 2D video disdrometer was deployed about 30 km from a polarimetric weather radar in Norman, Oklahoma, to observe winter precipitation events during the 2006/07 winter season.
Abstract: The study of precipitation in different phases is important to understanding the physical processes that occur in storms, as well as to improving their representation in numerical weather prediction models. A 2D video disdrometer was deployed about 30 km from a polarimetric weather radar in Norman, Oklahoma, (KOUN) to observe winter precipitation events during the 2006/07 winter season. These events contained periods of rain, snow, and mixed-phase precipitation. Five-minute particle size distributions were generated from the disdrometer data and fitted to a gamma distribution; polarimetric radar variables were also calculated for comparison with KOUN data. It is found that snow density adjustment improves the comparison substantially, indicating the importance of accounting for the density variability in representing model microphysics.

Journal ArticleDOI
TL;DR: In this article, the authors extended the previous cloud-resolving modeling study concerning the impact of cloud microphysics on convective-radiative quasi equilibrium (CRQE) over a surface with fixed characteristics and prescribed solar input, both mimicking the mean conditions on earth.
Abstract: This paper extends the previous cloud-resolving modeling study concerning the impact of cloud microphysics on convective–radiative quasi equilibrium (CRQE) over a surface with fixed characteristics and prescribed solar input, both mimicking the mean conditions on earth. The current study applies sophisticated double-moment warm-rain and ice microphysics schemes, which allow for a significantly more realistic representation of the impact of aerosols on precipitation processes and on the coupling between clouds and radiative transfer. Two contrasting cloud condensation nuclei (CCN) characteristics are assumed, representing pristine and polluted conditions, as well as contrasting representations of the effects of entrainment and mixing on the mean cloud droplet size. In addition, four sets of sensitivity simulations are also performed with changes that provide a reference for the main simulation set.As in the previous study, the CRQE mimics the estimates of globally and annually averaged water and en...

Journal ArticleDOI
TL;DR: In this article, an improved bin warm-rain microphysics scheme was proposed that applies the Twomey approach to represent CCN activation, which relates the concentration of activated droplets to the maximum supersaturation experienced by the air parcel during activation.

Journal ArticleDOI
TL;DR: In this paper, an algorithm is presented to generate realistic ice crystals and their aggregates from which radar backscattering cross sections may be calculated using a generalized solution for a cluster of spheres.
Abstract: [1] Arctic clouds are often mixed-phase, such that the radiative properties of the clouds are a strong function of the relative amounts of cloud liquid and ice. Modeling studies have shown that the poorly understood ice phase processes are the regulators of the liquid water fraction. However, evaluating the fidelity of the model ice parameterizations has proven to be a difficult task. This study evaluates results of different ice microphysics representations in a cloud resolving model (CRM) using cloud radar measurements. An algorithm is presented to generate realistic ice crystals and their aggregates from which radar backscattering cross sections may be calculated using a generalized solution for a cluster of spheres. The aggregate is composed of a collection of ice crystals, each of which is constructed from a cluster of tiny ice spheres. Each aggregate satisfies the constraints set by the component crystal type and the mass-dimensional relationship used in the cloud resolving model, but is free to adjust its aspect ratio. This model for calculating radar backscattering is compared to two spherical and two spheroidal (bulk model) representations for ice hydrometeors. It was found that a refined model for representing the ice hydrometeors, both pristine crystals and their aggregates, is required in order to obtain good comparisons between the CRM calculations and the radar measurements. The addition of the radar-CRM comparisons to CRM-in situ measurements comparisons allowed conclusions about the appropriateness of different CRM ice microphysics parameterizations.

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TL;DR: The authors explored the transition from maritime to continental convection by comparing the trends in Tropical Rainfall Measuring Mission (TRMM) radar and microwave (37 and 85 GHz) observations over islands of increasing size to those simulated by a cloud-resolving model.
Abstract: Moist convection is well known to be generally more intense over continental than maritime regions, with larger updraft velocities, graupel, and lightning production. This study explores the transition from maritime to continental convection by comparing the trends in Tropical Rainfall Measuring Mission (TRMM) radar and microwave (37 and 85 GHz) observations over islands of increasing size to those simulated by a cloudresolving model. The observed storms were essentially maritime over islands of ,100 km 2 and continental over islands .10 000 km 2 , with a gradual transition in between. Equivalent radar and microwave quantities were simulated from cloud-resolving runs of the Weather Research andForecasting model viaofflineradiation codes. The model configuration wasidealized,with islands represented by regions of uniform surface heat flux without orography, using a range of initial sounding conditions without strong horizontal winds or aerosols. Simulated storm strength varied with initial sounding, as expected, but also increased sharply with island size in a manner similar to observations. Stronger simulated storms were associated with higher concentrations of large hydrometeors. Although biases varied with different ice microphysical schemes, the trend was similar for all three schemes tested and was also seen in 2D and 3D model configurations. The successful reproduction of the trend with such idealized forcing supports previous suggestions that mesoscale variation in surface heating—rather than any difference in humidity, aerosol, or other aspects of the atmospheric state—is the main reason that convection is more intense over continents and large islands than over oceans. Some dynamical storm aspects, notably the peak rainfall and minimum surface pressure low, were more sensitive to surface forcing than to the atmospheric sounding or ice scheme. Large hydrometeor concentrations and simulated microwave and radar signatures, however, were at least as sensitive to initial humidity levels as to surface forcing and were more sensitive to the ice scheme. IssueswithrunningtheTRMMsimulatoron2Dsimulationsarediscussed,buttheyappeartobelessserious than sensitivities to model microphysics, which were similar in 2D and 3D. This supportsthe furtheruse of 2D simulations to economically explore modeling uncertainties.

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TL;DR: In this article, the authors improved on the lidar and radar retrieval algorithm developed by Okamoto et al. to extend the applicability of the microphysical retrieval scheme from the cloud region with lidar-radar overlap to lidar or radar-only cloud regions with an available radar-lidar overlap area in the vertical profile by use of the Levenberg-Marqardt method.
Abstract: [1] This work improved on the lidar and radar retrieval algorithm developed by Okamoto et al. to extend the applicability of the microphysical retrieval scheme from the cloud region with lidar-radar overlap to lidar- or radar-only cloud regions with an available radar-lidar overlap area in the vertical profile by use of the Levenberg-Marqardt method. The algorithm was formulated to efficiently reflect the information from the lidar-radar overlap region to the microphysical retrieval at the radar- or lidar-only region to avoid the use of a prescribed parameterization among the observables and cloud microphysics. The algorithm incorporated particle-type discrimination before the microphysical retrieval, consistent with the theoretical treatment of two-dimensional (2-D) and three-dimensional (3-D) ice particle mixtures in the radar and lidar forward models and the combined use of three observables (the radar reflectivity Ze, the lidar backscattering coefficient β, and the depolarization ratio δ) for the lidar- or radar-only cloud regimes. A full one-to-one comparison of the retrieved microphysical properties with the results of the previous algorithm revealed that reff could be retrieved consistently within about 10% uncertainty, on average. The ice water content (IWC) retrieval also performed well, except for extreme cases, and the uncertainties of IWC as well as reff were within about 40% for the radar-only region, despite the depth of the radar-only cloud layers. When considering only the cloud region with lidar-radar overlap, the zonal mean profiles of reff may be slightly larger and IWC may be slightly smaller when considering attenuation caused by the lidar-only region, which occasionally occurs above the region of lidar-radar overlap.

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TL;DR: In this article, the Weather Research and Forecasting model (WRF) is used at high resolution to simulate this extreme weather event and the model results indicate that WRF is able to capture the amount and location of the observed surface rainfall and that the typhoon-induced circulation, orographic lifting and a moisture-abundant southwest flow are the main mechanisms that together produced the tremendous rainfall in this case.
Abstract: Typhoon Morakot hit Taiwan the night of 7 August 2009 as a Category 1 storm and caused up to 3000 mm of rain, leadingto the worst flooding there in 50 years as well as devastating mudslides. The Weather Research and Forecasting model(WRF) is used at high resolution to simulate this extreme weather event. The model results indicate that WRF is able to capture the amount and location of the observed surface rainfall and that the typhoon-induced circulation, orographic lifting and a moisture-abundant southwest flow are the main mechanisms that together produced the tremendous rainfall in this case. Furthermore, the model results suggest that the agreement with the observed rainfall is due to the simulated storm track and intensity being in relatively good agreement with the observed. Additional simulations were made to examine the sensitivity of this case to model physics (microphysics and planetary boundary layer or PBL). Both warm rain only as well as improvedmicrophysics yield similar significant rain amounts at the same locations as the control case. The improved microphysics lead to a better storm intensity early on but later exceed the observed intensities by about 10 hPa. The stronger storm arises from less evaporative cooling from cloud and rain and consequently weaker simulated downdrafts. Warm rain results closely match the control (i.e., the track, intensity, and maximum rainfall locations/amounts), implying ice processes (i.e., additional heat release due to ice processes) have only a secondary effect on surface rainfall. Results are less sensitive to using different PBL schemes than different microphysics.

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TL;DR: In this article, a parameterization based on multi-variate probability density functions with dynamics (MVD PDFs) has been incorporated into the single-column version of GFDL AM3, extended to treat aerosol activation, and coupled with a two-moment microphysics scheme.
Abstract: [1] Successful simulation of aerosol indirect effects in climate models requires parameterizations that capture the full range of cloud-aerosol interactions, including positive and negative liquid water path (LWP) responses to increasing aerosol concentrations, as suggested by large eddy simulations (LESs). A parameterization based on multi-variate probability density functions with dynamics (MVD PDFs) has been incorporated into the single-column version of GFDL AM3, extended to treat aerosol activation, and coupled with a two-moment microphysics scheme. We use it to explore cloud-aerosol interactions. In agreement with LESs, our single-column simulations produce both positive and negative LWP responses to increasing aerosol concentrations, depending on precipitation and free atmosphere relative humidity. We have conducted sensitivity tests to vertical resolution and droplet sedimentation parameterization. The dependence of sedimentation on cloud droplet size is essential to capture the full LWP responses to aerosols. Further analyses reveal that the MVD PDFs are able to represent changes in buoyancy profiles induced by sedimentation as well as enhanced entrainment efficiency with aerosols comparable to LESs.

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TL;DR: In this article, the effect of sea spray on the thermodynamics and microphysical structure of the lowest 400m layer under strong wind speeds is investigated using a 2D hybrid Lagrangian-Eulerian model with spectral bin microphysics.
Abstract: The effect of sea spray on the thermodynamics and microphysical structure of the lowest 400-m layer under strong wind speeds is investigated using a 2D hybrid Lagrangian–Eulerian model with spectral bin microphysics. A large number of adjacent and interacting Lagrangian parcels move within a turbulent-like flow with the largest vortices being interpreted as large eddies (LE) with characteristic velocity of a few meters per second.It is shown that sea spray effect strongly depends on the environmental conditions, and largely on relative humidity (RH). When RH ~90% the effects of spray on the BL thermodynamics substantially decrease. Spray leads to formation of drizzle by collisions with droplets formed on background aerosols.It is also shown that LE transport about 20% of large spray drops with radius exceeding 150 μm to the upper levels of the atmospheric...

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TL;DR: In this paper, the authors compared capacitance theory with measurements from three independent laboratory studies and found that the predicted growth rates are consistent with the measured values to within about 20% in 14 of the experiments analyzed, over the temperature range −2.5° to −22°C.
Abstract: The physical and empirical relationships used by microphysics schemes to control the rate at which vapor is transferred to ice crystals growing in supercooled clouds are compared with laboratory data to evaluate the realism of various model formulations.Ice crystal growth rates predicted from capacitance theory are compared with measurements from three independent laboratory studies. When the growth is diffusion- limited, the predicted growth rates are consistent with the measured values to within about 20% in 14 of the experiments analyzed, over the temperature range −2.5° to −22°C. Only two experiments showed significant disagreement with theory (growth rate overestimated by about 30%–40% at −3.7° and −10.6°C).Growth predictions using various ventilation factor parameterizations were also calculated and compared with supercooled wind tunnel data. It was found that neither of the standard parameterizations used for ventilation adequately described both needle and dendrite growth; however, by choo...

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TL;DR: In this article, the authors analyzed coincident multisatellite and in situ aircraft measurements of three mixed-phase cloud cases during an intensive field experiment (C3VP/CLEX-10) to better understand the microphysics and radiative properties and provide a foundation for the improvement of the satellite retrieval algorithms for these clouds.
Abstract: [1] This work presents a study of midlevel, mixed-phase clouds using satellite (remote sensing) and aircraft (in situ) observations. In this study, we analyze coincident multisatellite and in situ aircraft measurements of three mixed-phase cloud cases during an intensive field experiment (C3VP/CLEX-10) to better understand the microphysics and radiative properties and provide a foundation for the improvement of the satellite retrieval algorithms for these clouds. For the selected cases, various aspects observed from different instruments are presented and compared for these clouds. It is found that many areas in the Moderate Resolution Imaging Spectroradiometer (MODIS) cloud phase product classified as “unknown” are more appropriately classified as “mixed phase” based on CloudSat and CALIPSO data as well as C3VP/CLEX-10 aircraft measurements. The aircraft measurements show that a significant amount of supercooled liquid water exists at or near cloud top at very low temperatures for these midlevel, mixed-phase clouds, contrary to the assumptions used in the CloudSat retrieval algorithms. The spatial distribution of liquid water content and ice water content and other cloud properties are examined for both the satellite remote sensing and in situ probe measurements. CloudSat and airborne radar reflectivity data are also compared through a structure function analysis. Radiative transfer simulations based on the aircraft and satellite observations indicate the importance of proper assignment of cloud phase within retrieval algorithms and numerical models, which use similar assumptions.